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Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation

[Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodolo...

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Autores principales: Jones, Steven, Andrén, Daniel, Antosiewicz, Tomasz J., Stilgoe, Alexander, Rubinsztein-Dunlop, Halina, Käll, Mikael
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7760215/
https://www.ncbi.nlm.nih.gov/pubmed/33290656
http://dx.doi.org/10.1021/acsnano.0c07763
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author Jones, Steven
Andrén, Daniel
Antosiewicz, Tomasz J.
Stilgoe, Alexander
Rubinsztein-Dunlop, Halina
Käll, Mikael
author_facet Jones, Steven
Andrén, Daniel
Antosiewicz, Tomasz J.
Stilgoe, Alexander
Rubinsztein-Dunlop, Halina
Käll, Mikael
author_sort Jones, Steven
collection PubMed
description [Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodology for the robust generation and precise quantification of extremely strong flow transients driven by vapor bubble nucleation on spatially isolated plasmonic nanoantennas excited by light. The system is capable of producing peak flow speeds of the order mm/s at modulation rates up to ∼100 Hz in water, thus allowing for a variety of high-throughput applications. Analysis of flow dynamics and fluid viscosity dependence indicates that the transient originates in the rapid bubble expansion that follows nucleation rather than being strictly thermocapillary in nature.
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spelling pubmed-77602152020-12-28 Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation Jones, Steven Andrén, Daniel Antosiewicz, Tomasz J. Stilgoe, Alexander Rubinsztein-Dunlop, Halina Käll, Mikael ACS Nano [Image: see text] The challenge of inducing and controlling localized fluid flows for generic force actuation and for achieving efficient mass transport in microfluidics is key to the development of next-generation miniaturized systems for chemistry and life sciences. Here we demonstrate a methodology for the robust generation and precise quantification of extremely strong flow transients driven by vapor bubble nucleation on spatially isolated plasmonic nanoantennas excited by light. The system is capable of producing peak flow speeds of the order mm/s at modulation rates up to ∼100 Hz in water, thus allowing for a variety of high-throughput applications. Analysis of flow dynamics and fluid viscosity dependence indicates that the transient originates in the rapid bubble expansion that follows nucleation rather than being strictly thermocapillary in nature. American Chemical Society 2020-12-08 2020-12-22 /pmc/articles/PMC7760215/ /pubmed/33290656 http://dx.doi.org/10.1021/acsnano.0c07763 Text en © 2020 American Chemical Society This is an open access article published under a Creative Commons Attribution (CC-BY) License (http://pubs.acs.org/page/policy/authorchoice_ccby_termsofuse.html) , which permits unrestricted use, distribution and reproduction in any medium, provided the author and source are cited.
spellingShingle Jones, Steven
Andrén, Daniel
Antosiewicz, Tomasz J.
Stilgoe, Alexander
Rubinsztein-Dunlop, Halina
Käll, Mikael
Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title_full Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title_fullStr Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title_full_unstemmed Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title_short Strong Transient Flows Generated by Thermoplasmonic Bubble Nucleation
title_sort strong transient flows generated by thermoplasmonic bubble nucleation
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7760215/
https://www.ncbi.nlm.nih.gov/pubmed/33290656
http://dx.doi.org/10.1021/acsnano.0c07763
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