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Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)

Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate...

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Autores principales: Li, Jiemin, Nag, Abhishek, Pelliciari, Jonathan, Robarts, Hannah, Walters, Andrew, Garcia-Fernandez, Mirian, Eisaki, Hiroshi, Song, Dongjoon, Ding, Hong, Johnston, Steven, Comin, Riccardo, Zhou, Ke-Jin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: National Academy of Sciences 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7368327/
https://www.ncbi.nlm.nih.gov/pubmed/32586955
http://dx.doi.org/10.1073/pnas.2001755117
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author Li, Jiemin
Nag, Abhishek
Pelliciari, Jonathan
Robarts, Hannah
Walters, Andrew
Garcia-Fernandez, Mirian
Eisaki, Hiroshi
Song, Dongjoon
Ding, Hong
Johnston, Steven
Comin, Riccardo
Zhou, Ke-Jin
author_facet Li, Jiemin
Nag, Abhishek
Pelliciari, Jonathan
Robarts, Hannah
Walters, Andrew
Garcia-Fernandez, Mirian
Eisaki, Hiroshi
Song, Dongjoon
Ding, Hong
Johnston, Steven
Comin, Riccardo
Zhou, Ke-Jin
author_sort Li, Jiemin
collection PubMed
description Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi(2)Sr(1.4)La(0.6)CuO(6+δ) using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO(2)) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi(2)Sr(1.8)La(0.2)CuO(6+δ), where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (Q(CDW)) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than Q(CDW). Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates.
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spelling pubmed-73683272020-07-29 Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ) Li, Jiemin Nag, Abhishek Pelliciari, Jonathan Robarts, Hannah Walters, Andrew Garcia-Fernandez, Mirian Eisaki, Hiroshi Song, Dongjoon Ding, Hong Johnston, Steven Comin, Riccardo Zhou, Ke-Jin Proc Natl Acad Sci U S A Physical Sciences Charge-density waves (CDWs) are ubiquitous in underdoped cuprate superconductors. As a modulation of the valence electron density, CDWs in hole-doped cuprates possess both Cu-3d and O-2p orbital character owing to the strong hybridization of these orbitals near the Fermi level. Here, we investigate underdoped Bi(2)Sr(1.4)La(0.6)CuO(6+δ) using resonant inelastic X-ray scattering (RIXS) and find that a short-range CDW exists at both Cu and O sublattices in the copper-oxide (CuO(2)) planes with a comparable periodicity and correlation length. Furthermore, we uncover bond-stretching and bond-buckling phonon anomalies concomitant to the CDWs. Comparing to slightly overdoped Bi(2)Sr(1.8)La(0.2)CuO(6+δ), where neither CDWs nor phonon anomalies appear, we highlight that a sharp intensity anomaly is induced in the proximity of the CDW wavevector (Q(CDW)) for the bond-buckling phonon, in concert with the diffused intensity enhancement of the bond-stretching phonon at wavevectors much greater than Q(CDW). Our results provide a comprehensive picture of the quasistatic CDWs, their dispersive excitations, and associated electron-phonon anomalies, which are key for understanding the competing electronic instabilities in cuprates. National Academy of Sciences 2020-07-14 2020-06-25 /pmc/articles/PMC7368327/ /pubmed/32586955 http://dx.doi.org/10.1073/pnas.2001755117 Text en Copyright © 2020 the Author(s). Published by PNAS. http://creativecommons.org/licenses/by/4.0/ https://creativecommons.org/licenses/by/4.0/This open access article is distributed under Creative Commons Attribution License 4.0 (CC BY) (http://creativecommons.org/licenses/by/4.0/) .
spellingShingle Physical Sciences
Li, Jiemin
Nag, Abhishek
Pelliciari, Jonathan
Robarts, Hannah
Walters, Andrew
Garcia-Fernandez, Mirian
Eisaki, Hiroshi
Song, Dongjoon
Ding, Hong
Johnston, Steven
Comin, Riccardo
Zhou, Ke-Jin
Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title_full Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title_fullStr Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title_full_unstemmed Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title_short Multiorbital charge-density wave excitations and concomitant phonon anomalies in Bi(2)Sr(2)LaCuO(6+δ)
title_sort multiorbital charge-density wave excitations and concomitant phonon anomalies in bi(2)sr(2)lacuo(6+δ)
topic Physical Sciences
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7368327/
https://www.ncbi.nlm.nih.gov/pubmed/32586955
http://dx.doi.org/10.1073/pnas.2001755117
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