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Size-dependent influence of NO(x) on the growth rates of organic aerosol particles
Atmospheric new-particle formation (NPF) affects climate by contributing to a large fraction of the cloud condensation nuclei (CCN). Highly oxygenated organic molecules (HOMs) drive the early particle growth and therefore substantially influence the survival of newly formed particles to CCN. Nitroge...
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| Formato: | Online Artículo Texto |
| Lenguaje: | English |
| Publicado: |
American Association for the Advancement of Science
2020
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| Materias: | |
| Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7253163/ https://www.ncbi.nlm.nih.gov/pubmed/32518819 http://dx.doi.org/10.1126/sciadv.aay4945 |
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| author | Yan, C. Nie, W. Vogel, A. L. Dada, L. Lehtipalo, K. Stolzenburg, D. Wagner, R. Rissanen, M. P. Xiao, M. Ahonen, L. Fischer, L. Rose, C. Bianchi, F. Gordon, H. Simon, M. Heinritzi, M. Garmash, O. Roldin, P. Dias, A. Ye, P. Hofbauer, V. Amorim, A. Bauer, P. S. Bergen, A. Bernhammer, A.-K. Breitenlechner, M. Brilke, S. Buchholz, A. Mazon, S. Buenrostro Canagaratna, M. R. Chen, X. Ding, A. Dommen, J. Draper, D. C. Duplissy, J. Frege, C. Heyn, C. Guida, R. Hakala, J. Heikkinen, L. Hoyle, C. R. Jokinen, T. Kangasluoma, J. Kirkby, J. Kontkanen, J. Kürten, A. Lawler, M. J. Mai, H. Mathot, S. Mauldin, R. L. Molteni, U. Nichman, L. Nieminen, T. Nowak, J. Ojdanic, A. Onnela, A. Pajunoja, A. Petäjä, T. Piel, F. Quéléver, L. L. J. Sarnela, N. Schallhart, S. Sengupta, K. Sipilä, M. Tomé, A. Tröstl, J. Väisänen, O. Wagner, A. C. Ylisirniö, A. Zha, Q. Baltensperger, U. Carslaw, K. S. Curtius, J. Flagan, R. C. Hansel, A. Riipinen, I. Smith, J. N. Virtanen, A. Winkler, P. M. Donahue, N. M. Kerminen, V.-M. Kulmala, M. Ehn, M. Worsnop, D. R. |
| author_facet | Yan, C. Nie, W. Vogel, A. L. Dada, L. Lehtipalo, K. Stolzenburg, D. Wagner, R. Rissanen, M. P. Xiao, M. Ahonen, L. Fischer, L. Rose, C. Bianchi, F. Gordon, H. Simon, M. Heinritzi, M. Garmash, O. Roldin, P. Dias, A. Ye, P. Hofbauer, V. Amorim, A. Bauer, P. S. Bergen, A. Bernhammer, A.-K. Breitenlechner, M. Brilke, S. Buchholz, A. Mazon, S. Buenrostro Canagaratna, M. R. Chen, X. Ding, A. Dommen, J. Draper, D. C. Duplissy, J. Frege, C. Heyn, C. Guida, R. Hakala, J. Heikkinen, L. Hoyle, C. R. Jokinen, T. Kangasluoma, J. Kirkby, J. Kontkanen, J. Kürten, A. Lawler, M. J. Mai, H. Mathot, S. Mauldin, R. L. Molteni, U. Nichman, L. Nieminen, T. Nowak, J. Ojdanic, A. Onnela, A. Pajunoja, A. Petäjä, T. Piel, F. Quéléver, L. L. J. Sarnela, N. Schallhart, S. Sengupta, K. Sipilä, M. Tomé, A. Tröstl, J. Väisänen, O. Wagner, A. C. Ylisirniö, A. Zha, Q. Baltensperger, U. Carslaw, K. S. Curtius, J. Flagan, R. C. Hansel, A. Riipinen, I. Smith, J. N. Virtanen, A. Winkler, P. M. Donahue, N. M. Kerminen, V.-M. Kulmala, M. Ehn, M. Worsnop, D. R. |
| author_sort | Yan, C. |
| collection | PubMed |
| description | Atmospheric new-particle formation (NPF) affects climate by contributing to a large fraction of the cloud condensation nuclei (CCN). Highly oxygenated organic molecules (HOMs) drive the early particle growth and therefore substantially influence the survival of newly formed particles to CCN. Nitrogen oxide (NO(x)) is known to suppress the NPF driven by HOMs, but the underlying mechanism remains largely unclear. Here, we examine the response of particle growth to the changes of HOM formation caused by NO(x). We show that NO(x) suppresses particle growth in general, but the suppression is rather nonuniform and size dependent, which can be quantitatively explained by the shifted HOM volatility after adding NO(x). By illustrating how NO(x) affects the early growth of new particles, a critical step of CCN formation, our results help provide a refined assessment of the potential climatic effects caused by the diverse changes of NO(x) level in forest regions around the globe. |
| format | Online Article Text |
| id | pubmed-7253163 |
| institution | National Center for Biotechnology Information |
| language | English |
| publishDate | 2020 |
| publisher | American Association for the Advancement of Science |
| record_format | MEDLINE/PubMed |
