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Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity

The use of renewable energy by means of electrochemical techniques by converting H(2)O, CO(2) and N(2) into chemical energy sources and raw materials, is the basis for securing a future sustainable “green” energy supply. Some weaknesses and inconsistencies in the practice of determining the electroc...

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Detalles Bibliográficos
Autores principales: Masa, Justus, Andronescu, Corina, Schuhmann, Wolfgang
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7496542/
https://www.ncbi.nlm.nih.gov/pubmed/32608122
http://dx.doi.org/10.1002/anie.202007672
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author Masa, Justus
Andronescu, Corina
Schuhmann, Wolfgang
author_facet Masa, Justus
Andronescu, Corina
Schuhmann, Wolfgang
author_sort Masa, Justus
collection PubMed
description The use of renewable energy by means of electrochemical techniques by converting H(2)O, CO(2) and N(2) into chemical energy sources and raw materials, is the basis for securing a future sustainable “green” energy supply. Some weaknesses and inconsistencies in the practice of determining the electrocatalytic performance, which prevents a rational bottom‐up catalyst design, are discussed. Large discrepancies in material properties as well as in electrocatalytic activity and stability become obvious when materials are tested under the conditions of their intended use as opposed to the usual laboratory conditions. They advocate for uniform activity/stability correlations under application‐relevant conditions, and the need for a clear representation of electrocatalytic performance by contextualization in terms of functional investigation or progress towards application is emphasized.
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spelling pubmed-74965422020-09-25 Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity Masa, Justus Andronescu, Corina Schuhmann, Wolfgang Angew Chem Int Ed Engl Minireviews The use of renewable energy by means of electrochemical techniques by converting H(2)O, CO(2) and N(2) into chemical energy sources and raw materials, is the basis for securing a future sustainable “green” energy supply. Some weaknesses and inconsistencies in the practice of determining the electrocatalytic performance, which prevents a rational bottom‐up catalyst design, are discussed. Large discrepancies in material properties as well as in electrocatalytic activity and stability become obvious when materials are tested under the conditions of their intended use as opposed to the usual laboratory conditions. They advocate for uniform activity/stability correlations under application‐relevant conditions, and the need for a clear representation of electrocatalytic performance by contextualization in terms of functional investigation or progress towards application is emphasized. John Wiley and Sons Inc. 2020-08-18 2020-09-01 /pmc/articles/PMC7496542/ /pubmed/32608122 http://dx.doi.org/10.1002/anie.202007672 Text en © 2020 The Authors. Published by Wiley-VCH GmbH This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Minireviews
Masa, Justus
Andronescu, Corina
Schuhmann, Wolfgang
Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title_full Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title_fullStr Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title_full_unstemmed Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title_short Electrocatalysis as the Nexus for Sustainable Renewable Energy: The Gordian Knot of Activity, Stability, and Selectivity
title_sort electrocatalysis as the nexus for sustainable renewable energy: the gordian knot of activity, stability, and selectivity
topic Minireviews
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7496542/
https://www.ncbi.nlm.nih.gov/pubmed/32608122
http://dx.doi.org/10.1002/anie.202007672
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