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Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes

[Image: see text] This paper describes a simple, reproducible, and scalable procedure for the preparation of a SiO(2)-containing supercapacitor with high cycle stability. A carbon mesoporous material (CMM) with a high specific surface area, CMK-3, was adopted as an electric double-layer capacitor (E...

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Autores principales: Lo, An-Ya, Chang, Chia-Chia, Lai, Yi-Wei, Chen, Peng-Ren, Xu, Bai-Cheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254803/
https://www.ncbi.nlm.nih.gov/pubmed/32478241
http://dx.doi.org/10.1021/acsomega.0c00669
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author Lo, An-Ya
Chang, Chia-Chia
Lai, Yi-Wei
Chen, Peng-Ren
Xu, Bai-Cheng
author_facet Lo, An-Ya
Chang, Chia-Chia
Lai, Yi-Wei
Chen, Peng-Ren
Xu, Bai-Cheng
author_sort Lo, An-Ya
collection PubMed
description [Image: see text] This paper describes a simple, reproducible, and scalable procedure for the preparation of a SiO(2)-containing supercapacitor with high cycle stability. A carbon mesoporous material (CMM) with a high specific surface area, CMK-3, was adopted as an electric double-layer capacitor (EDLC) active material for the preparation of electrodes for the supercapacitor. The optimized SiO(2) content decreased as the microsphere diameter decreased, and the optimal specific capacitance was obtained with 6 wt % SiO(2) microspheres (100 nm size). The capacitance improved from 133 to 298 F/g. The corresponding capacitance retention rate after 1000 cycles increased from 68.04 to 91.53%. In addition, the energy density increased from 21.05 to 26.25 Wh/kg with a current density of 1 A/g. Finally, similar results based on active carbon, CeO(2)/CMK-3, and graphene/CNT/MnO(v) composite electrodes demonstrated that the proposed method exhibits wide compatibility with diverse electrode materials.
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spelling pubmed-72548032020-05-29 Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes Lo, An-Ya Chang, Chia-Chia Lai, Yi-Wei Chen, Peng-Ren Xu, Bai-Cheng ACS Omega [Image: see text] This paper describes a simple, reproducible, and scalable procedure for the preparation of a SiO(2)-containing supercapacitor with high cycle stability. A carbon mesoporous material (CMM) with a high specific surface area, CMK-3, was adopted as an electric double-layer capacitor (EDLC) active material for the preparation of electrodes for the supercapacitor. The optimized SiO(2) content decreased as the microsphere diameter decreased, and the optimal specific capacitance was obtained with 6 wt % SiO(2) microspheres (100 nm size). The capacitance improved from 133 to 298 F/g. The corresponding capacitance retention rate after 1000 cycles increased from 68.04 to 91.53%. In addition, the energy density increased from 21.05 to 26.25 Wh/kg with a current density of 1 A/g. Finally, similar results based on active carbon, CeO(2)/CMK-3, and graphene/CNT/MnO(v) composite electrodes demonstrated that the proposed method exhibits wide compatibility with diverse electrode materials. American Chemical Society 2020-05-14 /pmc/articles/PMC7254803/ /pubmed/32478241 http://dx.doi.org/10.1021/acsomega.0c00669 Text en Copyright © 2020 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes.
spellingShingle Lo, An-Ya
Chang, Chia-Chia
Lai, Yi-Wei
Chen, Peng-Ren
Xu, Bai-Cheng
Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title_full Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title_fullStr Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title_full_unstemmed Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title_short Improving the Supercapacitor Performance by Dispersing SiO(2) Microspheres in Electrodes
title_sort improving the supercapacitor performance by dispersing sio(2) microspheres in electrodes
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7254803/
https://www.ncbi.nlm.nih.gov/pubmed/32478241
http://dx.doi.org/10.1021/acsomega.0c00669
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