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Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials

[Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells,...

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Autores principales: Bisen, Omeshwari Yadorao, Nandan, Ravi, Nanda, Karuna Kar
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Chemical Society 2020
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7774072/
https://www.ncbi.nlm.nih.gov/pubmed/33403245
http://dx.doi.org/10.1021/acsomega.0c04432
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author Bisen, Omeshwari Yadorao
Nandan, Ravi
Nanda, Karuna Kar
author_facet Bisen, Omeshwari Yadorao
Nandan, Ravi
Nanda, Karuna Kar
author_sort Bisen, Omeshwari Yadorao
collection PubMed
description [Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells, electrolyzers, and metal–air batteries. In this regard, we focus on three important categories of carbonaceous material, namely, metal-free heteroatom doped, transition metal heteroatom codoped, and carbon nitride (C(3)N(4)) based hybrid materials. Implications of various strategies, using one-step pyrolysis technique have been discussed for the effective design of heteroatom modified carbonaceous electrocatalysts. In this minireview, we outline the richness of one-step strategy for designing electrochemically active heteroatom doped carbon, transition metal–heteroatom codoped carbon, and C(3)N(4) derived hybrid materials in the perspective of electrochemical energy conversion and storage devices. We also outline the future research direction in the development of highly efficient and sustainable electrocatalysts for oxygen electrochemistry. Finally, we wind up the article with the challenges and outlook on heteroatoms and transition metal–heteroatom codoped carbon material as an efficient and low-cost electrocatalysts, thereby promoting the development of this important area.
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spelling pubmed-77740722021-01-04 Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials Bisen, Omeshwari Yadorao Nandan, Ravi Nanda, Karuna Kar ACS Omega [Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells, electrolyzers, and metal–air batteries. In this regard, we focus on three important categories of carbonaceous material, namely, metal-free heteroatom doped, transition metal heteroatom codoped, and carbon nitride (C(3)N(4)) based hybrid materials. Implications of various strategies, using one-step pyrolysis technique have been discussed for the effective design of heteroatom modified carbonaceous electrocatalysts. In this minireview, we outline the richness of one-step strategy for designing electrochemically active heteroatom doped carbon, transition metal–heteroatom codoped carbon, and C(3)N(4) derived hybrid materials in the perspective of electrochemical energy conversion and storage devices. We also outline the future research direction in the development of highly efficient and sustainable electrocatalysts for oxygen electrochemistry. Finally, we wind up the article with the challenges and outlook on heteroatoms and transition metal–heteroatom codoped carbon material as an efficient and low-cost electrocatalysts, thereby promoting the development of this important area. American Chemical Society 2020-12-14 /pmc/articles/PMC7774072/ /pubmed/33403245 http://dx.doi.org/10.1021/acsomega.0c04432 Text en © 2020 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes.
spellingShingle Bisen, Omeshwari Yadorao
Nandan, Ravi
Nanda, Karuna Kar
Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title_full Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title_fullStr Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title_full_unstemmed Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title_short Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
title_sort unique one-step strategy for nonmetallic and metallic heteroatom doped carbonaceous materials
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7774072/
https://www.ncbi.nlm.nih.gov/pubmed/33403245
http://dx.doi.org/10.1021/acsomega.0c04432
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