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Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data

X-ray dynamic tomographic microscopy offers new opportunities in the volumetric investigation of dynamic processes. Due to data complexity and their sheer amount, extraction of comprehensive quantitative information remains challenging due to the intensive manual interaction required. Particularly f...

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Autores principales: Bührer, Minna, Xu, Hong, Eller, Jens, Sijbers, Jan, Stampanoni, Marco, Marone, Federica
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7532214/
https://www.ncbi.nlm.nih.gov/pubmed/33009452
http://dx.doi.org/10.1038/s41598-020-73036-w
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author Bührer, Minna
Xu, Hong
Eller, Jens
Sijbers, Jan
Stampanoni, Marco
Marone, Federica
author_facet Bührer, Minna
Xu, Hong
Eller, Jens
Sijbers, Jan
Stampanoni, Marco
Marone, Federica
author_sort Bührer, Minna
collection PubMed
description X-ray dynamic tomographic microscopy offers new opportunities in the volumetric investigation of dynamic processes. Due to data complexity and their sheer amount, extraction of comprehensive quantitative information remains challenging due to the intensive manual interaction required. Particularly for dynamic investigations, these intensive manual requirements significantly extend the total data post-processing time, limiting possible dynamic analysis realistically to a few samples and time steps, hindering full exploitation of the new capabilities offered at dedicated time-resolved X-ray tomographic stations. In this paper, a fully automatized iterative tomographic reconstruction pipeline (rSIRT-PWC-DIFF) designed to reconstruct and segment dynamic processes within a static matrix is presented. The proposed algorithm includes automatic dynamic feature separation through difference sinograms, a virtual sinogram step for interior tomography datasets, time-regularization extended to small sub-regions for increased robustness and an automatic stopping criterion. We demonstrate the advantages of our approach on dynamic fuel cell data, for which the current data post-processing pipeline heavily relies on manual labor. The proposed approach reduces the post-processing time by at least a factor of 4 on limited computational resources. Full independence from manual interaction additionally allows straightforward up-scaling to efficiently process larger data, extensively boosting the possibilities in future dynamic X-ray tomographic investigations.
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spelling pubmed-75322142020-10-06 Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data Bührer, Minna Xu, Hong Eller, Jens Sijbers, Jan Stampanoni, Marco Marone, Federica Sci Rep Article X-ray dynamic tomographic microscopy offers new opportunities in the volumetric investigation of dynamic processes. Due to data complexity and their sheer amount, extraction of comprehensive quantitative information remains challenging due to the intensive manual interaction required. Particularly for dynamic investigations, these intensive manual requirements significantly extend the total data post-processing time, limiting possible dynamic analysis realistically to a few samples and time steps, hindering full exploitation of the new capabilities offered at dedicated time-resolved X-ray tomographic stations. In this paper, a fully automatized iterative tomographic reconstruction pipeline (rSIRT-PWC-DIFF) designed to reconstruct and segment dynamic processes within a static matrix is presented. The proposed algorithm includes automatic dynamic feature separation through difference sinograms, a virtual sinogram step for interior tomography datasets, time-regularization extended to small sub-regions for increased robustness and an automatic stopping criterion. We demonstrate the advantages of our approach on dynamic fuel cell data, for which the current data post-processing pipeline heavily relies on manual labor. The proposed approach reduces the post-processing time by at least a factor of 4 on limited computational resources. Full independence from manual interaction additionally allows straightforward up-scaling to efficiently process larger data, extensively boosting the possibilities in future dynamic X-ray tomographic investigations. Nature Publishing Group UK 2020-10-02 /pmc/articles/PMC7532214/ /pubmed/33009452 http://dx.doi.org/10.1038/s41598-020-73036-w Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Bührer, Minna
Xu, Hong
Eller, Jens
Sijbers, Jan
Stampanoni, Marco
Marone, Federica
Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title_full Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title_fullStr Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title_full_unstemmed Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title_short Unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
title_sort unveiling water dynamics in fuel cells from time-resolved tomographic microscopy data
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7532214/
https://www.ncbi.nlm.nih.gov/pubmed/33009452
http://dx.doi.org/10.1038/s41598-020-73036-w
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