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Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate...
Autores principales: | , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
National Academy of Sciences
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7368327/ https://www.ncbi.nlm.nih.gov/pubmed/32586955 http://dx.doi.org/10.1073/pnas.2001755117 |
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author | Li, Jiemin Nag, Abhishek Pelliciari, Jonathan Robarts, Hannah Walters, Andrew Garcia-Fernandez, Mirian Eisaki, Hiroshi Song, Dongjoon Ding, Hong Johnston, Steven Comin, Riccardo Zhou, Ke-Jin |
author_facet | Li, Jiemin Nag, Abhishek Pelliciari, Jonathan Robarts, Hannah Walters, Andrew Garcia-Fernandez, Mirian Eisaki, Hiroshi Song, Dongjoon Ding, Hong Johnston, Steven Comin, Riccardo Zhou, Ke-Jin |
author_sort | Li, Jiemin |
collection | PubMed |
description | Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi(2)Sr(1.4)La(0.6)CuO(6+δ) using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO(2)) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi(2)Sr(1.8)La(0.2)CuO(6+δ), where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (Q(CDW)) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than Q(CDW). Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates. |
format | Online Article Text |
id | pubmed-7368327 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | National Academy of Sciences |
record_format | MEDLINE/PubMed |
spelling | pubmed-73683272020-07-29 Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) Li, Jiemin Nag, Abhishek Pelliciari, Jonathan Robarts, Hannah Walters, Andrew Garcia-Fernandez, Mirian Eisaki, Hiroshi Song, Dongjoon Ding, Hong Johnston, Steven Comin, Riccardo Zhou, Ke-Jin Proc Natl Acad Sci U S A Physical Sciences Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi(2)Sr(1.4)La(0.6)CuO(6+δ) using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO(2)) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi(2)Sr(1.8)La(0.2)CuO(6+δ), where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (Q(CDW)) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than Q(CDW). Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates. National Academy of Sciences 2020-07-14 2020-06-25 /pmc/articles/PMC7368327/ /pubmed/32586955 http://dx.doi.org/10.1073/pnas.2001755117 Text en Copyright © 2020 the Author(s). Published by PNAS. http://creativecommons.org/licenses/by/4.0/ https://creativecommons.org/licenses/by/4.0/This open access article is distributed under Creative Commons Attribution License 4.0 (CC BY) (http://creativecommons.org/licenses/by/4.0/) . |
spellingShingle | Physical Sciences Li, Jiemin Nag, Abhishek Pelliciari, Jonathan Robarts, Hannah Walters, Andrew Garcia-Fernandez, Mirian Eisaki, Hiroshi Song, Dongjoon Ding, Hong Johnston, Steven Comin, Riccardo Zhou, Ke-Jin Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title | Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title_full | Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title_fullStr | Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title_full_unstemmed | Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title_short | Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) |
title_sort | multiorbital charge-density wave excitations and concomitant phonon anomalies in bi(2)sr(2)lacuo(6+δ) |
topic | Physical Sciences |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7368327/ https://www.ncbi.nlm.nih.gov/pubmed/32586955 http://dx.doi.org/10.1073/pnas.2001755117 |
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