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Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)

Amongst the rare-earth perovskite nickelates, LaNiO(3) (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic...

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Autores principales: Liu, Changjiang, Humbert, Vincent F. C., Bretz-Sullivan, Terence M., Wang, Gensheng, Hong, Deshun, Wrobel, Friederike, Zhang, Jianjie, Hoffman, Jason D., Pearson, John E., Jiang, J. Samuel, Chang, Clarence, Suslov, Alexey, Mason, Nadya, Norman, M. R., Bhattacharya, Anand
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7075863/
https://www.ncbi.nlm.nih.gov/pubmed/32179750
http://dx.doi.org/10.1038/s41467-020-15143-w
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author Liu, Changjiang
Humbert, Vincent F. C.
Bretz-Sullivan, Terence M.
Wang, Gensheng
Hong, Deshun
Wrobel, Friederike
Zhang, Jianjie
Hoffman, Jason D.
Pearson, John E.
Jiang, J. Samuel
Chang, Clarence
Suslov, Alexey
Mason, Nadya
Norman, M. R.
Bhattacharya, Anand
author_facet Liu, Changjiang
Humbert, Vincent F. C.
Bretz-Sullivan, Terence M.
Wang, Gensheng
Hong, Deshun
Wrobel, Friederike
Zhang, Jianjie
Hoffman, Jason D.
Pearson, John E.
Jiang, J. Samuel
Chang, Clarence
Suslov, Alexey
Mason, Nadya
Norman, M. R.
Bhattacharya, Anand
author_sort Liu, Changjiang
collection PubMed
description Amongst the rare-earth perovskite nickelates, LaNiO(3) (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP.
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spelling pubmed-70758632020-03-18 Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3) Liu, Changjiang Humbert, Vincent F. C. Bretz-Sullivan, Terence M. Wang, Gensheng Hong, Deshun Wrobel, Friederike Zhang, Jianjie Hoffman, Jason D. Pearson, John E. Jiang, J. Samuel Chang, Clarence Suslov, Alexey Mason, Nadya Norman, M. R. Bhattacharya, Anand Nat Commun Article Amongst the rare-earth perovskite nickelates, LaNiO(3) (LNO) is an exception. While the former have insulating and antiferromagnetic ground states, LNO remains metallic and non-magnetic down to the lowest temperatures. It is believed that LNO is a strange metal, on the verge of an antiferromagnetic instability. Our work suggests that LNO is a quantum critical metal, close to an antiferromagnetic quantum critical point (QCP). The QCP behavior in LNO is manifested in epitaxial thin films with unprecedented high purities. We find that the temperature and magnetic field dependences of the resistivity of LNO at low temperatures are consistent with scatterings of charge carriers from weak disorder and quantum fluctuations of an antiferromagnetic nature. Furthermore, we find that the introduction of a small concentration of magnetic impurities qualitatively changes the magnetotransport properties of LNO, resembling that found in some heavy-fermion Kondo lattice systems in the vicinity of an antiferromagnetic QCP. Nature Publishing Group UK 2020-03-16 /pmc/articles/PMC7075863/ /pubmed/32179750 http://dx.doi.org/10.1038/s41467-020-15143-w Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Liu, Changjiang
Humbert, Vincent F. C.
Bretz-Sullivan, Terence M.
Wang, Gensheng
Hong, Deshun
Wrobel, Friederike
Zhang, Jianjie
Hoffman, Jason D.
Pearson, John E.
Jiang, J. Samuel
Chang, Clarence
Suslov, Alexey
Mason, Nadya
Norman, M. R.
Bhattacharya, Anand
Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title_full Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title_fullStr Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title_full_unstemmed Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title_short Observation of an antiferromagnetic quantum critical point in high-purity LaNiO(3)
title_sort observation of an antiferromagnetic quantum critical point in high-purity lanio(3)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7075863/
https://www.ncbi.nlm.nih.gov/pubmed/32179750
http://dx.doi.org/10.1038/s41467-020-15143-w
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