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Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy

Flexible and self-powered deep ultraviolet (UV) photodetectors are pivotal for next-generation electronic skins to enrich human life quality. The fabrication of epitaxial β-Ga(2)O(3) thin films is challenging on flexible substrates due to high-temperature growth requirements. Herein, β-Ga(2)O(3) ([F...

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Autores principales: Tak, Bhera Ram, Yang, Ming-Min, Lai, Yu-Hong, Chu, Ying-Hao, Alexe, Marin, Singh, Rajendra
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7528161/
https://www.ncbi.nlm.nih.gov/pubmed/32999335
http://dx.doi.org/10.1038/s41598-020-73112-1
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author Tak, Bhera Ram
Yang, Ming-Min
Lai, Yu-Hong
Chu, Ying-Hao
Alexe, Marin
Singh, Rajendra
author_facet Tak, Bhera Ram
Yang, Ming-Min
Lai, Yu-Hong
Chu, Ying-Hao
Alexe, Marin
Singh, Rajendra
author_sort Tak, Bhera Ram
collection PubMed
description Flexible and self-powered deep ultraviolet (UV) photodetectors are pivotal for next-generation electronic skins to enrich human life quality. The fabrication of epitaxial β-Ga(2)O(3) thin films is challenging on flexible substrates due to high-temperature growth requirements. Herein, β-Ga(2)O(3) ([Formula: see text] 0 1) films are hetero-epitaxially grown on ultra-thin and environment-friendly muscovite mica which is the first time β-Ga(2)O(3) epitaxy growth on any flexible substrate. Integration of Gallium oxide with muscovite enables high-temperature processing as well as excellent flexibility compared to polymer substrates. Additionally, the metal–semiconductor-metal (MSM) photodetector on β-Ga(2)O(3) layer shows an ultra-low dark current of 800 fA at zero bias. The photovoltaic peak responsivity of 11.6 µA/W is obtained corresponding to very weak illumination of 75 μW/cm(2) of 265 nm wavelength. Thermally stimulated current (TSC) measurements are employed to investigate the optically active trap states. Among these traps, trap with an activation energy of 166 meV dominates the persistence photocurrent in the devices. Finally, photovoltaic detectors have shown excellent photocurrent stability under bending induced stress up to 0.32%. Hence, this novel heteroepitaxy opens the new way for flexible deep UV photodetectors.
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spelling pubmed-75281612020-10-02 Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy Tak, Bhera Ram Yang, Ming-Min Lai, Yu-Hong Chu, Ying-Hao Alexe, Marin Singh, Rajendra Sci Rep Article Flexible and self-powered deep ultraviolet (UV) photodetectors are pivotal for next-generation electronic skins to enrich human life quality. The fabrication of epitaxial β-Ga(2)O(3) thin films is challenging on flexible substrates due to high-temperature growth requirements. Herein, β-Ga(2)O(3) ([Formula: see text] 0 1) films are hetero-epitaxially grown on ultra-thin and environment-friendly muscovite mica which is the first time β-Ga(2)O(3) epitaxy growth on any flexible substrate. Integration of Gallium oxide with muscovite enables high-temperature processing as well as excellent flexibility compared to polymer substrates. Additionally, the metal–semiconductor-metal (MSM) photodetector on β-Ga(2)O(3) layer shows an ultra-low dark current of 800 fA at zero bias. The photovoltaic peak responsivity of 11.6 µA/W is obtained corresponding to very weak illumination of 75 μW/cm(2) of 265 nm wavelength. Thermally stimulated current (TSC) measurements are employed to investigate the optically active trap states. Among these traps, trap with an activation energy of 166 meV dominates the persistence photocurrent in the devices. Finally, photovoltaic detectors have shown excellent photocurrent stability under bending induced stress up to 0.32%. Hence, this novel heteroepitaxy opens the new way for flexible deep UV photodetectors. Nature Publishing Group UK 2020-09-30 /pmc/articles/PMC7528161/ /pubmed/32999335 http://dx.doi.org/10.1038/s41598-020-73112-1 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Tak, Bhera Ram
Yang, Ming-Min
Lai, Yu-Hong
Chu, Ying-Hao
Alexe, Marin
Singh, Rajendra
Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title_full Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title_fullStr Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title_full_unstemmed Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title_short Photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-Ga(2)O(3)/muscovite heteroepitaxy
title_sort photovoltaic and flexible deep ultraviolet wavelength detector based on novel β-ga(2)o(3)/muscovite heteroepitaxy
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7528161/
https://www.ncbi.nlm.nih.gov/pubmed/32999335
http://dx.doi.org/10.1038/s41598-020-73112-1
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