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Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field

Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to mod...

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Detalles Bibliográficos
Autores principales: Li, Zhipeng, Wang, Tianmeng, Miao, Shengnan, Li, Yunmei, Lu, Zhenguang, Jin, Chenhao, Lian, Zhen, Meng, Yuze, Blei, Mark, Taniguchi, Takashi, Watanabe, Kenji, Tongay, Sefaattin, Yao, Wang, Smirnov, Dmitry, Zhang, Chuanwei, Shi, Su-Fei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7305315/
https://www.ncbi.nlm.nih.gov/pubmed/32561746
http://dx.doi.org/10.1038/s41467-020-16934-x
Descripción
Sumario:Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to modify the exciton-phonon interactions by quantizing excitons into discrete Landau levels, which is largely unexplored. Here, we observe the Landau levels originating from phonon-exciton complexes and directly probe exciton-phonon interaction under a quantizing magnetic field. Phonon-exciton interaction lifts the inter-Landau-level transition selection rules for dark trions, manifested by a distinctively different Landau fan pattern compared to bright trions. This allows us to experimentally extract the effective mass of both holes and electrons. The onset of Landau quantization coincides with a significant increase of the valley-Zeeman shift, suggesting strong many-body effects on the phonon-exciton interaction. Our work demonstrates monolayer WSe(2) as an intriguing playground to study phonon-exciton interactions and their interplay with charge, spin, and valley.