Cargando…
Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen r...
Autores principales: | , , , , , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2020
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7055244/ https://www.ncbi.nlm.nih.gov/pubmed/32132527 http://dx.doi.org/10.1038/s41467-020-14822-y |
_version_ | 1783503334393511936 |
---|---|
author | Shen, Gurong Liu, Jing Wu, Hao Bin Xu, Pengcheng Liu, Fang Tongsh, Chasen Jiao, Kui Li, Jinlai Liu, Meilin Cai, Mei Lemmon, John P. Soloveichik, Grigorii Li, Hexing Zhu, Jian Lu, Yunfeng |
author_facet | Shen, Gurong Liu, Jing Wu, Hao Bin Xu, Pengcheng Liu, Fang Tongsh, Chasen Jiao, Kui Li, Jinlai Liu, Meilin Cai, Mei Lemmon, John P. Soloveichik, Grigorii Li, Hexing Zhu, Jian Lu, Yunfeng |
author_sort | Shen, Gurong |
collection | PubMed |
description | Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications. |
format | Online Article Text |
id | pubmed-7055244 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-70552442020-03-05 Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells Shen, Gurong Liu, Jing Wu, Hao Bin Xu, Pengcheng Liu, Fang Tongsh, Chasen Jiao, Kui Li, Jinlai Liu, Meilin Cai, Mei Lemmon, John P. Soloveichik, Grigorii Li, Hexing Zhu, Jian Lu, Yunfeng Nat Commun Article Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications. Nature Publishing Group UK 2020-03-04 /pmc/articles/PMC7055244/ /pubmed/32132527 http://dx.doi.org/10.1038/s41467-020-14822-y Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Shen, Gurong Liu, Jing Wu, Hao Bin Xu, Pengcheng Liu, Fang Tongsh, Chasen Jiao, Kui Li, Jinlai Liu, Meilin Cai, Mei Lemmon, John P. Soloveichik, Grigorii Li, Hexing Zhu, Jian Lu, Yunfeng Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title | Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title_full | Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title_fullStr | Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title_full_unstemmed | Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title_short | Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
title_sort | multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7055244/ https://www.ncbi.nlm.nih.gov/pubmed/32132527 http://dx.doi.org/10.1038/s41467-020-14822-y |
work_keys_str_mv | AT shengurong multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT liujing multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT wuhaobin multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT xupengcheng multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT liufang multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT tongshchasen multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT jiaokui multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT lijinlai multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT liumeilin multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT caimei multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT lemmonjohnp multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT soloveichikgrigorii multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT lihexing multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT zhujian multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells AT luyunfeng multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells |