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TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants

With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in...

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Autores principales: Jiang, Liushan, Zeng, Fanshan, Zhong, Rong, Xie, Yu, Wang, Jianli, Ye, Hao, Ling, Yun, Guo, Ruobin, Zhao, Jinsheng, Li, Shiqian, Hu, Yuying
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7835803/
https://www.ncbi.nlm.nih.gov/pubmed/33478044
http://dx.doi.org/10.3390/nano11010254
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author Jiang, Liushan
Zeng, Fanshan
Zhong, Rong
Xie, Yu
Wang, Jianli
Ye, Hao
Ling, Yun
Guo, Ruobin
Zhao, Jinsheng
Li, Shiqian
Hu, Yuying
author_facet Jiang, Liushan
Zeng, Fanshan
Zhong, Rong
Xie, Yu
Wang, Jianli
Ye, Hao
Ling, Yun
Guo, Ruobin
Zhao, Jinsheng
Li, Shiqian
Hu, Yuying
author_sort Jiang, Liushan
collection PubMed
description With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO(2) nanowires with a large specific surface area could provide enough space for loading more g-C(3)N(4) nanoparticles to obtain C(3)N(4)/TiO(2) composites. Of note, the g-C(3)N(4)/TiO(2) composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO(2) and g-C(3)N(4) could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C(3)N(4)/TiO(2) composite was also clarified in detail.
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spelling pubmed-78358032021-01-27 TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants Jiang, Liushan Zeng, Fanshan Zhong, Rong Xie, Yu Wang, Jianli Ye, Hao Ling, Yun Guo, Ruobin Zhao, Jinsheng Li, Shiqian Hu, Yuying Nanomaterials (Basel) Article With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO(2) nanowires with a large specific surface area could provide enough space for loading more g-C(3)N(4) nanoparticles to obtain C(3)N(4)/TiO(2) composites. Of note, the g-C(3)N(4)/TiO(2) composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO(2) and g-C(3)N(4) could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C(3)N(4)/TiO(2) composite was also clarified in detail. MDPI 2021-01-19 /pmc/articles/PMC7835803/ /pubmed/33478044 http://dx.doi.org/10.3390/nano11010254 Text en © 2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Jiang, Liushan
Zeng, Fanshan
Zhong, Rong
Xie, Yu
Wang, Jianli
Ye, Hao
Ling, Yun
Guo, Ruobin
Zhao, Jinsheng
Li, Shiqian
Hu, Yuying
TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title_full TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title_fullStr TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title_full_unstemmed TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title_short TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
title_sort tio(2) nanowires with doped g-c(3)n(4) nanoparticles for enhanced h(2) production and photodegradation of pollutants
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7835803/
https://www.ncbi.nlm.nih.gov/pubmed/33478044
http://dx.doi.org/10.3390/nano11010254
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