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Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes

In order to significantly enhance the absorption capability of solar energy absorbers in the visible wavelength region, a novel monolayer molybdenum disulfide (MoS(2))-based nanostructure was proposed. Local surface plasmon resonances (LSPRs) supported by Au nanocubes (NCs) can improve the absorptio...

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Autores principales: Li, Jiakun, Chen, Zeqiang, Yang, Hua, Yi, Zao, Chen, Xifang, Yao, Weitang, Duan, Tao, Wu, Pinghui, Li, Gongfa, Yi, Yougen
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7075212/
https://www.ncbi.nlm.nih.gov/pubmed/32024205
http://dx.doi.org/10.3390/nano10020257
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author Li, Jiakun
Chen, Zeqiang
Yang, Hua
Yi, Zao
Chen, Xifang
Yao, Weitang
Duan, Tao
Wu, Pinghui
Li, Gongfa
Yi, Yougen
author_facet Li, Jiakun
Chen, Zeqiang
Yang, Hua
Yi, Zao
Chen, Xifang
Yao, Weitang
Duan, Tao
Wu, Pinghui
Li, Gongfa
Yi, Yougen
author_sort Li, Jiakun
collection PubMed
description In order to significantly enhance the absorption capability of solar energy absorbers in the visible wavelength region, a novel monolayer molybdenum disulfide (MoS(2))-based nanostructure was proposed. Local surface plasmon resonances (LSPRs) supported by Au nanocubes (NCs) can improve the absorption of monolayer MoS(2). A theoretical simulation by a finite-difference time-domain method (FDTD) shows that the absorptions of proposed MoS(2)-based absorbers are above 94.0% and 99.7% at the resonant wavelengths of 422 and 545 nm, respectively. In addition, the optical properties of the proposed nanostructure can be tuned by the geometric parameters of the periodic Au nanocubes array, distributed Bragg mirror (DBR) and polarization angle of the incident light, which are of great pragmatic significance for improving the absorption efficiency and selectivity of monolayer MoS(2). The absorber is also able to withstand a wide range of incident angles, showing polarization-independence. Similar design ideas can also be implemented to other transition-metal dichalcogenides (TMDCs) to strengthen the interaction between light and MoS(2). This nanostructure is relatively simple to implement and has a potentially important application value in the development of high-efficiency solar energy absorbers and other optoelectronic devices.
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spelling pubmed-70752122020-03-20 Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes Li, Jiakun Chen, Zeqiang Yang, Hua Yi, Zao Chen, Xifang Yao, Weitang Duan, Tao Wu, Pinghui Li, Gongfa Yi, Yougen Nanomaterials (Basel) Article In order to significantly enhance the absorption capability of solar energy absorbers in the visible wavelength region, a novel monolayer molybdenum disulfide (MoS(2))-based nanostructure was proposed. Local surface plasmon resonances (LSPRs) supported by Au nanocubes (NCs) can improve the absorption of monolayer MoS(2). A theoretical simulation by a finite-difference time-domain method (FDTD) shows that the absorptions of proposed MoS(2)-based absorbers are above 94.0% and 99.7% at the resonant wavelengths of 422 and 545 nm, respectively. In addition, the optical properties of the proposed nanostructure can be tuned by the geometric parameters of the periodic Au nanocubes array, distributed Bragg mirror (DBR) and polarization angle of the incident light, which are of great pragmatic significance for improving the absorption efficiency and selectivity of monolayer MoS(2). The absorber is also able to withstand a wide range of incident angles, showing polarization-independence. Similar design ideas can also be implemented to other transition-metal dichalcogenides (TMDCs) to strengthen the interaction between light and MoS(2). This nanostructure is relatively simple to implement and has a potentially important application value in the development of high-efficiency solar energy absorbers and other optoelectronic devices. MDPI 2020-02-01 /pmc/articles/PMC7075212/ /pubmed/32024205 http://dx.doi.org/10.3390/nano10020257 Text en © 2020 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Li, Jiakun
Chen, Zeqiang
Yang, Hua
Yi, Zao
Chen, Xifang
Yao, Weitang
Duan, Tao
Wu, Pinghui
Li, Gongfa
Yi, Yougen
Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title_full Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title_fullStr Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title_full_unstemmed Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title_short Tunable Broadband Solar Energy Absorber Based on Monolayer Transition Metal Dichalcogenides Materials Using Au Nanocubes
title_sort tunable broadband solar energy absorber based on monolayer transition metal dichalcogenides materials using au nanocubes
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7075212/
https://www.ncbi.nlm.nih.gov/pubmed/32024205
http://dx.doi.org/10.3390/nano10020257
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