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Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)

The interplay between electronic correlations and topological protection may offer a rich avenue for discovering emergent quantum phenomena in condensed matter. However, electronic correlations have so far been little investigated in Weyl semimetals (WSMs) by experiments. Here, we report a combined...

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Autores principales: Xu, Yueshan, Zhao, Jianzhou, Yi, Changjiang, Wang, Qi, Yin, Qiangwei, Wang, Yilin, Hu, Xiaolei, Wang, Luyang, Liu, Enke, Xu, Gang, Lu, Ling, Soluyanov, Alexey A., Lei, Hechang, Shi, Youguo, Luo, Jianlin, Chen, Zhi-Guo
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7417588/
https://www.ncbi.nlm.nih.gov/pubmed/32778652
http://dx.doi.org/10.1038/s41467-020-17234-0
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author Xu, Yueshan
Zhao, Jianzhou
Yi, Changjiang
Wang, Qi
Yin, Qiangwei
Wang, Yilin
Hu, Xiaolei
Wang, Luyang
Liu, Enke
Xu, Gang
Lu, Ling
Soluyanov, Alexey A.
Lei, Hechang
Shi, Youguo
Luo, Jianlin
Chen, Zhi-Guo
author_facet Xu, Yueshan
Zhao, Jianzhou
Yi, Changjiang
Wang, Qi
Yin, Qiangwei
Wang, Yilin
Hu, Xiaolei
Wang, Luyang
Liu, Enke
Xu, Gang
Lu, Ling
Soluyanov, Alexey A.
Lei, Hechang
Shi, Youguo
Luo, Jianlin
Chen, Zhi-Guo
author_sort Xu, Yueshan
collection PubMed
description The interplay between electronic correlations and topological protection may offer a rich avenue for discovering emergent quantum phenomena in condensed matter. However, electronic correlations have so far been little investigated in Weyl semimetals (WSMs) by experiments. Here, we report a combined optical spectroscopy and theoretical calculation study on the strength and effect of electronic correlations in a magnet Co(3)Sn(2)S(2). The electronic kinetic energy estimated from our optical data is about half of that obtained from single-particle ab initio calculations in the ferromagnetic ground state, which indicates intermediate-strength electronic correlations in this system. Furthermore, comparing the energy and side-slope ratios between the interband-transition peaks at high energies in the experimental and single-particle-calculation-derived optical conductivity spectra with the bandwidth-renormalization factors obtained by many-body calculations enables us to estimate the Coulomb-interaction strength (U ∼ 4 eV) in Co(3)Sn(2)S(2). Besides, a sharp experimental optical conductivity peak at low energy, which is absent in the single-particle-calculation-derived spectrum but is consistent with the optical conductivity peaks obtained by many-body calculations with U ∼ 4 eV, indicates that an electronic band connecting the two Weyl cones is flattened by electronic correlations and emerges near the Fermi energy in Co(3)Sn(2)S(2). Our work paves the way for exploring flat-band-generated quantum phenomena in WSMs.
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spelling pubmed-74175882020-08-17 Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2) Xu, Yueshan Zhao, Jianzhou Yi, Changjiang Wang, Qi Yin, Qiangwei Wang, Yilin Hu, Xiaolei Wang, Luyang Liu, Enke Xu, Gang Lu, Ling Soluyanov, Alexey A. Lei, Hechang Shi, Youguo Luo, Jianlin Chen, Zhi-Guo Nat Commun Article The interplay between electronic correlations and topological protection may offer a rich avenue for discovering emergent quantum phenomena in condensed matter. However, electronic correlations have so far been little investigated in Weyl semimetals (WSMs) by experiments. Here, we report a combined optical spectroscopy and theoretical calculation study on the strength and effect of electronic correlations in a magnet Co(3)Sn(2)S(2). The electronic kinetic energy estimated from our optical data is about half of that obtained from single-particle ab initio calculations in the ferromagnetic ground state, which indicates intermediate-strength electronic correlations in this system. Furthermore, comparing the energy and side-slope ratios between the interband-transition peaks at high energies in the experimental and single-particle-calculation-derived optical conductivity spectra with the bandwidth-renormalization factors obtained by many-body calculations enables us to estimate the Coulomb-interaction strength (U ∼ 4 eV) in Co(3)Sn(2)S(2). Besides, a sharp experimental optical conductivity peak at low energy, which is absent in the single-particle-calculation-derived spectrum but is consistent with the optical conductivity peaks obtained by many-body calculations with U ∼ 4 eV, indicates that an electronic band connecting the two Weyl cones is flattened by electronic correlations and emerges near the Fermi energy in Co(3)Sn(2)S(2). Our work paves the way for exploring flat-band-generated quantum phenomena in WSMs. Nature Publishing Group UK 2020-08-10 /pmc/articles/PMC7417588/ /pubmed/32778652 http://dx.doi.org/10.1038/s41467-020-17234-0 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Xu, Yueshan
Zhao, Jianzhou
Yi, Changjiang
Wang, Qi
Yin, Qiangwei
Wang, Yilin
Hu, Xiaolei
Wang, Luyang
Liu, Enke
Xu, Gang
Lu, Ling
Soluyanov, Alexey A.
Lei, Hechang
Shi, Youguo
Luo, Jianlin
Chen, Zhi-Guo
Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title_full Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title_fullStr Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title_full_unstemmed Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title_short Electronic correlations and flattened band in magnetic Weyl semimetal candidate Co(3)Sn(2)S(2)
title_sort electronic correlations and flattened band in magnetic weyl semimetal candidate co(3)sn(2)s(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7417588/
https://www.ncbi.nlm.nih.gov/pubmed/32778652
http://dx.doi.org/10.1038/s41467-020-17234-0
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