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CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification

[Image: see text] Solar-driven water evaporation has been proven to be a promising and efficient method for the energy crisis and clean water shortage issues. Herein, we strategically design and fabricate a novel nonstoichiometric CoWO(4–x)-deposited foam nickel (NF) membrane (CoWO(4–x)@NF) that pos...

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Autores principales: Liu, Haixia, Yang, Chunyu, Guo, Wei, Zhang, Feng, Lin, Huiming, Zhao, Le, Ma, Tianyue, Lu, Xinxin, Qu, Fengyu
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7745215/
https://www.ncbi.nlm.nih.gov/pubmed/33344812
http://dx.doi.org/10.1021/acsomega.0c03887
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author Liu, Haixia
Yang, Chunyu
Guo, Wei
Zhang, Feng
Lin, Huiming
Zhao, Le
Ma, Tianyue
Lu, Xinxin
Qu, Fengyu
author_facet Liu, Haixia
Yang, Chunyu
Guo, Wei
Zhang, Feng
Lin, Huiming
Zhao, Le
Ma, Tianyue
Lu, Xinxin
Qu, Fengyu
author_sort Liu, Haixia
collection PubMed
description [Image: see text] Solar-driven water evaporation has been proven to be a promising and efficient method for the energy crisis and clean water shortage issues. Herein, we strategically design and fabricate a novel nonstoichiometric CoWO(4–x)-deposited foam nickel (NF) membrane (CoWO(4–x)@NF) that possesses all the desirable optical, thermal, and wetting properties for efficient water evaporation and purification. The broadband absorption of CoWO(4–x) nanoparticles (NPs) obtained by hydrogen reduction contributes to light-to-heat conversion, while NF with a three-dimensional porous structure can support CoWO(4–x) NPs and ensure the rapid flow of water molecules during the water evaporation process. We systematically explore and compare the outdoor water evaporation performance of the pure water group, NF group, and CoWO(4–x)@NF group, and the results show that CoWO(4–x)@NF performs well under natural sunlight irradiation (water evaporation: 2.91 kg m(–2)). Significantly, under solar irradiation, the remarkable reduction of Cyanophyta and Euglenophyta in lake water is achieved in the CoWO(4–x)@NF membrane-administered group, and these two algae are the main factors for eutrophication of the lake water. Our work highlights the great potentials of the CoWO(4–x)@NF membrane as a device for realizing outdoor solar energy-driven water evaporation and proposes a new strategy for purifying the eutrophication of the lake water.
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spelling pubmed-77452152020-12-18 CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification Liu, Haixia Yang, Chunyu Guo, Wei Zhang, Feng Lin, Huiming Zhao, Le Ma, Tianyue Lu, Xinxin Qu, Fengyu ACS Omega [Image: see text] Solar-driven water evaporation has been proven to be a promising and efficient method for the energy crisis and clean water shortage issues. Herein, we strategically design and fabricate a novel nonstoichiometric CoWO(4–x)-deposited foam nickel (NF) membrane (CoWO(4–x)@NF) that possesses all the desirable optical, thermal, and wetting properties for efficient water evaporation and purification. The broadband absorption of CoWO(4–x) nanoparticles (NPs) obtained by hydrogen reduction contributes to light-to-heat conversion, while NF with a three-dimensional porous structure can support CoWO(4–x) NPs and ensure the rapid flow of water molecules during the water evaporation process. We systematically explore and compare the outdoor water evaporation performance of the pure water group, NF group, and CoWO(4–x)@NF group, and the results show that CoWO(4–x)@NF performs well under natural sunlight irradiation (water evaporation: 2.91 kg m(–2)). Significantly, under solar irradiation, the remarkable reduction of Cyanophyta and Euglenophyta in lake water is achieved in the CoWO(4–x)@NF membrane-administered group, and these two algae are the main factors for eutrophication of the lake water. Our work highlights the great potentials of the CoWO(4–x)@NF membrane as a device for realizing outdoor solar energy-driven water evaporation and proposes a new strategy for purifying the eutrophication of the lake water. American Chemical Society 2020-12-03 /pmc/articles/PMC7745215/ /pubmed/33344812 http://dx.doi.org/10.1021/acsomega.0c03887 Text en © 2020 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes.
spellingShingle Liu, Haixia
Yang, Chunyu
Guo, Wei
Zhang, Feng
Lin, Huiming
Zhao, Le
Ma, Tianyue
Lu, Xinxin
Qu, Fengyu
CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title_full CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title_fullStr CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title_full_unstemmed CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title_short CoWO(4–x)-Based Photothermal Membranes for Solar-Driven Water Evaporation and Eutrophic Lake Water Purification
title_sort cowo(4–x)-based photothermal membranes for solar-driven water evaporation and eutrophic lake water purification
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7745215/
https://www.ncbi.nlm.nih.gov/pubmed/33344812
http://dx.doi.org/10.1021/acsomega.0c03887
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