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State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods

Core–shell nanorods (NRs) with InGaN/GaN quantum wells (QWs) are promising for monolithic white light-emitting diodes and multi-color displays. Such applications, however, are still a challenge because intensity of the red band is too weak compared with blue and green. To clarify this problem, we me...

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Autores principales: Evropeitsev, Evgenii A., Kazanov, Dmitrii R., Robin, Yoann, Smirnov, Alexander N., Eliseyev, Ilya A., Davydov, Valery Yu., Toropov, Alexey A., Nitta, Shugo, Shubina, Tatiana V., Amano, Hiroshi
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7643183/
https://www.ncbi.nlm.nih.gov/pubmed/33149244
http://dx.doi.org/10.1038/s41598-020-76042-0
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author Evropeitsev, Evgenii A.
Kazanov, Dmitrii R.
Robin, Yoann
Smirnov, Alexander N.
Eliseyev, Ilya A.
Davydov, Valery Yu.
Toropov, Alexey A.
Nitta, Shugo
Shubina, Tatiana V.
Amano, Hiroshi
author_facet Evropeitsev, Evgenii A.
Kazanov, Dmitrii R.
Robin, Yoann
Smirnov, Alexander N.
Eliseyev, Ilya A.
Davydov, Valery Yu.
Toropov, Alexey A.
Nitta, Shugo
Shubina, Tatiana V.
Amano, Hiroshi
author_sort Evropeitsev, Evgenii A.
collection PubMed
description Core–shell nanorods (NRs) with InGaN/GaN quantum wells (QWs) are promising for monolithic white light-emitting diodes and multi-color displays. Such applications, however, are still a challenge because intensity of the red band is too weak compared with blue and green. To clarify this problem, we measured photoluminescence of different NRs, depending on power and temperature, as well as with time resolution. These studies have shown that dominant emission bands come from nonpolar and semipolar QWs, while a broad yellow-red band arises mainly from defects in the GaN core. An emission from polar QWs located at the NR tip is indistinguishable against the background of defect-related luminescence. Our calculations of electromagnetic field distribution inside the NRs show a low density of photon states at the tip, which additionally suppresses the radiation of polar QWs. We propose placing polar QWs inside a cylindrical part of the core, where the density of photon states is higher and the well area is much larger. Such a hybrid design, in which the excess of blue radiation from shell QWs is converted to red radiation in core wells, can help solve the urgent problem of red light for many applications of NRs.
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spelling pubmed-76431832020-11-06 State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods Evropeitsev, Evgenii A. Kazanov, Dmitrii R. Robin, Yoann Smirnov, Alexander N. Eliseyev, Ilya A. Davydov, Valery Yu. Toropov, Alexey A. Nitta, Shugo Shubina, Tatiana V. Amano, Hiroshi Sci Rep Article Core–shell nanorods (NRs) with InGaN/GaN quantum wells (QWs) are promising for monolithic white light-emitting diodes and multi-color displays. Such applications, however, are still a challenge because intensity of the red band is too weak compared with blue and green. To clarify this problem, we measured photoluminescence of different NRs, depending on power and temperature, as well as with time resolution. These studies have shown that dominant emission bands come from nonpolar and semipolar QWs, while a broad yellow-red band arises mainly from defects in the GaN core. An emission from polar QWs located at the NR tip is indistinguishable against the background of defect-related luminescence. Our calculations of electromagnetic field distribution inside the NRs show a low density of photon states at the tip, which additionally suppresses the radiation of polar QWs. We propose placing polar QWs inside a cylindrical part of the core, where the density of photon states is higher and the well area is much larger. Such a hybrid design, in which the excess of blue radiation from shell QWs is converted to red radiation in core wells, can help solve the urgent problem of red light for many applications of NRs. Nature Publishing Group UK 2020-11-04 /pmc/articles/PMC7643183/ /pubmed/33149244 http://dx.doi.org/10.1038/s41598-020-76042-0 Text en © The Author(s) 2020 Open AccessThis article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Evropeitsev, Evgenii A.
Kazanov, Dmitrii R.
Robin, Yoann
Smirnov, Alexander N.
Eliseyev, Ilya A.
Davydov, Valery Yu.
Toropov, Alexey A.
Nitta, Shugo
Shubina, Tatiana V.
Amano, Hiroshi
State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title_full State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title_fullStr State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title_full_unstemmed State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title_short State-of-the-art and prospects for intense red radiation from core–shell InGaN/GaN nanorods
title_sort state-of-the-art and prospects for intense red radiation from core–shell ingan/gan nanorods
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7643183/
https://www.ncbi.nlm.nih.gov/pubmed/33149244
http://dx.doi.org/10.1038/s41598-020-76042-0
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