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Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator

[Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge o...

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Autores principales: Qi, Liqiang, Zhao, Zhikai, Wang, Ruitao, Gao, Weiheng, Li, Jingxin, Zhang, Yajuan
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7227058/
https://www.ncbi.nlm.nih.gov/pubmed/32426610
http://dx.doi.org/10.1021/acsomega.0c00808
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author Qi, Liqiang
Zhao, Zhikai
Wang, Ruitao
Gao, Weiheng
Li, Jingxin
Zhang, Yajuan
author_facet Qi, Liqiang
Zhao, Zhikai
Wang, Ruitao
Gao, Weiheng
Li, Jingxin
Zhang, Yajuan
author_sort Qi, Liqiang
collection PubMed
description [Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge on the activity of the catalyst were studied. The La(6%)–Ce(8%)–V(7%)–Cu(8%)–ZSM-5 catalyst prepared by successive impregnation methods had the optimum simultaneous desulfurization and denitrification efficiency at a roasting temperature of 600 °C. The desulfurization and denitrification rates reached 97.09 and 83.30%, respectively. BET and SEM characterization results showed that the loading of active components and additives improved the pore structure of the molecular sieve, which contributed to the high stability of the catalyst’s internal structure and large surface area, as well as better desulfurization and denitrification efficiency. Corona discharge can significantly improve the catalytic effect.
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spelling pubmed-72270582020-05-18 Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator Qi, Liqiang Zhao, Zhikai Wang, Ruitao Gao, Weiheng Li, Jingxin Zhang, Yajuan ACS Omega [Image: see text] Different catalysts were loaded onto the collecting plate of an electrostatic precipitator to achieve the simultaneous removal of multiple pollutants from coal-fired gas. The synergistic desulfurization and denitrification effect of the catalyst and the effect of corona discharge on the activity of the catalyst were studied. The La(6%)–Ce(8%)–V(7%)–Cu(8%)–ZSM-5 catalyst prepared by successive impregnation methods had the optimum simultaneous desulfurization and denitrification efficiency at a roasting temperature of 600 °C. The desulfurization and denitrification rates reached 97.09 and 83.30%, respectively. BET and SEM characterization results showed that the loading of active components and additives improved the pore structure of the molecular sieve, which contributed to the high stability of the catalyst’s internal structure and large surface area, as well as better desulfurization and denitrification efficiency. Corona discharge can significantly improve the catalytic effect. American Chemical Society 2020-04-28 /pmc/articles/PMC7227058/ /pubmed/32426610 http://dx.doi.org/10.1021/acsomega.0c00808 Text en Copyright © 2020 American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Qi, Liqiang
Zhao, Zhikai
Wang, Ruitao
Gao, Weiheng
Li, Jingxin
Zhang, Yajuan
Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title_full Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title_fullStr Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title_full_unstemmed Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title_short Simultaneous Desulfurization and Denitrification Using La–Ce–V–Cu–ZSM-5 Catalysts in an Electrostatic Precipitator
title_sort simultaneous desulfurization and denitrification using la–ce–v–cu–zsm-5 catalysts in an electrostatic precipitator
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7227058/
https://www.ncbi.nlm.nih.gov/pubmed/32426610
http://dx.doi.org/10.1021/acsomega.0c00808
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