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Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)

The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La(2)CuO(4) were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar therma...

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Autores principales: Boulanger, Marie-Eve, Grissonnanche, Gaël, Badoux, Sven, Allaire, Andréanne, Lefrançois, Étienne, Legros, Anaëlle, Gourgout, Adrien, Dion, Maxime, Wang, C. H., Chen, X. H., Liang, R., Hardy, W. N., Bonn, D. A., Taillefer, Louis
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7577976/
https://www.ncbi.nlm.nih.gov/pubmed/33087726
http://dx.doi.org/10.1038/s41467-020-18881-z
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author Boulanger, Marie-Eve
Grissonnanche, Gaël
Badoux, Sven
Allaire, Andréanne
Lefrançois, Étienne
Legros, Anaëlle
Gourgout, Adrien
Dion, Maxime
Wang, C. H.
Chen, X. H.
Liang, R.
Hardy, W. N.
Bonn, D. A.
Taillefer, Louis
author_facet Boulanger, Marie-Eve
Grissonnanche, Gaël
Badoux, Sven
Allaire, Andréanne
Lefrançois, Étienne
Legros, Anaëlle
Gourgout, Adrien
Dion, Maxime
Wang, C. H.
Chen, X. H.
Liang, R.
Hardy, W. N.
Bonn, D. A.
Taillefer, Louis
author_sort Boulanger, Marie-Eve
collection PubMed
description The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La(2)CuO(4) were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar thermal Hall conductivity in two cuprate Mott insulators with significantly different crystal structures and magnetic orders – Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2) – and show that two potential mechanisms can be excluded – the scattering of phonons by rare-earth impurities and by structural domains. Our comparative study further reveals that orthorhombicity, apical oxygens, the tilting of oxygen octahedra and the canting of spins out of the CuO(2) planes are not essential to the mechanism of chirality. Our findings point to a chiral mechanism coming from a coupling of acoustic phonons to the intrinsic excitations of the CuO(2) planes.
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spelling pubmed-75779762020-10-29 Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2) Boulanger, Marie-Eve Grissonnanche, Gaël Badoux, Sven Allaire, Andréanne Lefrançois, Étienne Legros, Anaëlle Gourgout, Adrien Dion, Maxime Wang, C. H. Chen, X. H. Liang, R. Hardy, W. N. Bonn, D. A. Taillefer, Louis Nat Commun Article The heat carriers responsible for the unexpectedly large thermal Hall conductivity of the cuprate Mott insulator La(2)CuO(4) were recently shown to be phonons. However, the mechanism by which phonons in cuprates acquire chirality in a magnetic field is still unknown. Here, we report a similar thermal Hall conductivity in two cuprate Mott insulators with significantly different crystal structures and magnetic orders – Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2) – and show that two potential mechanisms can be excluded – the scattering of phonons by rare-earth impurities and by structural domains. Our comparative study further reveals that orthorhombicity, apical oxygens, the tilting of oxygen octahedra and the canting of spins out of the CuO(2) planes are not essential to the mechanism of chirality. Our findings point to a chiral mechanism coming from a coupling of acoustic phonons to the intrinsic excitations of the CuO(2) planes. Nature Publishing Group UK 2020-10-21 /pmc/articles/PMC7577976/ /pubmed/33087726 http://dx.doi.org/10.1038/s41467-020-18881-z Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Boulanger, Marie-Eve
Grissonnanche, Gaël
Badoux, Sven
Allaire, Andréanne
Lefrançois, Étienne
Legros, Anaëlle
Gourgout, Adrien
Dion, Maxime
Wang, C. H.
Chen, X. H.
Liang, R.
Hardy, W. N.
Bonn, D. A.
Taillefer, Louis
Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title_full Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title_fullStr Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title_full_unstemmed Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title_short Thermal Hall conductivity in the cuprate Mott insulators Nd(2)CuO(4) and Sr(2)CuO(2)Cl(2)
title_sort thermal hall conductivity in the cuprate mott insulators nd(2)cuo(4) and sr(2)cuo(2)cl(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7577976/
https://www.ncbi.nlm.nih.gov/pubmed/33087726
http://dx.doi.org/10.1038/s41467-020-18881-z
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