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Fast CO(2) hydration kinetics impair heterogeneous but improve enzymatic CO(2) reduction catalysis

The performance of heterogeneous catalysts for electrocatalytic CO(2) reduction (CO(2)R) suffers from unwanted side reactions and kinetic inefficiencies at the required large overpotential. However, immobilised CO(2)R enzymes — such as formate dehydrogenase — can operate with high turnover and selec...

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Detalles Bibliográficos
Autores principales: Cobb, Samuel J., Badiani, Vivek M., Dharani, Azim M., Wagner, Andreas, Zacarias, Sónia, Olivera, Ana Rita, Pereira, Inês A. C., Reisner, Erwin
Formato: Online Artículo Texto
Lenguaje:English
Publicado: 2022
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7612589/
https://www.ncbi.nlm.nih.gov/pubmed/35228690
http://dx.doi.org/10.1038/s41557-021-00880-2