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Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials
[Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells,...
Autores principales: | , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2020
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7774072/ https://www.ncbi.nlm.nih.gov/pubmed/33403245 http://dx.doi.org/10.1021/acsomega.0c04432 |
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author | Bisen, Omeshwari Yadorao Nandan, Ravi Nanda, Karuna Kar |
author_facet | Bisen, Omeshwari Yadorao Nandan, Ravi Nanda, Karuna Kar |
author_sort | Bisen, Omeshwari Yadorao |
collection | PubMed |
description | [Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells, electrolyzers, and metal–air batteries. In this regard, we focus on three important categories of carbonaceous material, namely, metal-free heteroatom doped, transition metal heteroatom codoped, and carbon nitride (C(3)N(4)) based hybrid materials. Implications of various strategies, using one-step pyrolysis technique have been discussed for the effective design of heteroatom modified carbonaceous electrocatalysts. In this minireview, we outline the richness of one-step strategy for designing electrochemically active heteroatom doped carbon, transition metal–heteroatom codoped carbon, and C(3)N(4) derived hybrid materials in the perspective of electrochemical energy conversion and storage devices. We also outline the future research direction in the development of highly efficient and sustainable electrocatalysts for oxygen electrochemistry. Finally, we wind up the article with the challenges and outlook on heteroatoms and transition metal–heteroatom codoped carbon material as an efficient and low-cost electrocatalysts, thereby promoting the development of this important area. |
format | Online Article Text |
id | pubmed-7774072 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2020 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-77740722021-01-04 Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials Bisen, Omeshwari Yadorao Nandan, Ravi Nanda, Karuna Kar ACS Omega [Image: see text] Nonmetallic and metallic heteroatom doped carbonaceous materials have garnered tremendous research attention due to a potential replacement to the precious Pt-group and (Ru, Ir)-oxide based catalysts and are essential part of the next-generation electrode catalysts for fuel cells, electrolyzers, and metal–air batteries. In this regard, we focus on three important categories of carbonaceous material, namely, metal-free heteroatom doped, transition metal heteroatom codoped, and carbon nitride (C(3)N(4)) based hybrid materials. Implications of various strategies, using one-step pyrolysis technique have been discussed for the effective design of heteroatom modified carbonaceous electrocatalysts. In this minireview, we outline the richness of one-step strategy for designing electrochemically active heteroatom doped carbon, transition metal–heteroatom codoped carbon, and C(3)N(4) derived hybrid materials in the perspective of electrochemical energy conversion and storage devices. We also outline the future research direction in the development of highly efficient and sustainable electrocatalysts for oxygen electrochemistry. Finally, we wind up the article with the challenges and outlook on heteroatoms and transition metal–heteroatom codoped carbon material as an efficient and low-cost electrocatalysts, thereby promoting the development of this important area. American Chemical Society 2020-12-14 /pmc/articles/PMC7774072/ /pubmed/33403245 http://dx.doi.org/10.1021/acsomega.0c04432 Text en © 2020 American Chemical Society This is an open access article published under a Creative Commons Non-Commercial No Derivative Works (CC-BY-NC-ND) Attribution License (http://pubs.acs.org/page/policy/authorchoice_ccbyncnd_termsofuse.html) , which permits copying and redistribution of the article, and creation of adaptations, all for non-commercial purposes. |
spellingShingle | Bisen, Omeshwari Yadorao Nandan, Ravi Nanda, Karuna Kar Unique One-Step Strategy for Nonmetallic and Metallic Heteroatom Doped Carbonaceous Materials |
title | Unique One-Step Strategy for Nonmetallic and Metallic
Heteroatom Doped Carbonaceous Materials |
title_full | Unique One-Step Strategy for Nonmetallic and Metallic
Heteroatom Doped Carbonaceous Materials |
title_fullStr | Unique One-Step Strategy for Nonmetallic and Metallic
Heteroatom Doped Carbonaceous Materials |
title_full_unstemmed | Unique One-Step Strategy for Nonmetallic and Metallic
Heteroatom Doped Carbonaceous Materials |
title_short | Unique One-Step Strategy for Nonmetallic and Metallic
Heteroatom Doped Carbonaceous Materials |
title_sort | unique one-step strategy for nonmetallic and metallic
heteroatom doped carbonaceous materials |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7774072/ https://www.ncbi.nlm.nih.gov/pubmed/33403245 http://dx.doi.org/10.1021/acsomega.0c04432 |
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