| spelling | pubmed-72531632020-06-08 Size-dependent influence of NO(x) on the growth rates of organic aerosol particles Yan, C. Nie, W. Vogel, A. L. Dada, L. Lehtipalo, K. Stolzenburg, D. Wagner, R. Rissanen, M. P. Xiao, M. Ahonen, L. Fischer, L. Rose, C. Bianchi, F. Gordon, H. Simon, M. Heinritzi, M. Garmash, O. Roldin, P. Dias, A. Ye, P. Hofbauer, V. Amorim, A. Bauer, P. S. Bergen, A. Bernhammer, A.-K. Breitenlechner, M. Brilke, S. Buchholz, A. Mazon, S. Buenrostro Canagaratna, M. R. Chen, X. Ding, A. Dommen, J. Draper, D. C. Duplissy, J. Frege, C. Heyn, C. Guida, R. Hakala, J. Heikkinen, L. Hoyle, C. R. Jokinen, T. Kangasluoma, J. Kirkby, J. Kontkanen, J. Kürten, A. Lawler, M. J. Mai, H. Mathot, S. Mauldin, R. L. Molteni, U. Nichman, L. Nieminen, T. Nowak, J. Ojdanic, A. Onnela, A. Pajunoja, A. Petäjä, T. Piel, F. Quéléver, L. L. J. Sarnela, N. Schallhart, S. Sengupta, K. Sipilä, M. Tomé, A. Tröstl, J. Väisänen, O. Wagner, A. C. Ylisirniö, A. Zha, Q. Baltensperger, U. Carslaw, K. S. Curtius, J. Flagan, R. C. Hansel, A. Riipinen, I. Smith, J. N. Virtanen, A. Winkler, P. M. Donahue, N. M. Kerminen, V.-M. Kulmala, M. Ehn, M. Worsnop, D. R. Sci Adv Research Articles Atmospheric new-particle formation (NPF) affects climate by contributing to a large fraction of the cloud condensation nuclei (CCN). Highly oxygenated organic molecules (HOMs) drive the early particle growth and therefore substantially influence the survival of newly formed particles to CCN. Nitrogen oxide (NO(x)) is known to suppress the NPF driven by HOMs, but the underlying mechanism remains largely unclear. Here, we examine the response of particle growth to the changes of HOM formation caused by NO(x). We show that NO(x) suppresses particle growth in general, but the suppression is rather nonuniform and size dependent, which can be quantitatively explained by the shifted HOM volatility after adding NO(x). By illustrating how NO(x) affects the early growth of new particles, a critical step of CCN formation, our results help provide a refined assessment of the potential climatic effects caused by the diverse changes of NO(x) level in forest regions around the globe. American Association for the Advancement of Science 2020-05-27 /pmc/articles/PMC7253163/ /pubmed/32518819 http://dx.doi.org/10.1126/sciadv.aay4945 Text en Copyright © 2020 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). http://creativecommons.org/licenses/by-nc/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (http://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited. |
| spellingShingle | Research Articles Yan, C. Nie, W. Vogel, A. L. Dada, L. Lehtipalo, K. Stolzenburg, D. Wagner, R. Rissanen, M. P. Xiao, M. Ahonen, L. Fischer, L. Rose, C. Bianchi, F. Gordon, H. Simon, M. Heinritzi, M. Garmash, O. Roldin, P. Dias, A. Ye, P. Hofbauer, V. Amorim, A. Bauer, P. S. Bergen, A. Bernhammer, A.-K. Breitenlechner, M. Brilke, S. Buchholz, A. Mazon, S. Buenrostro Canagaratna, M. R. Chen, X. Ding, A. Dommen, J. Draper, D. C. Duplissy, J. Frege, C. Heyn, C. Guida, R. Hakala, J. Heikkinen, L. Hoyle, C. R. Jokinen, T. Kangasluoma, J. Kirkby, J. Kontkanen, J. Kürten, A. Lawler, M. J. Mai, H. Mathot, S. Mauldin, R. L. Molteni, U. Nichman, L. Nieminen, T. Nowak, J. Ojdanic, A. Onnela, A. Pajunoja, A. Petäjä, T. Piel, F. Quéléver, L. L. J. Sarnela, N. Schallhart, S. Sengupta, K. Sipilä, M. Tomé, A. Tröstl, J. Väisänen, O. Wagner, A. C. Ylisirniö, A. Zha, Q. Baltensperger, U. Carslaw, K. S. Curtius, J. Flagan, R. C. Hansel, A. Riipinen, I. Smith, J. N. Virtanen, A. Winkler, P. M. Donahue, N. M. Kerminen, V.-M. Kulmala, M. Ehn, M. Worsnop, D. R. Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title | Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title_full | Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title_fullStr | Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title_full_unstemmed | Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title_short | Size-dependent influence of NO(x) on the growth rates of organic aerosol particles |
| title_sort | size-dependent influence of no(x) on the growth rates of organic aerosol particles |
| topic | Research Articles |
| url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7253163/ https://www.ncbi.nlm.nih.gov/pubmed/32518819 http://dx.doi.org/10.1126/sciadv.aay4945 |
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