Cargando…

Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration

[Image: see text] The development of high-efficiency and low-cost new catalysts is an extremely attractive topic. In this study, two different matrix bentonite-modified fly ash catalysts were successfully prepared, and the compressive strength of the catalyst was studied by using unsaturated dynamic...

Descripción completa

Detalles Bibliográficos
Autores principales: Lei, Zhang, Lingbo, Qi, Hao, Shu, Yang, Jia, Chao, Yang, Fang, Bai, Zhiyu, Sun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7745216/
https://www.ncbi.nlm.nih.gov/pubmed/33344809
http://dx.doi.org/10.1021/acsomega.0c03642
_version_ 1783624569136873472
author Lei, Zhang
Lingbo, Qi
Hao, Shu
Yang, Jia
Lei, Zhang
Chao, Yang
Fang, Bai
Zhiyu, Sun
author_facet Lei, Zhang
Lingbo, Qi
Hao, Shu
Yang, Jia
Lei, Zhang
Chao, Yang
Fang, Bai
Zhiyu, Sun
author_sort Lei, Zhang
collection PubMed
description [Image: see text] The development of high-efficiency and low-cost new catalysts is an extremely attractive topic. In this study, two different matrix bentonite-modified fly ash catalysts were successfully prepared, and the compressive strength of the catalyst was studied by using unsaturated dynamic and static triaxial technology. The axial compressive strength of FC (fly ash catalysts added with Ca-based bentonite) was greater than that of FN (fly ash catalysts added with Na-based bentonite). The catalyst reached 978 kPa. The prepared catalyst was characterized by X-ray diffraction analysis, Fourier transform infrared spectroscopy, scanning electron microscopy, and specific surface area analysis (BET) of the catalyst. In addition, denitration performance of different catalysts was explored, and the reaction conditions were optimized. The results demonstrate that when the mixing ratio of fly ash and calcium-based bentonite in the FC is 4:1, the compressive strength is relatively high, and the denitration rate reaches about 82%.
format Online
Article
Text
id pubmed-7745216
institution National Center for Biotechnology Information
language English
publishDate 2020
publisher American Chemical Society
record_format MEDLINE/PubMed
spelling pubmed-77452162020-12-18 Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration Lei, Zhang Lingbo, Qi Hao, Shu Yang, Jia Lei, Zhang Chao, Yang Fang, Bai Zhiyu, Sun ACS Omega [Image: see text] The development of high-efficiency and low-cost new catalysts is an extremely attractive topic. In this study, two different matrix bentonite-modified fly ash catalysts were successfully prepared, and the compressive strength of the catalyst was studied by using unsaturated dynamic and static triaxial technology. The axial compressive strength of FC (fly ash catalysts added with Ca-based bentonite) was greater than that of FN (fly ash catalysts added with Na-based bentonite). The catalyst reached 978 kPa. The prepared catalyst was characterized by X-ray diffraction analysis, Fourier transform infrared spectroscopy, scanning electron microscopy, and specific surface area analysis (BET) of the catalyst. In addition, denitration performance of different catalysts was explored, and the reaction conditions were optimized. The results demonstrate that when the mixing ratio of fly ash and calcium-based bentonite in the FC is 4:1, the compressive strength is relatively high, and the denitration rate reaches about 82%. American Chemical Society 2020-12-02 /pmc/articles/PMC7745216/ /pubmed/33344809 http://dx.doi.org/10.1021/acsomega.0c03642 Text en © 2020 The Authors. Published by American Chemical Society This is an open access article published under an ACS AuthorChoice License (http://pubs.acs.org/page/policy/authorchoice_termsofuse.html) , which permits copying and redistribution of the article or any adaptations for non-commercial purposes.
spellingShingle Lei, Zhang
Lingbo, Qi
Hao, Shu
Yang, Jia
Lei, Zhang
Chao, Yang
Fang, Bai
Zhiyu, Sun
Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title_full Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title_fullStr Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title_full_unstemmed Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title_short Formation of Fly Ash Catalysts and Selection of a Matrix Binder and Its Application in Denitration
title_sort formation of fly ash catalysts and selection of a matrix binder and its application in denitration
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7745216/
https://www.ncbi.nlm.nih.gov/pubmed/33344809
http://dx.doi.org/10.1021/acsomega.0c03642
work_keys_str_mv AT leizhang formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT lingboqi formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT haoshu formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT yangjia formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT leizhang formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT chaoyang formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT fangbai formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration
AT zhiyusun formationofflyashcatalystsandselectionofamatrixbinderanditsapplicationindenitration