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Disordered hyperuniformity in two-dimensional amorphous silica
Disordered hyperuniformity (DHU) is a recently proposed new state of matter, which has been observed in a variety of classical and quantum many-body systems. DHU systems are characterized by vanishing infinite-wavelength normalized density fluctuations and are endowed with unique novel physical prop...
Autores principales: | , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Association for the Advancement of Science
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7164937/ https://www.ncbi.nlm.nih.gov/pubmed/32494625 http://dx.doi.org/10.1126/sciadv.aba0826 |
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author | Zheng, Yu Liu, Lei Nan, Hanqing Shen, Zhen-Xiong Zhang, Ge Chen, Duyu He, Lixin Xu, Wenxiang Chen, Mohan Jiao, Yang Zhuang, Houlong |
author_facet | Zheng, Yu Liu, Lei Nan, Hanqing Shen, Zhen-Xiong Zhang, Ge Chen, Duyu He, Lixin Xu, Wenxiang Chen, Mohan Jiao, Yang Zhuang, Houlong |
author_sort | Zheng, Yu |
collection | PubMed |
description | Disordered hyperuniformity (DHU) is a recently proposed new state of matter, which has been observed in a variety of classical and quantum many-body systems. DHU systems are characterized by vanishing infinite-wavelength normalized density fluctuations and are endowed with unique novel physical properties. Here, we report the discovery of disordered hyperuniformity in atomic-scale two-dimensional materials, i.e., amorphous silica composed of a single layer of atoms, based on spectral-density analysis of high-resolution transmission electron microscopy images. Moreover, we show via large-scale density functional theory calculations that DHU leads to almost complete closure of the electronic bandgap compared to the crystalline counterpart, making the material effectively a metal. This is in contrast to the conventional wisdom that disorder generally diminishes electronic transport and is due to the unique electron wave localization induced by the topological defects in the DHU state. |
format | Online Article Text |
id | pubmed-7164937 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | American Association for the Advancement of Science |
record_format | MEDLINE/PubMed |
spelling | pubmed-71649372020-06-02 Disordered hyperuniformity in two-dimensional amorphous silica Zheng, Yu Liu, Lei Nan, Hanqing Shen, Zhen-Xiong Zhang, Ge Chen, Duyu He, Lixin Xu, Wenxiang Chen, Mohan Jiao, Yang Zhuang, Houlong Sci Adv Research Articles Disordered hyperuniformity (DHU) is a recently proposed new state of matter, which has been observed in a variety of classical and quantum many-body systems. DHU systems are characterized by vanishing infinite-wavelength normalized density fluctuations and are endowed with unique novel physical properties. Here, we report the discovery of disordered hyperuniformity in atomic-scale two-dimensional materials, i.e., amorphous silica composed of a single layer of atoms, based on spectral-density analysis of high-resolution transmission electron microscopy images. Moreover, we show via large-scale density functional theory calculations that DHU leads to almost complete closure of the electronic bandgap compared to the crystalline counterpart, making the material effectively a metal. This is in contrast to the conventional wisdom that disorder generally diminishes electronic transport and is due to the unique electron wave localization induced by the topological defects in the DHU state. American Association for the Advancement of Science 2020-04-17 /pmc/articles/PMC7164937/ /pubmed/32494625 http://dx.doi.org/10.1126/sciadv.aba0826 Text en Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
spellingShingle | Research Articles Zheng, Yu Liu, Lei Nan, Hanqing Shen, Zhen-Xiong Zhang, Ge Chen, Duyu He, Lixin Xu, Wenxiang Chen, Mohan Jiao, Yang Zhuang, Houlong Disordered hyperuniformity in two-dimensional amorphous silica |
title | Disordered hyperuniformity in two-dimensional amorphous silica |
title_full | Disordered hyperuniformity in two-dimensional amorphous silica |
title_fullStr | Disordered hyperuniformity in two-dimensional amorphous silica |
title_full_unstemmed | Disordered hyperuniformity in two-dimensional amorphous silica |
title_short | Disordered hyperuniformity in two-dimensional amorphous silica |
title_sort | disordered hyperuniformity in two-dimensional amorphous silica |
topic | Research Articles |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7164937/ https://www.ncbi.nlm.nih.gov/pubmed/32494625 http://dx.doi.org/10.1126/sciadv.aba0826 |
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