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Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field

Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to mod...

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Autores principales: Li, Zhipeng, Wang, Tianmeng, Miao, Shengnan, Li, Yunmei, Lu, Zhenguang, Jin, Chenhao, Lian, Zhen, Meng, Yuze, Blei, Mark, Taniguchi, Takashi, Watanabe, Kenji, Tongay, Sefaattin, Yao, Wang, Smirnov, Dmitry, Zhang, Chuanwei, Shi, Su-Fei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7305315/
https://www.ncbi.nlm.nih.gov/pubmed/32561746
http://dx.doi.org/10.1038/s41467-020-16934-x
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author Li, Zhipeng
Wang, Tianmeng
Miao, Shengnan
Li, Yunmei
Lu, Zhenguang
Jin, Chenhao
Lian, Zhen
Meng, Yuze
Blei, Mark
Taniguchi, Takashi
Watanabe, Kenji
Tongay, Sefaattin
Yao, Wang
Smirnov, Dmitry
Zhang, Chuanwei
Shi, Su-Fei
author_facet Li, Zhipeng
Wang, Tianmeng
Miao, Shengnan
Li, Yunmei
Lu, Zhenguang
Jin, Chenhao
Lian, Zhen
Meng, Yuze
Blei, Mark
Taniguchi, Takashi
Watanabe, Kenji
Tongay, Sefaattin
Yao, Wang
Smirnov, Dmitry
Zhang, Chuanwei
Shi, Su-Fei
author_sort Li, Zhipeng
collection PubMed
description Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to modify the exciton-phonon interactions by quantizing excitons into discrete Landau levels, which is largely unexplored. Here, we observe the Landau levels originating from phonon-exciton complexes and directly probe exciton-phonon interaction under a quantizing magnetic field. Phonon-exciton interaction lifts the inter-Landau-level transition selection rules for dark trions, manifested by a distinctively different Landau fan pattern compared to bright trions. This allows us to experimentally extract the effective mass of both holes and electrons. The onset of Landau quantization coincides with a significant increase of the valley-Zeeman shift, suggesting strong many-body effects on the phonon-exciton interaction. Our work demonstrates monolayer WSe(2) as an intriguing playground to study phonon-exciton interactions and their interplay with charge, spin, and valley.
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spelling pubmed-73053152020-06-26 Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field Li, Zhipeng Wang, Tianmeng Miao, Shengnan Li, Yunmei Lu, Zhenguang Jin, Chenhao Lian, Zhen Meng, Yuze Blei, Mark Taniguchi, Takashi Watanabe, Kenji Tongay, Sefaattin Yao, Wang Smirnov, Dmitry Zhang, Chuanwei Shi, Su-Fei Nat Commun Article Strong many-body interaction in two-dimensional transitional metal dichalcogenides provides a unique platform to study the interplay between different quasiparticles, such as prominent phonon replica emission and modified valley-selection rules. A large out-of-plane magnetic field is expected to modify the exciton-phonon interactions by quantizing excitons into discrete Landau levels, which is largely unexplored. Here, we observe the Landau levels originating from phonon-exciton complexes and directly probe exciton-phonon interaction under a quantizing magnetic field. Phonon-exciton interaction lifts the inter-Landau-level transition selection rules for dark trions, manifested by a distinctively different Landau fan pattern compared to bright trions. This allows us to experimentally extract the effective mass of both holes and electrons. The onset of Landau quantization coincides with a significant increase of the valley-Zeeman shift, suggesting strong many-body effects on the phonon-exciton interaction. Our work demonstrates monolayer WSe(2) as an intriguing playground to study phonon-exciton interactions and their interplay with charge, spin, and valley. Nature Publishing Group UK 2020-06-19 /pmc/articles/PMC7305315/ /pubmed/32561746 http://dx.doi.org/10.1038/s41467-020-16934-x Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Li, Zhipeng
Wang, Tianmeng
Miao, Shengnan
Li, Yunmei
Lu, Zhenguang
Jin, Chenhao
Lian, Zhen
Meng, Yuze
Blei, Mark
Taniguchi, Takashi
Watanabe, Kenji
Tongay, Sefaattin
Yao, Wang
Smirnov, Dmitry
Zhang, Chuanwei
Shi, Su-Fei
Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title_full Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title_fullStr Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title_full_unstemmed Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title_short Phonon-exciton Interactions in WSe(2) under a quantizing magnetic field
title_sort phonon-exciton interactions in wse(2) under a quantizing magnetic field
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7305315/
https://www.ncbi.nlm.nih.gov/pubmed/32561746
http://dx.doi.org/10.1038/s41467-020-16934-x
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