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Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids

[Image: see text] Localizing light to nanoscale volumes through nanoscale resonators that are low loss and precisely tailored in spectrum to properties of matter is crucial for classical and quantum light sources, cavity QED, molecular spectroscopy, and many other applications. To date, two opposite...

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Autores principales: Doeleman, Hugo M., Dieleman, Christian D., Mennes, Christiaan, Ehrler, Bruno, Koenderink, A. Femius
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7513474/
https://www.ncbi.nlm.nih.gov/pubmed/32870669
http://dx.doi.org/10.1021/acsnano.0c05233
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author Doeleman, Hugo M.
Dieleman, Christian D.
Mennes, Christiaan
Ehrler, Bruno
Koenderink, A. Femius
author_facet Doeleman, Hugo M.
Dieleman, Christian D.
Mennes, Christiaan
Ehrler, Bruno
Koenderink, A. Femius
author_sort Doeleman, Hugo M.
collection PubMed
description [Image: see text] Localizing light to nanoscale volumes through nanoscale resonators that are low loss and precisely tailored in spectrum to properties of matter is crucial for classical and quantum light sources, cavity QED, molecular spectroscopy, and many other applications. To date, two opposite strategies have been identified: to use either plasmonics with deep subwavelength confinement yet high loss and very poor spectral control or instead microcavities with exquisite quality factors yet poor confinement. In this work we realize hybrid plasmonic–photonic resonators that enhance the emission of single quantum dots, profiting from both plasmonic confinement and microcavity quality factors. Our experiments directly demonstrate how cavity and antenna jointly realize large cooperative Purcell enhancements through interferences. These can be controlled to engineer arbitrary Fano lineshapes in the local density of optical states.
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spelling pubmed-75134742020-09-25 Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids Doeleman, Hugo M. Dieleman, Christian D. Mennes, Christiaan Ehrler, Bruno Koenderink, A. Femius ACS Nano [Image: see text] Localizing light to nanoscale volumes through nanoscale resonators that are low loss and precisely tailored in spectrum to properties of matter is crucial for classical and quantum light sources, cavity QED, molecular spectroscopy, and many other applications. To date, two opposite strategies have been identified: to use either plasmonics with deep subwavelength confinement yet high loss and very poor spectral control or instead microcavities with exquisite quality factors yet poor confinement. In this work we realize hybrid plasmonic–photonic resonators that enhance the emission of single quantum dots, profiting from both plasmonic confinement and microcavity quality factors. Our experiments directly demonstrate how cavity and antenna jointly realize large cooperative Purcell enhancements through interferences. These can be controlled to engineer arbitrary Fano lineshapes in the local density of optical states. American Chemical Society 2020-09-01 2020-09-22 /pmc/articles/PMC7513474/ /pubmed/32870669 http://dx.doi.org/10.1021/acsnano.0c05233 Text en Copyright © 2020 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes.
spellingShingle Doeleman, Hugo M.
Dieleman, Christian D.
Mennes, Christiaan
Ehrler, Bruno
Koenderink, A. Femius
Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title_full Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title_fullStr Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title_full_unstemmed Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title_short Observation of Cooperative Purcell Enhancements in Antenna–Cavity Hybrids
title_sort observation of cooperative purcell enhancements in antenna–cavity hybrids
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7513474/
https://www.ncbi.nlm.nih.gov/pubmed/32870669
http://dx.doi.org/10.1021/acsnano.0c05233
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