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Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal

Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications....

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Autores principales: Han, Fei, Andrejevic, Nina, Nguyen, Thanh, Kozii, Vladyslav, Nguyen, Quynh T., Hogan, Tom, Ding, Zhiwei, Pablo-Pedro, Ricardo, Parjan, Shreya, Skinner, Brian, Alatas, Ahmet, Alp, Ercan, Chi, Songxue, Fernandez-Baca, Jaime, Huang, Shengxi, Fu, Liang, Li, Mingda
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7710760/
https://www.ncbi.nlm.nih.gov/pubmed/33268778
http://dx.doi.org/10.1038/s41467-020-19850-2
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author Han, Fei
Andrejevic, Nina
Nguyen, Thanh
Kozii, Vladyslav
Nguyen, Quynh T.
Hogan, Tom
Ding, Zhiwei
Pablo-Pedro, Ricardo
Parjan, Shreya
Skinner, Brian
Alatas, Ahmet
Alp, Ercan
Chi, Songxue
Fernandez-Baca, Jaime
Huang, Shengxi
Fu, Liang
Li, Mingda
author_facet Han, Fei
Andrejevic, Nina
Nguyen, Thanh
Kozii, Vladyslav
Nguyen, Quynh T.
Hogan, Tom
Ding, Zhiwei
Pablo-Pedro, Ricardo
Parjan, Shreya
Skinner, Brian
Alatas, Ahmet
Alp, Ercan
Chi, Songxue
Fernandez-Baca, Jaime
Huang, Shengxi
Fu, Liang
Li, Mingda
author_sort Han, Fei
collection PubMed
description Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric Hall effect in the topological Weyl semimetal (WSM) tantalum phosphide (TaP). An ultrahigh longitudinal thermopower [Formula: see text] and giant power factor [Formula: see text] are observed at ~40 K, which is largely attributed to the quantized thermoelectric Hall effect. Our work highlights the unique quantized thermoelectric Hall effect realized in a WSM toward low-temperature energy harvesting applications.
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spelling pubmed-77107602020-12-03 Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal Han, Fei Andrejevic, Nina Nguyen, Thanh Kozii, Vladyslav Nguyen, Quynh T. Hogan, Tom Ding, Zhiwei Pablo-Pedro, Ricardo Parjan, Shreya Skinner, Brian Alatas, Ahmet Alp, Ercan Chi, Songxue Fernandez-Baca, Jaime Huang, Shengxi Fu, Liang Li, Mingda Nat Commun Article Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric Hall effect in the topological Weyl semimetal (WSM) tantalum phosphide (TaP). An ultrahigh longitudinal thermopower [Formula: see text] and giant power factor [Formula: see text] are observed at ~40 K, which is largely attributed to the quantized thermoelectric Hall effect. Our work highlights the unique quantized thermoelectric Hall effect realized in a WSM toward low-temperature energy harvesting applications. Nature Publishing Group UK 2020-12-02 /pmc/articles/PMC7710760/ /pubmed/33268778 http://dx.doi.org/10.1038/s41467-020-19850-2 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/.
spellingShingle Article
Han, Fei
Andrejevic, Nina
Nguyen, Thanh
Kozii, Vladyslav
Nguyen, Quynh T.
Hogan, Tom
Ding, Zhiwei
Pablo-Pedro, Ricardo
Parjan, Shreya
Skinner, Brian
Alatas, Ahmet
Alp, Ercan
Chi, Songxue
Fernandez-Baca, Jaime
Huang, Shengxi
Fu, Liang
Li, Mingda
Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title_full Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title_fullStr Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title_full_unstemmed Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title_short Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
title_sort quantized thermoelectric hall effect induces giant power factor in a topological semimetal
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7710760/
https://www.ncbi.nlm.nih.gov/pubmed/33268778
http://dx.doi.org/10.1038/s41467-020-19850-2
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