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Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces

[Image: see text] We studied the impact dynamics of a droplet on two types of surfaces, i.e., nanostructured/hierarchical (NS/HS) surfaces, with different extents of hydrophobicity. It was found that the contact time is related to wetting hysteresis. It can be concluded that wetting hysteresis plays...

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Autores principales: Li, Jiang, Wang, Wenjun, Mei, Xuesong, Pan, Aifei
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7659140/
https://www.ncbi.nlm.nih.gov/pubmed/33195931
http://dx.doi.org/10.1021/acsomega.0c04106
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author Li, Jiang
Wang, Wenjun
Mei, Xuesong
Pan, Aifei
author_facet Li, Jiang
Wang, Wenjun
Mei, Xuesong
Pan, Aifei
author_sort Li, Jiang
collection PubMed
description [Image: see text] We studied the impact dynamics of a droplet on two types of surfaces, i.e., nanostructured/hierarchical (NS/HS) surfaces, with different extents of hydrophobicity. It was found that the contact time is related to wetting hysteresis. It can be concluded that wetting hysteresis plays a significant role in the contact process of bouncing drops based on the work done against resistance produced by contact angle hysteresis (CAH). For similar surface roughness, the work done by CAH dominates, and a lower CAH creates a smaller contact time. Compared with NS surfaces, the energy stored during the Cassie–Baxter/Wenzel state transition because of the more pronounced air pocket formation provides the upward kinetic energy, resulting in rapid detachment of a droplet from HS surfaces. Thus, HS-3 has a smaller contact/elongation time (∼8/2 ms) because of the enhanced air pocket formation and more favorable wettability (larger contact angle (CA) and smaller contact angle hysteresis (CAH)) than other surfaces. In addition, the results show that surface morphology affects the contact time of bouncing drops mainly by influencing the elongation stage. For different Weber numbers (We), the upward energy storage dominates and results in different varying trends of contact time with We for NS-3 and HS-3. For further study, the morphology evolution of bouncing drops with We was also investigated in detail. The results show that a satellite droplet is launched in a certain We range because of high adhesion resulting from the Cassie–Baxter/Wenzel state transition. These findings provide guidelines for the preparation of surfaces for both self-cleaning and anti-icing purposes.
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spelling pubmed-76591402020-11-13 Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces Li, Jiang Wang, Wenjun Mei, Xuesong Pan, Aifei ACS Omega [Image: see text] We studied the impact dynamics of a droplet on two types of surfaces, i.e., nanostructured/hierarchical (NS/HS) surfaces, with different extents of hydrophobicity. It was found that the contact time is related to wetting hysteresis. It can be concluded that wetting hysteresis plays a significant role in the contact process of bouncing drops based on the work done against resistance produced by contact angle hysteresis (CAH). For similar surface roughness, the work done by CAH dominates, and a lower CAH creates a smaller contact time. Compared with NS surfaces, the energy stored during the Cassie–Baxter/Wenzel state transition because of the more pronounced air pocket formation provides the upward kinetic energy, resulting in rapid detachment of a droplet from HS surfaces. Thus, HS-3 has a smaller contact/elongation time (∼8/2 ms) because of the enhanced air pocket formation and more favorable wettability (larger contact angle (CA) and smaller contact angle hysteresis (CAH)) than other surfaces. In addition, the results show that surface morphology affects the contact time of bouncing drops mainly by influencing the elongation stage. For different Weber numbers (We), the upward energy storage dominates and results in different varying trends of contact time with We for NS-3 and HS-3. For further study, the morphology evolution of bouncing drops with We was also investigated in detail. The results show that a satellite droplet is launched in a certain We range because of high adhesion resulting from the Cassie–Baxter/Wenzel state transition. These findings provide guidelines for the preparation of surfaces for both self-cleaning and anti-icing purposes. American Chemical Society 2020-10-30 /pmc/articles/PMC7659140/ /pubmed/33195931 http://dx.doi.org/10.1021/acsomega.0c04106 Text en © 2020 The Authors. Published by American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Li, Jiang
Wang, Wenjun
Mei, Xuesong
Pan, Aifei
Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title_full Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title_fullStr Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title_full_unstemmed Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title_short Effects of Surface Wettability on the Dewetting Performance of Hydrophobic Surfaces
title_sort effects of surface wettability on the dewetting performance of hydrophobic surfaces
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7659140/
https://www.ncbi.nlm.nih.gov/pubmed/33195931
http://dx.doi.org/10.1021/acsomega.0c04106
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