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Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption

[Image: see text] The effects of ozone concentration, NaOH concentration, type and concentration of additives, initial pH, temperature, and NO and SO(2) concentration on simultaneous removal of NO and SO(2) were studied through ozone oxidation combined with wet absorption. Results indicated that ozo...

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Autores principales: Xu, Zheng-Hui, Xiao, Xiang, Jia, Yan, Fang, Ping, Huang, Jian-Hang, Wu, Hai-Wen, Tang, Zi-Jun, Chen, Dong-Yao
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7097996/
https://www.ncbi.nlm.nih.gov/pubmed/32226864
http://dx.doi.org/10.1021/acsomega.9b04031
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author Xu, Zheng-Hui
Xiao, Xiang
Jia, Yan
Fang, Ping
Huang, Jian-Hang
Wu, Hai-Wen
Tang, Zi-Jun
Chen, Dong-Yao
author_facet Xu, Zheng-Hui
Xiao, Xiang
Jia, Yan
Fang, Ping
Huang, Jian-Hang
Wu, Hai-Wen
Tang, Zi-Jun
Chen, Dong-Yao
author_sort Xu, Zheng-Hui
collection PubMed
description [Image: see text] The effects of ozone concentration, NaOH concentration, type and concentration of additives, initial pH, temperature, and NO and SO(2) concentration on simultaneous removal of NO and SO(2) were studied through ozone oxidation combined with wet absorption. Results indicated that ozone concentration and the type and concentration of additives had the most significant effect on NO removal. The optimal ozone concentration was 250 ppm (NO/NO(2) = 1), and the best additive was KMnO(4). The removal efficiency of NO(x) was as high as 97.86% when NO/NO(2) = 1, and the concentration of KMnO(4) was 0.025 mol/L. Considering economic and other factors, the KMnO(4) concentration was selected to be 0.006 mol/L. At this time, the removal efficiencies of NO(x) and SO(2) were 81.35 and 100%, respectively. This method has potential application prospects for simultaneous removal of SO(2) and NO in the industrial flue gas.
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spelling pubmed-70979962020-03-27 Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption Xu, Zheng-Hui Xiao, Xiang Jia, Yan Fang, Ping Huang, Jian-Hang Wu, Hai-Wen Tang, Zi-Jun Chen, Dong-Yao ACS Omega [Image: see text] The effects of ozone concentration, NaOH concentration, type and concentration of additives, initial pH, temperature, and NO and SO(2) concentration on simultaneous removal of NO and SO(2) were studied through ozone oxidation combined with wet absorption. Results indicated that ozone concentration and the type and concentration of additives had the most significant effect on NO removal. The optimal ozone concentration was 250 ppm (NO/NO(2) = 1), and the best additive was KMnO(4). The removal efficiency of NO(x) was as high as 97.86% when NO/NO(2) = 1, and the concentration of KMnO(4) was 0.025 mol/L. Considering economic and other factors, the KMnO(4) concentration was selected to be 0.006 mol/L. At this time, the removal efficiencies of NO(x) and SO(2) were 81.35 and 100%, respectively. This method has potential application prospects for simultaneous removal of SO(2) and NO in the industrial flue gas. American Chemical Society 2020-03-12 /pmc/articles/PMC7097996/ /pubmed/32226864 http://dx.doi.org/10.1021/acsomega.9b04031 Text en Copyright © 2020 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Xu, Zheng-Hui
Xiao, Xiang
Jia, Yan
Fang, Ping
Huang, Jian-Hang
Wu, Hai-Wen
Tang, Zi-Jun
Chen, Dong-Yao
Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title_full Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title_fullStr Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title_full_unstemmed Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title_short Simultaneous Removal of SO(2) and NO by O(3) Oxidation Combined with Wet Absorption
title_sort simultaneous removal of so(2) and no by o(3) oxidation combined with wet absorption
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7097996/
https://www.ncbi.nlm.nih.gov/pubmed/32226864
http://dx.doi.org/10.1021/acsomega.9b04031
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