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Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
[Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodolo...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American
Chemical Society
2020
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7760215/ https://www.ncbi.nlm.nih.gov/pubmed/33290656 http://dx.doi.org/10.1021/acsnano.0c07763 |
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author | Jones, Steven Andrén, Daniel Antosiewicz, Tomasz J. Stilgoe, Alexander Rubinsztein-Dunlop, Halina Käll, Mikael |
author_facet | Jones, Steven Andrén, Daniel Antosiewicz, Tomasz J. Stilgoe, Alexander Rubinsztein-Dunlop, Halina Käll, Mikael |
author_sort | Jones, Steven |
collection | PubMed |
description | [Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodology for the robust generation and precise quantification of extremely strong flow transients driven by vapor bubble nucleation on spatially isolated plasmonic nanoantennas excited by light. The system is capable of producing peak flow speeds of the order mm/s at modulation rates up to ∼100 Hz in water, thus allowing for a variety of high-throughput applications. Analysis of flow dynamics and fluid viscosity dependence indicates that the transient originates in the rapid bubble expansion that follows nucleation rather than being strictly thermocapillary in nature. |
format | Online Article Text |
id | pubmed-7760215 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | American
Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-77602152020-12-28 Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation Jones, Steven Andrén, Daniel Antosiewicz, Tomasz J. Stilgoe, Alexander Rubinsztein-Dunlop, Halina Käll, Mikael ACS Nano [Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodology for the robust generation and precise quantification of extremely strong flow transients driven by vapor bubble nucleation on spatially isolated plasmonic nanoantennas excited by light. The system is capable of producing peak flow speeds of the order mm/s at modulation rates up to ∼100 Hz in water, thus allowing for a variety of high-throughput applications. Analysis of flow dynamics and fluid viscosity dependence indicates that the transient originates in the rapid bubble expansion that follows nucleation rather than being strictly thermocapillary in nature. American Chemical Society 2020-12-08 2020-12-22 /pmc/articles/PMC7760215/ /pubmed/33290656 http://dx.doi.org/10.1021/acsnano.0c07763 Text en © 2020 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited. |
spellingShingle | Jones, Steven Andrén, Daniel Antosiewicz, Tomasz J. Stilgoe, Alexander Rubinsztein-Dunlop, Halina Käll, Mikael Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation |
title | Strong
Transient Flows Generated by Thermoplasmonic
Bubble Nucleation |
title_full | Strong
Transient Flows Generated by Thermoplasmonic
Bubble Nucleation |
title_fullStr | Strong
Transient Flows Generated by Thermoplasmonic
Bubble Nucleation |
title_full_unstemmed | Strong
Transient Flows Generated by Thermoplasmonic
Bubble Nucleation |
title_short | Strong
Transient Flows Generated by Thermoplasmonic
Bubble Nucleation |
title_sort | strong
transient flows generated by thermoplasmonic
bubble nucleation |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7760215/ https://www.ncbi.nlm.nih.gov/pubmed/33290656 http://dx.doi.org/10.1021/acsnano.0c07763 |
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