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Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells

A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubu...

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Autores principales: Bermúdez Agudelo, María Catalina, Hampe, Manfred, Reiber, Thorsten, Abele, Eberhard
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254196/
https://www.ncbi.nlm.nih.gov/pubmed/32370006
http://dx.doi.org/10.3390/ma13092096
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author Bermúdez Agudelo, María Catalina
Hampe, Manfred
Reiber, Thorsten
Abele, Eberhard
author_facet Bermúdez Agudelo, María Catalina
Hampe, Manfred
Reiber, Thorsten
Abele, Eberhard
author_sort Bermúdez Agudelo, María Catalina
collection PubMed
description A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m(2) after 5 h of operation at 125.52 A/m(2) and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development.
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spelling pubmed-72541962020-06-10 Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells Bermúdez Agudelo, María Catalina Hampe, Manfred Reiber, Thorsten Abele, Eberhard Materials (Basel) Article A high-temperature proton exchange membrane fuel cell (HT-PEMFC) conventionally uses a planar design with carbon-based substrates as the gas diffusion layer (GDL) materials. However, the metal-based substrates allow for alternative designs. In this study, the applicability of porous thin-walled tubular elements made of 316L stainless steel as the anode GDL in a multi-layer tubular HT-PEMFC was investigated. The anode GDLs were fabricated via powder bed fusion using a laser beam (PBF-LB) process with defined porosities (14% and 16%). The morphology of the porous elements was compared using scanning electron microscopy (SEM) micrographs. The influence of the porosity on the fuel cell performance was evaluated through electrochemical characterization and a short-term stability test (45 h) in a commercial test station operated at 160 °C and ambient pressure, using hydrogen as the fuel and air as the oxidant. The results showed that the fuel cell manufactured upon the anode GDL with a porosity of 16% had a higher performance with a peak power density of 329.25 W/m(2) after 5 h of operation at 125.52 A/m(2) and a voltage degradation rate of 0.511 mV/h over the stability test period. Moreover, this work indicates that additive manufacturing could be a useful tool for further fuel cell development. MDPI 2020-05-01 /pmc/articles/PMC7254196/ /pubmed/32370006 http://dx.doi.org/10.3390/ma13092096 Text en © 2020 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Bermúdez Agudelo, María Catalina
Hampe, Manfred
Reiber, Thorsten
Abele, Eberhard
Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title_full Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title_fullStr Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title_full_unstemmed Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title_short Investigation of Porous Metal-Based 3D-Printed Anode GDLs for Tubular High Temperature Proton Exchange Membrane Fuel Cells
title_sort investigation of porous metal-based 3d-printed anode gdls for tubular high temperature proton exchange membrane fuel cells
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254196/
https://www.ncbi.nlm.nih.gov/pubmed/32370006
http://dx.doi.org/10.3390/ma13092096
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