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Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells

We studied mechanisms of recombination in InGaN quantum wells in polar and semipolar structures. Photoluminescence measurements show that the optical emission linewidths for polar and semipolar structures are almost identical suggesting the same level of indium fluctuations in quanutm wells. Their “...

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Autores principales: Marona, Lucja, Schiavon, Dario, Baranowski, Michał, Kudrawiec, Robert, Gorczyca, Iza, Kafar, Anna, Perlin, Piotr
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6985216/
https://www.ncbi.nlm.nih.gov/pubmed/31988430
http://dx.doi.org/10.1038/s41598-020-58295-x
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author Marona, Lucja
Schiavon, Dario
Baranowski, Michał
Kudrawiec, Robert
Gorczyca, Iza
Kafar, Anna
Perlin, Piotr
author_facet Marona, Lucja
Schiavon, Dario
Baranowski, Michał
Kudrawiec, Robert
Gorczyca, Iza
Kafar, Anna
Perlin, Piotr
author_sort Marona, Lucja
collection PubMed
description We studied mechanisms of recombination in InGaN quantum wells in polar and semipolar structures. Photoluminescence measurements show that the optical emission linewidths for polar and semipolar structures are almost identical suggesting the same level of indium fluctuations in quanutm wells. Their “peak-energy-versus-temperature” relations demonstrate very pronounced “s-shape” effect. Emission linewidth measured by cathodoluminescence does not depend on area from which the light is collected meaning that the fluctuations are smaller that 100 nm. The time scale of recombination process are of the order of 80 ns for polar and 2 ns for semipolar. Energy dispersion of the recombination time is strong in polar structures and very weak in semipolar ones which can be interperted in terms of electric field influence on photoluminescence lifetime energy dispersion. At room temparture emmission is dominated by Schockley-Hall-Read recombination and does not show any dispersion. Rate equation analysis of photoluminescence transients show domination of excitonic recombination in the case of polar samples (low temperature) and bimolecular in the case of semipolar ones. Both types of quantum wells, polar and semipolar look similar from the point of view of localization but differ in their radiative recombination mechanisms.
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spelling pubmed-69852162020-01-31 Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells Marona, Lucja Schiavon, Dario Baranowski, Michał Kudrawiec, Robert Gorczyca, Iza Kafar, Anna Perlin, Piotr Sci Rep Article We studied mechanisms of recombination in InGaN quantum wells in polar and semipolar structures. Photoluminescence measurements show that the optical emission linewidths for polar and semipolar structures are almost identical suggesting the same level of indium fluctuations in quanutm wells. Their “peak-energy-versus-temperature” relations demonstrate very pronounced “s-shape” effect. Emission linewidth measured by cathodoluminescence does not depend on area from which the light is collected meaning that the fluctuations are smaller that 100 nm. The time scale of recombination process are of the order of 80 ns for polar and 2 ns for semipolar. Energy dispersion of the recombination time is strong in polar structures and very weak in semipolar ones which can be interperted in terms of electric field influence on photoluminescence lifetime energy dispersion. At room temparture emmission is dominated by Schockley-Hall-Read recombination and does not show any dispersion. Rate equation analysis of photoluminescence transients show domination of excitonic recombination in the case of polar samples (low temperature) and bimolecular in the case of semipolar ones. Both types of quantum wells, polar and semipolar look similar from the point of view of localization but differ in their radiative recombination mechanisms. Nature Publishing Group UK 2020-01-27 /pmc/articles/PMC6985216/ /pubmed/31988430 http://dx.doi.org/10.1038/s41598-020-58295-x Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Marona, Lucja
Schiavon, Dario
Baranowski, Michał
Kudrawiec, Robert
Gorczyca, Iza
Kafar, Anna
Perlin, Piotr
Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title_full Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title_fullStr Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title_full_unstemmed Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title_short Kinetics of the radiative and nonradiative recombination in polar and semipolar InGaN quantum wells
title_sort kinetics of the radiative and nonradiative recombination in polar and semipolar ingan quantum wells
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC6985216/
https://www.ncbi.nlm.nih.gov/pubmed/31988430
http://dx.doi.org/10.1038/s41598-020-58295-x
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