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Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring

Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation...

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Autores principales: Yu, Dejian, Wang, Peng, Cao, Fei, Gu, Yu, Liu, Jiaxin, Han, Zeyao, Huang, Bo, Zou, Yousheng, Xu, Xiaobao, Zeng, Haibo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7341884/
https://www.ncbi.nlm.nih.gov/pubmed/32636471
http://dx.doi.org/10.1038/s41467-020-17114-7
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author Yu, Dejian
Wang, Peng
Cao, Fei
Gu, Yu
Liu, Jiaxin
Han, Zeyao
Huang, Bo
Zou, Yousheng
Xu, Xiaobao
Zeng, Haibo
author_facet Yu, Dejian
Wang, Peng
Cao, Fei
Gu, Yu
Liu, Jiaxin
Han, Zeyao
Huang, Bo
Zou, Yousheng
Xu, Xiaobao
Zeng, Haibo
author_sort Yu, Dejian
collection PubMed
description Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation damage. Here, we report a type of β-ray scintillator with good thermotolerance and irradiation hardness based on a two-dimensional halide perovskite. Comprehensive composition engineering and doping are carried out with the rationale elaborated. Consequently, effective β-ray scintillation is obtained, the scintillator shows satisfactory thermal quenching and high decomposition temperature, no functionality decay or hysteresis is observed after an accumulated radiation dose of 10 kGy (dose rate 0.67 kGy h(−1)). Besides, the two-dimensional halide perovskite β-ray scintillator also overcomes the notorious intrinsic water instability, and benefits from low-cost aqueous synthesis along with superior waterproofness, thus paving the way towards practical application.
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spelling pubmed-73418842020-07-09 Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring Yu, Dejian Wang, Peng Cao, Fei Gu, Yu Liu, Jiaxin Han, Zeyao Huang, Bo Zou, Yousheng Xu, Xiaobao Zeng, Haibo Nat Commun Article Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation damage. Here, we report a type of β-ray scintillator with good thermotolerance and irradiation hardness based on a two-dimensional halide perovskite. Comprehensive composition engineering and doping are carried out with the rationale elaborated. Consequently, effective β-ray scintillation is obtained, the scintillator shows satisfactory thermal quenching and high decomposition temperature, no functionality decay or hysteresis is observed after an accumulated radiation dose of 10 kGy (dose rate 0.67 kGy h(−1)). Besides, the two-dimensional halide perovskite β-ray scintillator also overcomes the notorious intrinsic water instability, and benefits from low-cost aqueous synthesis along with superior waterproofness, thus paving the way towards practical application. Nature Publishing Group UK 2020-07-07 /pmc/articles/PMC7341884/ /pubmed/32636471 http://dx.doi.org/10.1038/s41467-020-17114-7 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Yu, Dejian
Wang, Peng
Cao, Fei
Gu, Yu
Liu, Jiaxin
Han, Zeyao
Huang, Bo
Zou, Yousheng
Xu, Xiaobao
Zeng, Haibo
Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title_full Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title_fullStr Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title_full_unstemmed Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title_short Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
title_sort two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7341884/
https://www.ncbi.nlm.nih.gov/pubmed/32636471
http://dx.doi.org/10.1038/s41467-020-17114-7
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