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Colossal flexoresistance in dielectrics
Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to st...
Autores principales: | , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7244591/ https://www.ncbi.nlm.nih.gov/pubmed/32444818 http://dx.doi.org/10.1038/s41467-020-16207-7 |
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author | Park, Sung Min Wang, Bo Paudel, Tula Park, Se Young Das, Saikat Kim, Jeong Rae Ko, Eun Kyo Lee, Han Gyeol Park, Nahee Tao, Lingling Suh, Dongseok Tsymbal, Evgeny Y. Chen, Long-Qing Noh, Tae Won Lee, Daesu |
author_facet | Park, Sung Min Wang, Bo Paudel, Tula Park, Se Young Das, Saikat Kim, Jeong Rae Ko, Eun Kyo Lee, Han Gyeol Park, Nahee Tao, Lingling Suh, Dongseok Tsymbal, Evgeny Y. Chen, Long-Qing Noh, Tae Won Lee, Daesu |
author_sort | Park, Sung Min |
collection | PubMed |
description | Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to strong electric fields, leading to reversible switching between electrical states—insulating and conducting. Applying strain gradients with an atomic force microscope tip polarizes an ultrathin film of an archetypal dielectric SrTiO(3) via flexoelectricity, which in turn generates non-destructive, strong electrostatic fields. When the applied strain gradient exceeds a certain value, SrTiO(3) suddenly becomes highly conductive, yielding at least around a 10(8)-fold decrease in room-temperature resistivity. We explain this phenomenon, which we call the colossal flexoresistance, based on the abrupt increase in the tunneling conductance of ultrathin SrTiO(3) under strain gradients. Our work extends the scope of electrical control in solids, and inspires further exploration of dielectric responses to strong electromechanical fields. |
format | Online Article Text |
id | pubmed-7244591 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-72445912020-06-03 Colossal flexoresistance in dielectrics Park, Sung Min Wang, Bo Paudel, Tula Park, Se Young Das, Saikat Kim, Jeong Rae Ko, Eun Kyo Lee, Han Gyeol Park, Nahee Tao, Lingling Suh, Dongseok Tsymbal, Evgeny Y. Chen, Long-Qing Noh, Tae Won Lee, Daesu Nat Commun Article Dielectrics have long been considered as unsuitable for pure electrical switches; under weak electric fields, they show extremely low conductivity, whereas under strong fields, they suffer from irreversible damage. Here, we show that flexoelectricity enables damage-free exposure of dielectrics to strong electric fields, leading to reversible switching between electrical states—insulating and conducting. Applying strain gradients with an atomic force microscope tip polarizes an ultrathin film of an archetypal dielectric SrTiO(3) via flexoelectricity, which in turn generates non-destructive, strong electrostatic fields. When the applied strain gradient exceeds a certain value, SrTiO(3) suddenly becomes highly conductive, yielding at least around a 10(8)-fold decrease in room-temperature resistivity. We explain this phenomenon, which we call the colossal flexoresistance, based on the abrupt increase in the tunneling conductance of ultrathin SrTiO(3) under strain gradients. Our work extends the scope of electrical control in solids, and inspires further exploration of dielectric responses to strong electromechanical fields. Nature Publishing Group UK 2020-05-22 /pmc/articles/PMC7244591/ /pubmed/32444818 http://dx.doi.org/10.1038/s41467-020-16207-7 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Park, Sung Min Wang, Bo Paudel, Tula Park, Se Young Das, Saikat Kim, Jeong Rae Ko, Eun Kyo Lee, Han Gyeol Park, Nahee Tao, Lingling Suh, Dongseok Tsymbal, Evgeny Y. Chen, Long-Qing Noh, Tae Won Lee, Daesu Colossal flexoresistance in dielectrics |
title | Colossal flexoresistance in dielectrics |
title_full | Colossal flexoresistance in dielectrics |
title_fullStr | Colossal flexoresistance in dielectrics |
title_full_unstemmed | Colossal flexoresistance in dielectrics |
title_short | Colossal flexoresistance in dielectrics |
title_sort | colossal flexoresistance in dielectrics |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7244591/ https://www.ncbi.nlm.nih.gov/pubmed/32444818 http://dx.doi.org/10.1038/s41467-020-16207-7 |
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