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Colossal flexoresistance in dielectrics

Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to st...

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Autores principales: Park, Sung Min, Wang, Bo, Paudel, Tula, Park, Se Young, Das, Saikat, Kim, Jeong Rae, Ko, Eun Kyo, Lee, Han Gyeol, Park, Nahee, Tao, Lingling, Suh, Dongseok, Tsymbal, Evgeny Y., Chen, Long-Qing, Noh, Tae Won, Lee, Daesu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7244591/
https://www.ncbi.nlm.nih.gov/pubmed/32444818
http://dx.doi.org/10.1038/s41467-020-16207-7
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author Park, Sung Min
Wang, Bo
Paudel, Tula
Park, Se Young
Das, Saikat
Kim, Jeong Rae
Ko, Eun Kyo
Lee, Han Gyeol
Park, Nahee
Tao, Lingling
Suh, Dongseok
Tsymbal, Evgeny Y.
Chen, Long-Qing
Noh, Tae Won
Lee, Daesu
author_facet Park, Sung Min
Wang, Bo
Paudel, Tula
Park, Se Young
Das, Saikat
Kim, Jeong Rae
Ko, Eun Kyo
Lee, Han Gyeol
Park, Nahee
Tao, Lingling
Suh, Dongseok
Tsymbal, Evgeny Y.
Chen, Long-Qing
Noh, Tae Won
Lee, Daesu
author_sort Park, Sung Min
collection PubMed
description Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to strong electric fields, leading to reversible switching between electrical states—insulating and conducting. Applying strain gradients with an atomic force microscope tip polarizes an ultrathin film of an archetypal dielectric SrTiO(3) via flexoelectricity, which in turn generates non-destructive, strong electrostatic fields. When the applied strain gradient exceeds a certain value, SrTiO(3) suddenly becomes highly conductive, yielding at least around a 10(8)-fold decrease in room-temperature resistivity. We explain this phenomenon, which we call the colossal flexoresistance, based on the abrupt increase in the tunneling conductance of ultrathin SrTiO(3) under strain gradients. Our work extends the scope of electrical control in solids, and inspires further exploration of dielectric responses to strong electromechanical fields.
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spelling pubmed-72445912020-06-03 Colossal flexoresistance in dielectrics Park, Sung Min Wang, Bo Paudel, Tula Park, Se Young Das, Saikat Kim, Jeong Rae Ko, Eun Kyo Lee, Han Gyeol Park, Nahee Tao, Lingling Suh, Dongseok Tsymbal, Evgeny Y. Chen, Long-Qing Noh, Tae Won Lee, Daesu Nat Commun Article Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to strong electric fields, leading to reversible switching between electrical states—insulating and conducting. Applying strain gradients with an atomic force microscope tip polarizes an ultrathin film of an archetypal dielectric SrTiO(3) via flexoelectricity, which in turn generates non-destructive, strong electrostatic fields. When the applied strain gradient exceeds a certain value, SrTiO(3) suddenly becomes highly conductive, yielding at least around a 10(8)-fold decrease in room-temperature resistivity. We explain this phenomenon, which we call the colossal flexoresistance, based on the abrupt increase in the tunneling conductance of ultrathin SrTiO(3) under strain gradients. Our work extends the scope of electrical control in solids, and inspires further exploration of dielectric responses to strong electromechanical fields. Nature Publishing Group UK 2020-05-22 /pmc/articles/PMC7244591/ /pubmed/32444818 http://dx.doi.org/10.1038/s41467-020-16207-7 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Park, Sung Min
Wang, Bo
Paudel, Tula
Park, Se Young
Das, Saikat
Kim, Jeong Rae
Ko, Eun Kyo
Lee, Han Gyeol
Park, Nahee
Tao, Lingling
Suh, Dongseok
Tsymbal, Evgeny Y.
Chen, Long-Qing
Noh, Tae Won
Lee, Daesu
Colossal flexoresistance in dielectrics
title Colossal flexoresistance in dielectrics
title_full Colossal flexoresistance in dielectrics
title_fullStr Colossal flexoresistance in dielectrics
title_full_unstemmed Colossal flexoresistance in dielectrics
title_short Colossal flexoresistance in dielectrics
title_sort colossal flexoresistance in dielectrics
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7244591/
https://www.ncbi.nlm.nih.gov/pubmed/32444818
http://dx.doi.org/10.1038/s41467-020-16207-7
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