Cargando…

Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure

A time-dependent two-dimensional (2D) axisymmetric simulation was conducted for arc plasma with dynamically fluctuating fluid generating iron nanoparticles in a direct-current discharge condition. The nonequilibrium process of simultaneous growth and transport of nanoparticles is simulated using a s...

Descripción completa

Detalles Bibliográficos
Autores principales: Shigeta, Masaya, Tanaka, Manabu, Ghedini, Emanuele
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2019
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6956131/
https://www.ncbi.nlm.nih.gov/pubmed/31817612
http://dx.doi.org/10.3390/nano9121736
_version_ 1783487089437835264
author Shigeta, Masaya
Tanaka, Manabu
Ghedini, Emanuele
author_facet Shigeta, Masaya
Tanaka, Manabu
Ghedini, Emanuele
author_sort Shigeta, Masaya
collection PubMed
description A time-dependent two-dimensional (2D) axisymmetric simulation was conducted for arc plasma with dynamically fluctuating fluid generating iron nanoparticles in a direct-current discharge condition. The nonequilibrium process of simultaneous growth and transport of nanoparticles is simulated using a simple model with a low computational cost. To ascertain fluid dynamic instability and steep gradients in plasma temperature and particle distributions, a highly accurate method is adopted for computation. The core region of the arc plasma is almost stationary, whereas the fringe fluctuates because of fluid dynamic instability between the arc plasma and the shielding gas. In the downstream region, the vapor molecules decrease by condensation. The nanoparticles decrease by coagulation. These results suggest that both of the simultaneous processes make important contributions to particle growth. The fluctuation of nanoparticle number density in a distant region exhibits stronger correlation with the temperature fluctuation at the plasma fringe. The correlation analysis results suggest that the distribution of growing nanoparticles distant from the arc plasma can be controlled via control of temperature fluctuation at the arc plasma fringe.
format Online
Article
Text
id pubmed-6956131
institution National Center for Biotechnology Information
language English
publishDate 2019
publisher MDPI
record_format MEDLINE/PubMed
spelling pubmed-69561312020-01-23 Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure Shigeta, Masaya Tanaka, Manabu Ghedini, Emanuele Nanomaterials (Basel) Article A time-dependent two-dimensional (2D) axisymmetric simulation was conducted for arc plasma with dynamically fluctuating fluid generating iron nanoparticles in a direct-current discharge condition. The nonequilibrium process of simultaneous growth and transport of nanoparticles is simulated using a simple model with a low computational cost. To ascertain fluid dynamic instability and steep gradients in plasma temperature and particle distributions, a highly accurate method is adopted for computation. The core region of the arc plasma is almost stationary, whereas the fringe fluctuates because of fluid dynamic instability between the arc plasma and the shielding gas. In the downstream region, the vapor molecules decrease by condensation. The nanoparticles decrease by coagulation. These results suggest that both of the simultaneous processes make important contributions to particle growth. The fluctuation of nanoparticle number density in a distant region exhibits stronger correlation with the temperature fluctuation at the plasma fringe. The correlation analysis results suggest that the distribution of growing nanoparticles distant from the arc plasma can be controlled via control of temperature fluctuation at the arc plasma fringe. MDPI 2019-12-06 /pmc/articles/PMC6956131/ /pubmed/31817612 http://dx.doi.org/10.3390/nano9121736 Text en © 2019 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Shigeta, Masaya
Tanaka, Manabu
Ghedini, Emanuele
Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title_full Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title_fullStr Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title_full_unstemmed Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title_short Numerical Analysis of the Correlation between Arc Plasma Fluctuation and Nanoparticle Growth–Transport under Atmospheric Pressure
title_sort numerical analysis of the correlation between arc plasma fluctuation and nanoparticle growth–transport under atmospheric pressure
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6956131/
https://www.ncbi.nlm.nih.gov/pubmed/31817612
http://dx.doi.org/10.3390/nano9121736
work_keys_str_mv AT shigetamasaya numericalanalysisofthecorrelationbetweenarcplasmafluctuationandnanoparticlegrowthtransportunderatmosphericpressure
AT tanakamanabu numericalanalysisofthecorrelationbetweenarcplasmafluctuationandnanoparticlegrowthtransportunderatmosphericpressure
AT ghediniemanuele numericalanalysisofthecorrelationbetweenarcplasmafluctuationandnanoparticlegrowthtransportunderatmosphericpressure