Cargando…
A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue
Carbon aerogels (CA) derived from bamboo cellulose fibers were coupled with TiO(2) to form CA/TiO(2) hybrids, which exhibited extraordinary performance on the photo-catalytic degradation of methylene blue (MB). The structure and morphology of CA/TiO(2) were characterized by field emission scanning e...
Autores principales: | , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2021
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7831082/ https://www.ncbi.nlm.nih.gov/pubmed/33477531 http://dx.doi.org/10.3390/nano11010239 |
_version_ | 1783641561215533056 |
---|---|
author | Zhang, Jian Yuan, Wei Xia, Tian Ao, Chenghong Zhao, Jiangqi Huang, Bingxue Wang, Qunhao Zhang, Wei Lu, Canhui |
author_facet | Zhang, Jian Yuan, Wei Xia, Tian Ao, Chenghong Zhao, Jiangqi Huang, Bingxue Wang, Qunhao Zhang, Wei Lu, Canhui |
author_sort | Zhang, Jian |
collection | PubMed |
description | Carbon aerogels (CA) derived from bamboo cellulose fibers were coupled with TiO(2) to form CA/TiO(2) hybrids, which exhibited extraordinary performance on the photo-catalytic degradation of methylene blue (MB). The structure and morphology of CA/TiO(2) were characterized by field emission scanning electron microscopy, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and Raman spectrum. The CA displayed a highly porous and interconnected three-dimensional framework structure, while introducing the catalytic active sites of TiO(2) onto the aerogel scaffold could remarkably enhance its photo-catalytic activity. The adsorption and photo-catalytic degradation of MB by the CA/TiO(2) hybrid were investigated. The maximum adsorption capacity of CA/TiO(2) for MB was 18.5 mg/g, which outperformed many similar materials reported in the literature. In addition, compared with other photo-catalysts, the present CA/TiO(2) demonstrated superior photo-catalytic performance. Almost 85% of MB in 50 mL solution with a MB concentration of 10 mg/L could be effectively degraded by 15 mg CA/TiO(2) in 300 min. |
format | Online Article Text |
id | pubmed-7831082 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-78310822021-01-26 A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue Zhang, Jian Yuan, Wei Xia, Tian Ao, Chenghong Zhao, Jiangqi Huang, Bingxue Wang, Qunhao Zhang, Wei Lu, Canhui Nanomaterials (Basel) Article Carbon aerogels (CA) derived from bamboo cellulose fibers were coupled with TiO(2) to form CA/TiO(2) hybrids, which exhibited extraordinary performance on the photo-catalytic degradation of methylene blue (MB). The structure and morphology of CA/TiO(2) were characterized by field emission scanning electron microscopy, Fourier transform infrared spectroscopy, X-ray photoelectron spectroscopy, X-ray diffraction, and Raman spectrum. The CA displayed a highly porous and interconnected three-dimensional framework structure, while introducing the catalytic active sites of TiO(2) onto the aerogel scaffold could remarkably enhance its photo-catalytic activity. The adsorption and photo-catalytic degradation of MB by the CA/TiO(2) hybrid were investigated. The maximum adsorption capacity of CA/TiO(2) for MB was 18.5 mg/g, which outperformed many similar materials reported in the literature. In addition, compared with other photo-catalysts, the present CA/TiO(2) demonstrated superior photo-catalytic performance. Almost 85% of MB in 50 mL solution with a MB concentration of 10 mg/L could be effectively degraded by 15 mg CA/TiO(2) in 300 min. MDPI 2021-01-18 /pmc/articles/PMC7831082/ /pubmed/33477531 http://dx.doi.org/10.3390/nano11010239 Text en © 2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Zhang, Jian Yuan, Wei Xia, Tian Ao, Chenghong Zhao, Jiangqi Huang, Bingxue Wang, Qunhao Zhang, Wei Lu, Canhui A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title | A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title_full | A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title_fullStr | A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title_full_unstemmed | A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title_short | A TiO(2) Coated Carbon Aerogel Derived from Bamboo Pulp Fibers for Enhanced Visible Light Photo-Catalytic Degradation of Methylene Blue |
title_sort | tio(2) coated carbon aerogel derived from bamboo pulp fibers for enhanced visible light photo-catalytic degradation of methylene blue |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7831082/ https://www.ncbi.nlm.nih.gov/pubmed/33477531 http://dx.doi.org/10.3390/nano11010239 |
work_keys_str_mv | AT zhangjian atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT yuanwei atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT xiatian atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT aochenghong atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT zhaojiangqi atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT huangbingxue atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT wangqunhao atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT zhangwei atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT lucanhui atio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT zhangjian tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT yuanwei tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT xiatian tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT aochenghong tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT zhaojiangqi tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT huangbingxue tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT wangqunhao tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT zhangwei tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue AT lucanhui tio2coatedcarbonaerogelderivedfrombamboopulpfibersforenhancedvisiblelightphotocatalyticdegradationofmethyleneblue |