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Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr

An efficient application of a material is only possible if we know its physical and chemical properties, which is frequently obstructed by the presence of micro‐ or macroscopic inclusions of secondary phases. While sometimes a sophisticated synthesis route can address this issue, often obtaining pur...

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Autores principales: Antonyshyn, I., Wagner, F. R., Bobnar, M., Sichevych, O., Burkhardt, U., Schmidt, M., König, M., Poeppelmeier, K., Mackenzie, A. P., Svanidze, E., Grin, Yu.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7318276/
https://www.ncbi.nlm.nih.gov/pubmed/32202036
http://dx.doi.org/10.1002/anie.202002693
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author Antonyshyn, I.
Wagner, F. R.
Bobnar, M.
Sichevych, O.
Burkhardt, U.
Schmidt, M.
König, M.
Poeppelmeier, K.
Mackenzie, A. P.
Svanidze, E.
Grin, Yu.
author_facet Antonyshyn, I.
Wagner, F. R.
Bobnar, M.
Sichevych, O.
Burkhardt, U.
Schmidt, M.
König, M.
Poeppelmeier, K.
Mackenzie, A. P.
Svanidze, E.
Grin, Yu.
author_sort Antonyshyn, I.
collection PubMed
description An efficient application of a material is only possible if we know its physical and chemical properties, which is frequently obstructed by the presence of micro‐ or macroscopic inclusions of secondary phases. While sometimes a sophisticated synthesis route can address this issue, often obtaining pure material is not possible. One example is TaGeIr, which has highly sample‐dependent properties resulting from the presence of several impurity phases, which influence electronic transport in the material. The effect of these minority phases was avoided by manufacturing, with the help of focused‐ion‐beam, a μm‐scale device containing only one phase—TaGeIr. This work provides evidence for intrinsic semiconducting behavior of TaGeIr and serves as an example of selective single‐domain device manufacturing. This approach gives a unique access to the properties of compounds that cannot be synthesized in single‐phase form, sparing costly and time‐consuming synthesis efforts.
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spelling pubmed-73182762020-06-29 Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr Antonyshyn, I. Wagner, F. R. Bobnar, M. Sichevych, O. Burkhardt, U. Schmidt, M. König, M. Poeppelmeier, K. Mackenzie, A. P. Svanidze, E. Grin, Yu. Angew Chem Int Ed Engl Research Articles An efficient application of a material is only possible if we know its physical and chemical properties, which is frequently obstructed by the presence of micro‐ or macroscopic inclusions of secondary phases. While sometimes a sophisticated synthesis route can address this issue, often obtaining pure material is not possible. One example is TaGeIr, which has highly sample‐dependent properties resulting from the presence of several impurity phases, which influence electronic transport in the material. The effect of these minority phases was avoided by manufacturing, with the help of focused‐ion‐beam, a μm‐scale device containing only one phase—TaGeIr. This work provides evidence for intrinsic semiconducting behavior of TaGeIr and serves as an example of selective single‐domain device manufacturing. This approach gives a unique access to the properties of compounds that cannot be synthesized in single‐phase form, sparing costly and time‐consuming synthesis efforts. John Wiley and Sons Inc. 2020-04-30 2020-06-26 /pmc/articles/PMC7318276/ /pubmed/32202036 http://dx.doi.org/10.1002/anie.202002693 Text en © 2020 The Authors. Published by Wiley-VCH Verlag GmbH & Co. KGaA. This is an open access article under the terms of the http://creativecommons.org/licenses/by-nc/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited and is not used for commercial purposes.
spellingShingle Research Articles
Antonyshyn, I.
Wagner, F. R.
Bobnar, M.
Sichevych, O.
Burkhardt, U.
Schmidt, M.
König, M.
Poeppelmeier, K.
Mackenzie, A. P.
Svanidze, E.
Grin, Yu.
Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title_full Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title_fullStr Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title_full_unstemmed Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title_short Micro‐Scale Device—An Alternative Route for Studying the Intrinsic Properties of Solid‐State Materials: The Case of Semiconducting TaGeIr
title_sort micro‐scale device—an alternative route for studying the intrinsic properties of solid‐state materials: the case of semiconducting tageir
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7318276/
https://www.ncbi.nlm.nih.gov/pubmed/32202036
http://dx.doi.org/10.1002/anie.202002693
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