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Attosecond optoelectronic field measurement in solids

The sub-cycle interaction of light and matter is one of the key frontiers of inquiry made accessible by attosecond science. Here, we show that when light excites a pair of charge carriers inside of a solid, the transition probability is strongly localized to instants slightly after the extrema of th...

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Autores principales: Sederberg, Shawn, Zimin, Dmitry, Keiber, Sabine, Siegrist, Florian, Wismer, Michael S., Yakovlev, Vladislav S., Floss, Isabella, Lemell, Christoph, Burgdörfer, Joachim, Schultze, Martin, Krausz, Ferenc, Karpowicz, Nicholas
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6976600/
https://www.ncbi.nlm.nih.gov/pubmed/31969568
http://dx.doi.org/10.1038/s41467-019-14268-x
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author Sederberg, Shawn
Zimin, Dmitry
Keiber, Sabine
Siegrist, Florian
Wismer, Michael S.
Yakovlev, Vladislav S.
Floss, Isabella
Lemell, Christoph
Burgdörfer, Joachim
Schultze, Martin
Krausz, Ferenc
Karpowicz, Nicholas
author_facet Sederberg, Shawn
Zimin, Dmitry
Keiber, Sabine
Siegrist, Florian
Wismer, Michael S.
Yakovlev, Vladislav S.
Floss, Isabella
Lemell, Christoph
Burgdörfer, Joachim
Schultze, Martin
Krausz, Ferenc
Karpowicz, Nicholas
author_sort Sederberg, Shawn
collection PubMed
description The sub-cycle interaction of light and matter is one of the key frontiers of inquiry made accessible by attosecond science. Here, we show that when light excites a pair of charge carriers inside of a solid, the transition probability is strongly localized to instants slightly after the extrema of the electric field. The extreme temporal localization is utilized in a simple electronic circuit to record the waveforms of infrared to ultraviolet light fields. This form of petahertz-bandwidth field metrology gives access to both the modulated transition probability and its temporal offset from the laser field, providing sub-fs temporal precision in reconstructing the sub-cycle electronic response of a solid state structure.
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spelling pubmed-69766002020-01-24 Attosecond optoelectronic field measurement in solids Sederberg, Shawn Zimin, Dmitry Keiber, Sabine Siegrist, Florian Wismer, Michael S. Yakovlev, Vladislav S. Floss, Isabella Lemell, Christoph Burgdörfer, Joachim Schultze, Martin Krausz, Ferenc Karpowicz, Nicholas Nat Commun Article The sub-cycle interaction of light and matter is one of the key frontiers of inquiry made accessible by attosecond science. Here, we show that when light excites a pair of charge carriers inside of a solid, the transition probability is strongly localized to instants slightly after the extrema of the electric field. The extreme temporal localization is utilized in a simple electronic circuit to record the waveforms of infrared to ultraviolet light fields. This form of petahertz-bandwidth field metrology gives access to both the modulated transition probability and its temporal offset from the laser field, providing sub-fs temporal precision in reconstructing the sub-cycle electronic response of a solid state structure. Nature Publishing Group UK 2020-01-22 /pmc/articles/PMC6976600/ /pubmed/31969568 http://dx.doi.org/10.1038/s41467-019-14268-x Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Sederberg, Shawn
Zimin, Dmitry
Keiber, Sabine
Siegrist, Florian
Wismer, Michael S.
Yakovlev, Vladislav S.
Floss, Isabella
Lemell, Christoph
Burgdörfer, Joachim
Schultze, Martin
Krausz, Ferenc
Karpowicz, Nicholas
Attosecond optoelectronic field measurement in solids
title Attosecond optoelectronic field measurement in solids
title_full Attosecond optoelectronic field measurement in solids
title_fullStr Attosecond optoelectronic field measurement in solids
title_full_unstemmed Attosecond optoelectronic field measurement in solids
title_short Attosecond optoelectronic field measurement in solids
title_sort attosecond optoelectronic field measurement in solids
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6976600/
https://www.ncbi.nlm.nih.gov/pubmed/31969568
http://dx.doi.org/10.1038/s41467-019-14268-x
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