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Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs

The valleys of two-dimensional transition metal dichalcogenides (TMDCs) offer a new degree of freedom for information processing. To take advantage of this valley degree of freedom, on the one hand, it is feasible to control valleys by utilizing different external stimuli, such as optical and electr...

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Autores principales: Wang, Jiajun, Li, Han, Ma, Yating, Zhao, Maoxiong, Liu, Wenzhe, Wang, Bo, Wu, Shiwei, Liu, Xiaohan, Shi, Lei, Jiang, Tian, Zi, Jian
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7442784/
https://www.ncbi.nlm.nih.gov/pubmed/32884677
http://dx.doi.org/10.1038/s41377-020-00387-4
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author Wang, Jiajun
Li, Han
Ma, Yating
Zhao, Maoxiong
Liu, Wenzhe
Wang, Bo
Wu, Shiwei
Liu, Xiaohan
Shi, Lei
Jiang, Tian
Zi, Jian
author_facet Wang, Jiajun
Li, Han
Ma, Yating
Zhao, Maoxiong
Liu, Wenzhe
Wang, Bo
Wu, Shiwei
Liu, Xiaohan
Shi, Lei
Jiang, Tian
Zi, Jian
author_sort Wang, Jiajun
collection PubMed
description The valleys of two-dimensional transition metal dichalcogenides (TMDCs) offer a new degree of freedom for information processing. To take advantage of this valley degree of freedom, on the one hand, it is feasible to control valleys by utilizing different external stimuli, such as optical and electric fields. On the other hand, nanostructures are also used to separate the valleys by near-field coupling. However, for both of the above methods, either the required low-temperature environment or low degree of coherence properties limit their further applications. Here, we demonstrate that all-dielectric photonic crystal (PhC) slabs without in-plane inversion symmetry (C(2) symmetry) can separate and route valley exciton emission of a WS(2) monolayer at room temperature. Coupling with circularly polarized photonic Bloch modes of such PhC slabs, valley photons emitted by a WS(2) monolayer are routed directionally and are efficiently separated in the far field. In addition, far-field emissions are directionally enhanced and have long-distance spatial coherence properties.
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spelling pubmed-74427842020-09-02 Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs Wang, Jiajun Li, Han Ma, Yating Zhao, Maoxiong Liu, Wenzhe Wang, Bo Wu, Shiwei Liu, Xiaohan Shi, Lei Jiang, Tian Zi, Jian Light Sci Appl Article The valleys of two-dimensional transition metal dichalcogenides (TMDCs) offer a new degree of freedom for information processing. To take advantage of this valley degree of freedom, on the one hand, it is feasible to control valleys by utilizing different external stimuli, such as optical and electric fields. On the other hand, nanostructures are also used to separate the valleys by near-field coupling. However, for both of the above methods, either the required low-temperature environment or low degree of coherence properties limit their further applications. Here, we demonstrate that all-dielectric photonic crystal (PhC) slabs without in-plane inversion symmetry (C(2) symmetry) can separate and route valley exciton emission of a WS(2) monolayer at room temperature. Coupling with circularly polarized photonic Bloch modes of such PhC slabs, valley photons emitted by a WS(2) monolayer are routed directionally and are efficiently separated in the far field. In addition, far-field emissions are directionally enhanced and have long-distance spatial coherence properties. Nature Publishing Group UK 2020-08-21 /pmc/articles/PMC7442784/ /pubmed/32884677 http://dx.doi.org/10.1038/s41377-020-00387-4 Text en © The Author(s) 2020 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Wang, Jiajun
Li, Han
Ma, Yating
Zhao, Maoxiong
Liu, Wenzhe
Wang, Bo
Wu, Shiwei
Liu, Xiaohan
Shi, Lei
Jiang, Tian
Zi, Jian
Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title_full Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title_fullStr Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title_full_unstemmed Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title_short Routing valley exciton emission of a WS(2) monolayer via delocalized Bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
title_sort routing valley exciton emission of a ws(2) monolayer via delocalized bloch modes of in-plane inversion-symmetry-broken photonic crystal slabs
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7442784/
https://www.ncbi.nlm.nih.gov/pubmed/32884677
http://dx.doi.org/10.1038/s41377-020-00387-4
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