Cargando…
TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants
With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in...
Autores principales: | , , , , , , , , , , |
---|---|
Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
MDPI
2021
|
Materias: | |
Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7835803/ https://www.ncbi.nlm.nih.gov/pubmed/33478044 http://dx.doi.org/10.3390/nano11010254 |
_version_ | 1783642611394805760 |
---|---|
author | Jiang, Liushan Zeng, Fanshan Zhong, Rong Xie, Yu Wang, Jianli Ye, Hao Ling, Yun Guo, Ruobin Zhao, Jinsheng Li, Shiqian Hu, Yuying |
author_facet | Jiang, Liushan Zeng, Fanshan Zhong, Rong Xie, Yu Wang, Jianli Ye, Hao Ling, Yun Guo, Ruobin Zhao, Jinsheng Li, Shiqian Hu, Yuying |
author_sort | Jiang, Liushan |
collection | PubMed |
description | With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO(2) nanowires with a large specific surface area could provide enough space for loading more g-C(3)N(4) nanoparticles to obtain C(3)N(4)/TiO(2) composites. Of note, the g-C(3)N(4)/TiO(2) composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO(2) and g-C(3)N(4) could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C(3)N(4)/TiO(2) composite was also clarified in detail. |
format | Online Article Text |
id | pubmed-7835803 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | MDPI |
record_format | MEDLINE/PubMed |
spelling | pubmed-78358032021-01-27 TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants Jiang, Liushan Zeng, Fanshan Zhong, Rong Xie, Yu Wang, Jianli Ye, Hao Ling, Yun Guo, Ruobin Zhao, Jinsheng Li, Shiqian Hu, Yuying Nanomaterials (Basel) Article With the rapid consumption of fossil fuels, along with the ever-increasing environmental pollution, it is becoming a top priority to explore efficient photocatalysts for the production of renewable hydrogen and degradation of pollutants. Here, we fabricated a composite of g-C(3)N(4)/TiO(2) via an in situ growth method under the conditions of high-temperature calcination. In this method, TiO(2) nanowires with a large specific surface area could provide enough space for loading more g-C(3)N(4) nanoparticles to obtain C(3)N(4)/TiO(2) composites. Of note, the g-C(3)N(4)/TiO(2) composite could effectively photocatalyze both the degradation of several pollutants and production of hydrogen, both of which are essential for environmental governance. Combining multiple characterizations and experiments, we found that the heterojunction constructed by the TiO(2) and g-C(3)N(4) could increase the photocatalytic ability of materials by prompting the separation of photogenerated carriers. Furthermore, the photocatalytic mechanism of the g-C(3)N(4)/TiO(2) composite was also clarified in detail. MDPI 2021-01-19 /pmc/articles/PMC7835803/ /pubmed/33478044 http://dx.doi.org/10.3390/nano11010254 Text en © 2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/). |
spellingShingle | Article Jiang, Liushan Zeng, Fanshan Zhong, Rong Xie, Yu Wang, Jianli Ye, Hao Ling, Yun Guo, Ruobin Zhao, Jinsheng Li, Shiqian Hu, Yuying TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title | TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title_full | TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title_fullStr | TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title_full_unstemmed | TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title_short | TiO(2) Nanowires with Doped g-C(3)N(4) Nanoparticles for Enhanced H(2) Production and Photodegradation of Pollutants |
title_sort | tio(2) nanowires with doped g-c(3)n(4) nanoparticles for enhanced h(2) production and photodegradation of pollutants |
topic | Article |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7835803/ https://www.ncbi.nlm.nih.gov/pubmed/33478044 http://dx.doi.org/10.3390/nano11010254 |
work_keys_str_mv | AT jiangliushan tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT zengfanshan tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT zhongrong tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT xieyu tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT wangjianli tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT yehao tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT lingyun tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT guoruobin tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT zhaojinsheng tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT lishiqian tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants AT huyuying tio2nanowireswithdopedgc3n4nanoparticlesforenhancedh2productionandphotodegradationofpollutants |