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Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene

In recent years, graphene oxide has been considered as a soluble precursor of graphene for electronic applications. However, the performance lags behind that of graphene due to lattice defects. Here, the relation between the density of defects in the range of 0.2 % and 1.5 % and the transport proper...

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Detalles Bibliográficos
Autores principales: Wang, Zhenping, Yao, Qirong, Eigler, Siegfried
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7317977/
https://www.ncbi.nlm.nih.gov/pubmed/31851390
http://dx.doi.org/10.1002/chem.201905252
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author Wang, Zhenping
Yao, Qirong
Eigler, Siegfried
author_facet Wang, Zhenping
Yao, Qirong
Eigler, Siegfried
author_sort Wang, Zhenping
collection PubMed
description In recent years, graphene oxide has been considered as a soluble precursor of graphene for electronic applications. However, the performance lags behind that of graphene due to lattice defects. Here, the relation between the density of defects in the range of 0.2 % and 1.5 % and the transport properties is quantitatively studied. Therefore, the related flakes of monolayers of graphene were prepared from oxo‐functionalized graphene (oxo‐G). The morphologic structure of oxo‐G was imaged by atomic force microscopy (AFM) and scanning tunneling microscopy (STM). Field‐effect mobility values were determined to range between 0.3 cm(2) V(−1) s(−1) and 33.2 cm(2) V(−1) s(−1), which were inversely proportional to the density of defects. These results provide the first quantitative description of the density of defects and transport properties, which plays an important role for potential applications.
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spelling pubmed-73179772020-06-29 Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene Wang, Zhenping Yao, Qirong Eigler, Siegfried Chemistry Communications In recent years, graphene oxide has been considered as a soluble precursor of graphene for electronic applications. However, the performance lags behind that of graphene due to lattice defects. Here, the relation between the density of defects in the range of 0.2 % and 1.5 % and the transport properties is quantitatively studied. Therefore, the related flakes of monolayers of graphene were prepared from oxo‐functionalized graphene (oxo‐G). The morphologic structure of oxo‐G was imaged by atomic force microscopy (AFM) and scanning tunneling microscopy (STM). Field‐effect mobility values were determined to range between 0.3 cm(2) V(−1) s(−1) and 33.2 cm(2) V(−1) s(−1), which were inversely proportional to the density of defects. These results provide the first quantitative description of the density of defects and transport properties, which plays an important role for potential applications. John Wiley and Sons Inc. 2020-02-03 2020-05-20 /pmc/articles/PMC7317977/ /pubmed/31851390 http://dx.doi.org/10.1002/chem.201905252 Text en © 2019 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Communications
Wang, Zhenping
Yao, Qirong
Eigler, Siegfried
Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title_full Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title_fullStr Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title_full_unstemmed Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title_short Room‐Temperature Transport Properties of Graphene with Defects Derived from Oxo‐Graphene
title_sort room‐temperature transport properties of graphene with defects derived from oxo‐graphene
topic Communications
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7317977/
https://www.ncbi.nlm.nih.gov/pubmed/31851390
http://dx.doi.org/10.1002/chem.201905252
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