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Strange semimetal dynamics in SrIrO(3)
The interplay of electronic correlations, multi-orbital excitations, and spin-orbit coupling is a fertile ground for new states of matter in quantum materials. Here, we report on a polarized Raman scattering study of semimetallic SrIrO(3). The momentum-space selectivity of Raman scattering allows to...
Autores principales: | , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7450065/ https://www.ncbi.nlm.nih.gov/pubmed/32848163 http://dx.doi.org/10.1038/s41467-020-18092-6 |
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author | Sen, K. Fuchs, D. Heid, R. Kleindienst, K. Wolff, K. Schmalian, J. Le Tacon, M. |
author_facet | Sen, K. Fuchs, D. Heid, R. Kleindienst, K. Wolff, K. Schmalian, J. Le Tacon, M. |
author_sort | Sen, K. |
collection | PubMed |
description | The interplay of electronic correlations, multi-orbital excitations, and spin-orbit coupling is a fertile ground for new states of matter in quantum materials. Here, we report on a polarized Raman scattering study of semimetallic SrIrO(3). The momentum-space selectivity of Raman scattering allows to circumvent the challenge to resolve the dynamics of charges with very different mobilities. The Raman responses of both holes and electrons display an electronic continuum extending far beyond the energies allowed in a regular Fermi liquid. Analyzing this response within a memory function formalism, we extract their frequency dependent scattering rate and mass enhancement, from which we determine their DC-mobilities and electrical resistivities that agree well with transport measurement. We demonstrate that its charge dynamics is well described by a marginal Fermi liquid phenomenology, with a scattering rate close to the Planckian limit. This demonstrates the potential of this approach to investigate the charge dynamics in multi-band systems. |
format | Online Article Text |
id | pubmed-7450065 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-74500652020-09-02 Strange semimetal dynamics in SrIrO(3) Sen, K. Fuchs, D. Heid, R. Kleindienst, K. Wolff, K. Schmalian, J. Le Tacon, M. Nat Commun Article The interplay of electronic correlations, multi-orbital excitations, and spin-orbit coupling is a fertile ground for new states of matter in quantum materials. Here, we report on a polarized Raman scattering study of semimetallic SrIrO(3). The momentum-space selectivity of Raman scattering allows to circumvent the challenge to resolve the dynamics of charges with very different mobilities. The Raman responses of both holes and electrons display an electronic continuum extending far beyond the energies allowed in a regular Fermi liquid. Analyzing this response within a memory function formalism, we extract their frequency dependent scattering rate and mass enhancement, from which we determine their DC-mobilities and electrical resistivities that agree well with transport measurement. We demonstrate that its charge dynamics is well described by a marginal Fermi liquid phenomenology, with a scattering rate close to the Planckian limit. This demonstrates the potential of this approach to investigate the charge dynamics in multi-band systems. Nature Publishing Group UK 2020-08-26 /pmc/articles/PMC7450065/ /pubmed/32848163 http://dx.doi.org/10.1038/s41467-020-18092-6 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Sen, K. Fuchs, D. Heid, R. Kleindienst, K. Wolff, K. Schmalian, J. Le Tacon, M. Strange semimetal dynamics in SrIrO(3) |
title | Strange semimetal dynamics in SrIrO(3) |
title_full | Strange semimetal dynamics in SrIrO(3) |
title_fullStr | Strange semimetal dynamics in SrIrO(3) |
title_full_unstemmed | Strange semimetal dynamics in SrIrO(3) |
title_short | Strange semimetal dynamics in SrIrO(3) |
title_sort | strange semimetal dynamics in sriro(3) |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7450065/ https://www.ncbi.nlm.nih.gov/pubmed/32848163 http://dx.doi.org/10.1038/s41467-020-18092-6 |
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