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Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal

Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications....

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Detalles Bibliográficos
Autores principales: Han, Fei, Andrejevic, Nina, Nguyen, Thanh, Kozii, Vladyslav, Nguyen, Quynh T., Hogan, Tom, Ding, Zhiwei, Pablo-Pedro, Ricardo, Parjan, Shreya, Skinner, Brian, Alatas, Ahmet, Alp, Ercan, Chi, Songxue, Fernandez-Baca, Jaime, Huang, Shengxi, Fu, Liang, Li, Mingda
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7710760/
https://www.ncbi.nlm.nih.gov/pubmed/33268778
http://dx.doi.org/10.1038/s41467-020-19850-2
Descripción
Sumario:Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric Hall effect in the topological Weyl semimetal (WSM) tantalum phosphide (TaP). An ultrahigh longitudinal thermopower [Formula: see text] and giant power factor [Formula: see text] are observed at ~40 K, which is largely attributed to the quantized thermoelectric Hall effect. Our work highlights the unique quantized thermoelectric Hall effect realized in a WSM toward low-temperature energy harvesting applications.