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Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors

Metamaterials have recently established a new paradigm for enhanced light absorption in state-of-the-art photodetectors. Here, we demonstrate broadband, highly efficient, polarization-insensitive, and gate-tunable photodetection at room temperature in a novel metadevice based on gold/graphene Sierpi...

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Autores principales: De Nicola, Francesco, Puthiya Purayil, Nikhil Santh, Miŝeikis, Vaidotas, Spirito, Davide, Tomadin, Andrea, Coletti, Camilla, Polini, Marco, Krahne, Roman, Pellegrini, Vittorio
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7181626/
https://www.ncbi.nlm.nih.gov/pubmed/32327667
http://dx.doi.org/10.1038/s41598-020-63099-0
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author De Nicola, Francesco
Puthiya Purayil, Nikhil Santh
Miŝeikis, Vaidotas
Spirito, Davide
Tomadin, Andrea
Coletti, Camilla
Polini, Marco
Krahne, Roman
Pellegrini, Vittorio
author_facet De Nicola, Francesco
Puthiya Purayil, Nikhil Santh
Miŝeikis, Vaidotas
Spirito, Davide
Tomadin, Andrea
Coletti, Camilla
Polini, Marco
Krahne, Roman
Pellegrini, Vittorio
author_sort De Nicola, Francesco
collection PubMed
description Metamaterials have recently established a new paradigm for enhanced light absorption in state-of-the-art photodetectors. Here, we demonstrate broadband, highly efficient, polarization-insensitive, and gate-tunable photodetection at room temperature in a novel metadevice based on gold/graphene Sierpinski carpet plasmonic fractals. We observed an unprecedented internal quantum efficiency up to 100% from the near-infrared to the visible range with an upper bound of optical detectivity of 10(11) Jones and a gain up to 10(6), which is a fingerprint of multiple hot carriers photogenerated in graphene. Also, we show a 100-fold enhanced photodetection due to highly focused (up to a record factor of |E/E(0)| ≈ 20 for graphene) electromagnetic fields induced by electrically tunable multimodal plasmons, spatially localized in self-similar fashion on the metasurface. Our findings give direct insight into the physical processes governing graphene plasmonic fractal metamaterials. The proposed structure represents a promising route for the realization of a broadband, compact, and active platform for future optoelectronic devices including multiband bio/chemical and light sensors.
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spelling pubmed-71816262020-04-27 Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors De Nicola, Francesco Puthiya Purayil, Nikhil Santh Miŝeikis, Vaidotas Spirito, Davide Tomadin, Andrea Coletti, Camilla Polini, Marco Krahne, Roman Pellegrini, Vittorio Sci Rep Article Metamaterials have recently established a new paradigm for enhanced light absorption in state-of-the-art photodetectors. Here, we demonstrate broadband, highly efficient, polarization-insensitive, and gate-tunable photodetection at room temperature in a novel metadevice based on gold/graphene Sierpinski carpet plasmonic fractals. We observed an unprecedented internal quantum efficiency up to 100% from the near-infrared to the visible range with an upper bound of optical detectivity of 10(11) Jones and a gain up to 10(6), which is a fingerprint of multiple hot carriers photogenerated in graphene. Also, we show a 100-fold enhanced photodetection due to highly focused (up to a record factor of |E/E(0)| ≈ 20 for graphene) electromagnetic fields induced by electrically tunable multimodal plasmons, spatially localized in self-similar fashion on the metasurface. Our findings give direct insight into the physical processes governing graphene plasmonic fractal metamaterials. The proposed structure represents a promising route for the realization of a broadband, compact, and active platform for future optoelectronic devices including multiband bio/chemical and light sensors. Nature Publishing Group UK 2020-04-23 /pmc/articles/PMC7181626/ /pubmed/32327667 http://dx.doi.org/10.1038/s41598-020-63099-0 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
De Nicola, Francesco
Puthiya Purayil, Nikhil Santh
Miŝeikis, Vaidotas
Spirito, Davide
Tomadin, Andrea
Coletti, Camilla
Polini, Marco
Krahne, Roman
Pellegrini, Vittorio
Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title_full Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title_fullStr Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title_full_unstemmed Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title_short Graphene Plasmonic Fractal Metamaterials for Broadband Photodetectors
title_sort graphene plasmonic fractal metamaterials for broadband photodetectors
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7181626/
https://www.ncbi.nlm.nih.gov/pubmed/32327667
http://dx.doi.org/10.1038/s41598-020-63099-0
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