Cargando…
Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
[Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge o...
Autores principales: | , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2020
|
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7227058/ https://www.ncbi.nlm.nih.gov/pubmed/32426610 http://dx.doi.org/10.1021/acsomega.0c00808 |
_version_ | 1783534422344073216 |
---|---|
author | Qi, Liqiang Zhao, Zhikai Wang, Ruitao Gao, Weiheng Li, Jingxin Zhang, Yajuan |
author_facet | Qi, Liqiang Zhao, Zhikai Wang, Ruitao Gao, Weiheng Li, Jingxin Zhang, Yajuan |
author_sort | Qi, Liqiang |
collection | PubMed |
description | [Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge on the activity of the catalyst were studied. The La(6%)–Ce(8%)–V(7%)–Cu(8%)–ZSM-5 catalyst prepared by successive impregnation methods had the optimum simultaneous desulfurization and denitrification efficiency at a roasting temperature of 600 °C. The desulfurization and denitrification rates reached 97.09 and 83.30%, respectively. BET and SEM characterization results showed that the loading of active components and additives improved the pore structure of the molecular sieve, which contributed to the high stability of the catalyst’s internal structure and large surface area, as well as better desulfurization and denitrification efficiency. Corona discharge can significantly improve the catalytic effect. |
format | Online Article Text |
id | pubmed-7227058 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-72270582020-05-18 Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator Qi, Liqiang Zhao, Zhikai Wang, Ruitao Gao, Weiheng Li, Jingxin Zhang, Yajuan ACS Omega [Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge on the activity of the catalyst were studied. The La(6%)–Ce(8%)–V(7%)–Cu(8%)–ZSM-5 catalyst prepared by successive impregnation methods had the optimum simultaneous desulfurization and denitrification efficiency at a roasting temperature of 600 °C. The desulfurization and denitrification rates reached 97.09 and 83.30%, respectively. BET and SEM characterization results showed that the loading of active components and additives improved the pore structure of the molecular sieve, which contributed to the high stability of the catalyst’s internal structure and large surface area, as well as better desulfurization and denitrification efficiency. Corona discharge can significantly improve the catalytic effect. American Chemical Society 2020-04-28 /pmc/articles/PMC7227058/ /pubmed/32426610 http://dx.doi.org/10.1021/acsomega.0c00808 Text en Copyright © 2020 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes. |
spellingShingle | Qi, Liqiang Zhao, Zhikai Wang, Ruitao Gao, Weiheng Li, Jingxin Zhang, Yajuan Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator |
title | Simultaneous Desulfurization and Denitrification Using
La–Ce–V–Cu–ZSM-5 Catalysts in an
Electrostatic Precipitator |
title_full | Simultaneous Desulfurization and Denitrification Using
La–Ce–V–Cu–ZSM-5 Catalysts in an
Electrostatic Precipitator |
title_fullStr | Simultaneous Desulfurization and Denitrification Using
La–Ce–V–Cu–ZSM-5 Catalysts in an
Electrostatic Precipitator |
title_full_unstemmed | Simultaneous Desulfurization and Denitrification Using
La–Ce–V–Cu–ZSM-5 Catalysts in an
Electrostatic Precipitator |
title_short | Simultaneous Desulfurization and Denitrification Using
La–Ce–V–Cu–ZSM-5 Catalysts in an
Electrostatic Precipitator |
title_sort | simultaneous desulfurization and denitrification using
la–ce–v–cu–zsm-5 catalysts in an
electrostatic precipitator |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7227058/ https://www.ncbi.nlm.nih.gov/pubmed/32426610 http://dx.doi.org/10.1021/acsomega.0c00808 |
work_keys_str_mv | AT qiliqiang simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator AT zhaozhikai simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator AT wangruitao simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator AT gaoweiheng simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator AT lijingxin simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator AT zhangyajuan simultaneousdesulfurizationanddenitrificationusinglacevcuzsm5catalystsinanelectrostaticprecipitator |