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Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring
Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation...
Autores principales: | , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7341884/ https://www.ncbi.nlm.nih.gov/pubmed/32636471 http://dx.doi.org/10.1038/s41467-020-17114-7 |
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author | Yu, Dejian Wang, Peng Cao, Fei Gu, Yu Liu, Jiaxin Han, Zeyao Huang, Bo Zou, Yousheng Xu, Xiaobao Zeng, Haibo |
author_facet | Yu, Dejian Wang, Peng Cao, Fei Gu, Yu Liu, Jiaxin Han, Zeyao Huang, Bo Zou, Yousheng Xu, Xiaobao Zeng, Haibo |
author_sort | Yu, Dejian |
collection | PubMed |
description | Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation damage. Here, we report a type of β-ray scintillator with good thermotolerance and irradiation hardness based on a two-dimensional halide perovskite. Comprehensive composition engineering and doping are carried out with the rationale elaborated. Consequently, effective β-ray scintillation is obtained, the scintillator shows satisfactory thermal quenching and high decomposition temperature, no functionality decay or hysteresis is observed after an accumulated radiation dose of 10 kGy (dose rate 0.67 kGy h(−1)). Besides, the two-dimensional halide perovskite β-ray scintillator also overcomes the notorious intrinsic water instability, and benefits from low-cost aqueous synthesis along with superior waterproofness, thus paving the way towards practical application. |
format | Online Article Text |
id | pubmed-7341884 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-73418842020-07-09 Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring Yu, Dejian Wang, Peng Cao, Fei Gu, Yu Liu, Jiaxin Han, Zeyao Huang, Bo Zou, Yousheng Xu, Xiaobao Zeng, Haibo Nat Commun Article Ensuring nuclear safety has become of great significance as nuclear power is playing an increasingly important role in supplying worldwide electricity. β-ray monitoring is a crucial method, but commercial organic scintillators for β-ray detection suffer from high temperature failure and irradiation damage. Here, we report a type of β-ray scintillator with good thermotolerance and irradiation hardness based on a two-dimensional halide perovskite. Comprehensive composition engineering and doping are carried out with the rationale elaborated. Consequently, effective β-ray scintillation is obtained, the scintillator shows satisfactory thermal quenching and high decomposition temperature, no functionality decay or hysteresis is observed after an accumulated radiation dose of 10 kGy (dose rate 0.67 kGy h(−1)). Besides, the two-dimensional halide perovskite β-ray scintillator also overcomes the notorious intrinsic water instability, and benefits from low-cost aqueous synthesis along with superior waterproofness, thus paving the way towards practical application. Nature Publishing Group UK 2020-07-07 /pmc/articles/PMC7341884/ /pubmed/32636471 http://dx.doi.org/10.1038/s41467-020-17114-7 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Yu, Dejian Wang, Peng Cao, Fei Gu, Yu Liu, Jiaxin Han, Zeyao Huang, Bo Zou, Yousheng Xu, Xiaobao Zeng, Haibo Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title | Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title_full | Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title_fullStr | Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title_full_unstemmed | Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title_short | Two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
title_sort | two-dimensional halide perovskite as β-ray scintillator for nuclear radiation monitoring |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7341884/ https://www.ncbi.nlm.nih.gov/pubmed/32636471 http://dx.doi.org/10.1038/s41467-020-17114-7 |
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