Cargando…

Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells

Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen r...

Descripción completa

Detalles Bibliográficos
Autores principales: Shen, Gurong, Liu, Jing, Wu, Hao Bin, Xu, Pengcheng, Liu, Fang, Tongsh, Chasen, Jiao, Kui, Li, Jinlai, Liu, Meilin, Cai, Mei, Lemmon, John P., Soloveichik, Grigorii, Li, Hexing, Zhu, Jian, Lu, Yunfeng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7055244/
https://www.ncbi.nlm.nih.gov/pubmed/32132527
http://dx.doi.org/10.1038/s41467-020-14822-y
_version_ 1783503334393511936
author Shen, Gurong
Liu, Jing
Wu, Hao Bin
Xu, Pengcheng
Liu, Fang
Tongsh, Chasen
Jiao, Kui
Li, Jinlai
Liu, Meilin
Cai, Mei
Lemmon, John P.
Soloveichik, Grigorii
Li, Hexing
Zhu, Jian
Lu, Yunfeng
author_facet Shen, Gurong
Liu, Jing
Wu, Hao Bin
Xu, Pengcheng
Liu, Fang
Tongsh, Chasen
Jiao, Kui
Li, Jinlai
Liu, Meilin
Cai, Mei
Lemmon, John P.
Soloveichik, Grigorii
Li, Hexing
Zhu, Jian
Lu, Yunfeng
author_sort Shen, Gurong
collection PubMed
description Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications.
format Online
Article
Text
id pubmed-7055244
institution National Center for Biotechnology Information
language English
publishDate 2020
publisher Nature Publishing Group UK
record_format MEDLINE/PubMed
spelling pubmed-70552442020-03-05 Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells Shen, Gurong Liu, Jing Wu, Hao Bin Xu, Pengcheng Liu, Fang Tongsh, Chasen Jiao, Kui Li, Jinlai Liu, Meilin Cai, Mei Lemmon, John P. Soloveichik, Grigorii Li, Hexing Zhu, Jian Lu, Yunfeng Nat Commun Article Proton exchange membrane fuel cells have been regarded as the most promising candidate for fuel cell vehicles and tools. Their broader adaption, however, has been impeded by cost and lifetime. By integrating a thin layer of tungsten oxide within the anode, which serves as a rapid-response hydrogen reservoir, oxygen scavenger, sensor for power demand, and regulator for hydrogen-disassociation reaction, we herein report proton exchange membrane fuel cells with significantly enhanced power performance for transient operation and low humidified conditions, as well as improved durability against adverse operating conditions. Meanwhile, the enhanced power performance minimizes the use of auxiliary energy-storage systems and reduces costs. Scale fabrication of such devices can be readily achieved based on the current fabrication techniques with negligible extra expense. This work provides proton exchange membrane fuel cells with enhanced power performance, improved durability, prolonged lifetime, and reduced cost for automotive and other applications. Nature Publishing Group UK 2020-03-04 /pmc/articles/PMC7055244/ /pubmed/32132527 http://dx.doi.org/10.1038/s41467-020-14822-y Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Shen, Gurong
Liu, Jing
Wu, Hao Bin
Xu, Pengcheng
Liu, Fang
Tongsh, Chasen
Jiao, Kui
Li, Jinlai
Liu, Meilin
Cai, Mei
Lemmon, John P.
Soloveichik, Grigorii
Li, Hexing
Zhu, Jian
Lu, Yunfeng
Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title_full Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title_fullStr Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title_full_unstemmed Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title_short Multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
title_sort multi-functional anodes boost the transient power and durability of proton exchange membrane fuel cells
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7055244/
https://www.ncbi.nlm.nih.gov/pubmed/32132527
http://dx.doi.org/10.1038/s41467-020-14822-y
work_keys_str_mv AT shengurong multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT liujing multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT wuhaobin multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT xupengcheng multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT liufang multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT tongshchasen multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT jiaokui multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT lijinlai multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT liumeilin multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT caimei multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT lemmonjohnp multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT soloveichikgrigorii multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT lihexing multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT zhujian multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells
AT luyunfeng multifunctionalanodesboostthetransientpoweranddurabilityofprotonexchangemembranefuelcells