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Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal
Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications....
Autores principales: | , , , , , , , , , , , , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
Nature Publishing Group UK
2020
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Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7710760/ https://www.ncbi.nlm.nih.gov/pubmed/33268778 http://dx.doi.org/10.1038/s41467-020-19850-2 |
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author | Han, Fei Andrejevic, Nina Nguyen, Thanh Kozii, Vladyslav Nguyen, Quynh T. Hogan, Tom Ding, Zhiwei Pablo-Pedro, Ricardo Parjan, Shreya Skinner, Brian Alatas, Ahmet Alp, Ercan Chi, Songxue Fernandez-Baca, Jaime Huang, Shengxi Fu, Liang Li, Mingda |
author_facet | Han, Fei Andrejevic, Nina Nguyen, Thanh Kozii, Vladyslav Nguyen, Quynh T. Hogan, Tom Ding, Zhiwei Pablo-Pedro, Ricardo Parjan, Shreya Skinner, Brian Alatas, Ahmet Alp, Ercan Chi, Songxue Fernandez-Baca, Jaime Huang, Shengxi Fu, Liang Li, Mingda |
author_sort | Han, Fei |
collection | PubMed |
description | Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric Hall effect in the topological Weyl semimetal (WSM) tantalum phosphide (TaP). An ultrahigh longitudinal thermopower [Formula: see text] and giant power factor [Formula: see text] are observed at ~40 K, which is largely attributed to the quantized thermoelectric Hall effect. Our work highlights the unique quantized thermoelectric Hall effect realized in a WSM toward low-temperature energy harvesting applications. |
format | Online Article Text |
id | pubmed-7710760 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | Nature Publishing Group UK |
record_format | MEDLINE/PubMed |
spelling | pubmed-77107602020-12-03 Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal Han, Fei Andrejevic, Nina Nguyen, Thanh Kozii, Vladyslav Nguyen, Quynh T. Hogan, Tom Ding, Zhiwei Pablo-Pedro, Ricardo Parjan, Shreya Skinner, Brian Alatas, Ahmet Alp, Ercan Chi, Songxue Fernandez-Baca, Jaime Huang, Shengxi Fu, Liang Li, Mingda Nat Commun Article Thermoelectrics are promising by directly generating electricity from waste heat. However, (sub-)room-temperature thermoelectrics have been a long-standing challenge due to vanishing electronic entropy at low temperatures. Topological materials offer a new avenue for energy harvesting applications. Recent theories predicted that topological semimetals at the quantum limit can lead to a large, non-saturating thermopower and a quantized thermoelectric Hall conductivity approaching a universal value. Here, we experimentally demonstrate the non-saturating thermopower and quantized thermoelectric Hall effect in the topological Weyl semimetal (WSM) tantalum phosphide (TaP). An ultrahigh longitudinal thermopower [Formula: see text] and giant power factor [Formula: see text] are observed at ~40 K, which is largely attributed to the quantized thermoelectric Hall effect. Our work highlights the unique quantized thermoelectric Hall effect realized in a WSM toward low-temperature energy harvesting applications. Nature Publishing Group UK 2020-12-02 /pmc/articles/PMC7710760/ /pubmed/33268778 http://dx.doi.org/10.1038/s41467-020-19850-2 Text en © The Author(s) 2020 Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/. |
spellingShingle | Article Han, Fei Andrejevic, Nina Nguyen, Thanh Kozii, Vladyslav Nguyen, Quynh T. Hogan, Tom Ding, Zhiwei Pablo-Pedro, Ricardo Parjan, Shreya Skinner, Brian Alatas, Ahmet Alp, Ercan Chi, Songxue Fernandez-Baca, Jaime Huang, Shengxi Fu, Liang Li, Mingda Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title | Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title_full | Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title_fullStr | Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title_full_unstemmed | Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title_short | Quantized thermoelectric Hall effect induces giant power factor in a topological semimetal |
title_sort | quantized thermoelectric hall effect induces giant power factor in a topological semimetal |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7710760/ https://www.ncbi.nlm.nih.gov/pubmed/33268778 http://dx.doi.org/10.1038/s41467-020-19850-2 |
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