Cargando…

Water enables mild oxidation of methane to methanol on gold single-atom catalysts

As a 100% atom-economy process, direct oxidation of methane into methanol remains as a grand challenge due to the dilemma between activation of methane and over-oxidation of methanol. Here, we report that water enabled mild oxidation of methane into methanol with >99% selectivity over Au single a...

Descripción completa

Detalles Bibliográficos
Autores principales:	Luo, Laihao, Luo, Jie, Li, Hongliang, Ren, Fangning, Zhang, Yifei, Liu, Andong, Li, Wei-Xue, Zeng, Jie
Formato:	Online Artículo Texto
Lenguaje:	English
Publicado:	Nature Publishing Group UK 2021
Materias:	Article
Acceso en línea:	https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7900127/ https://www.ncbi.nlm.nih.gov/pubmed/33619263 http://dx.doi.org/10.1038/s41467-021-21482-z

Ejemplares similares

Static Regulation and Dynamic Evolution of Single‐Atom Catalysts in Thermal Catalytic Reactions
por: Li, Hongliang, et al.
Publicado: (2018)

Single‐Atom Catalysis: Static Regulation and Dynamic Evolution of Single‐Atom Catalysts in Thermal Catalytic Reactions (Adv. Sci. 3/2019)
por: Li, Hongliang, et al.
Publicado: (2019)

Manipulating local coordination of copper single atom catalyst enables efficient CO(2)-to-CH(4) conversion
por: Dai, Yizhou, et al.
Publicado: (2023)

Single-atom catalyst for high-performance methanol oxidation
por: Zhang, Zhiqi, et al.
Publicado: (2021)

Atomic cerium modulated palladium nanoclusters exsolved ferrite catalysts for lean methane conversion
por: Yang, Yanling, et al.
Publicado: (2022)

Methane Oxidation to Methanol
por: Dummer, Nicholas F., et al.
Publicado: (2022)

Atomic-level insights in optimizing reaction paths for hydroformylation reaction over Rh/CoO single-atom catalyst
por: Wang, Liangbing, et al.
Publicado: (2016)

Electrochemical Reoxidation Enables Continuous Methane-to-Methanol Catalysis with Aqueous Pt Salts
por: Kim, R. Soyoung, et al.
Publicado: (2019)

One-step direct conversion of methane to methanol with water in non-thermal plasma
por: Bi, Wenfei, et al.
Publicado: (2022)

Cu and Zn Bimetallic Co-Modified H-MOR Catalyst for Direct Oxidation of Low-Concentration Methane to Methanol
por: Fu, Yan, et al.
Publicado: (2023)

Silver and Copper Dual Single Atoms Boosting Direct Oxidation of Methane to Methanol via Synergistic Catalysis
por: Yu, Baiyang, et al.
Publicado: (2023)

Direct Catalytic Oxidation of Low-Concentration Methane to Methanol in One Step on Ni-Promoted BiOCl Catalysts
por: Zhu, Chen, et al.
Publicado: (2023)

Electrochemical deposition as a universal route for fabricating single-atom catalysts
por: Zhang, Zhirong, et al.
Publicado: (2020)

Volcano-type relationship between oxidation states and catalytic activity of single-atom catalysts towards hydrogen evolution
por: Cao, Dong, et al.
Publicado: (2022)

New Strategies for Direct Methane-to-Methanol Conversion from Active Learning Exploration of 16 Million Catalysts
por: Nandy, Aditya, et al.
Publicado: (2022)

Sub-nanometer Copper Clusters as Alternative Catalysts for the Selective Oxidation of Methane to Methanol with Molecular O(2)
por: Gallego, Mario, et al.
Publicado: (2022)

Insights on forming N,O-coordinated Cu single-atom catalysts for electrochemical reduction CO(2) to methane
por: Cai, Yanming, et al.
Publicado: (2021)

Secondary-Atom-Doping Enables Robust Fe–N–C Single-Atom Catalysts with Enhanced Oxygen Reduction Reaction
por: Luo, Xin, et al.
Publicado: (2020)

Coalbed methane diffusion and water blocking effects investigated by mesoscale all-atom molecular dynamic simulations
por: Zhu, Qingzhong, et al.
Publicado: (2020)

Tuning methane decomposition on stepped Ni surface: The role of subsurface atoms in catalyst design
por: Arevalo, Ryan Lacdao, et al.
Publicado: (2017)

Single rhodium atoms anchored in micropores for efficient transformation of methane under mild conditions
por: Tang, Yu, et al.
Publicado: (2018)

Photothermal-enabled single-atom catalysts for high-efficiency hydrogen peroxide photosynthesis from natural seawater
por: Wang, Wei, et al.
Publicado: (2023)

Coordination modulation of iridium single-atom catalyst maximizing water oxidation activity
por: Lei, Zhanwu, et al.
Publicado: (2022)

Structural Evolution of Iron-Loaded Metal–Organic Framework Catalysts for Continuous Gas-Phase Oxidation of Methane to Methanol
por: Rungtaweevoranit, Bunyarat, et al.
Publicado: (2023)

Gold catalysts containing interstitial carbon atoms boost hydrogenation activity
por: Sun, Yafei, et al.
Publicado: (2020)

Recent Advances in Photocatalytic Oxidation of Methane to Methanol
por: Yuniar, Gita, et al.
Publicado: (2022)

Shifting the scaling relations of single-atom catalysts for facile methane activation by tuning the coordination number
por: Choi, Changhyeok, et al.
Publicado: (2021)

Mechanistic and microkinetic study of non-oxidative methane coupling on a single-atom iron catalyst
por: Kim, Seok Ki, et al.
Publicado: (2020)

The effect of oxidant species on direct, non-syngas conversion of methane to methanol over an FePO(4) catalyst material
por: Dasireddy, Venkata D. B. C., et al.
Publicado: (2019)

Recent Advances in the Catalytic Conversion of Methane to Methanol: From the Challenges of Traditional Catalysts to the Use of Nanomaterials and Metal-Organic Frameworks
por: Vali, Seyed Alireza, et al.
Publicado: (2023)

Selective light absorber-assisted single nickel atom catalysts for ambient sunlight-driven CO(2) methanation
por: Li, Yaguang, et al.
Publicado: (2019)

Site-specific electrodeposition enables self-terminating growth of atomically dispersed metal catalysts
por: Shi, Yi, et al.
Publicado: (2020)

Atomic Cu Sites Engineering Enables Efficient CO(2) Electroreduction to Methane with High CH(4)/C(2)H(4) Ratio
por: Li, Minhan, et al.
Publicado: (2023)

In aqua dual selective photocatalytic conversion of methane to formic acid and methanol with oxygen and water as oxidants without overoxidation
por: Han, Jing-Tan, et al.
Publicado: (2023)

Reutilizing Methane Reforming Spent Catalysts as Efficient Overall Water-Splitting Electrocatalysts
por: Khan, Muhammad Awais, et al.
Publicado: (2021)

Preparation of Ni based mesoporous Al(2)O(3) catalyst with enhanced CO(2) methanation performance
por: Lin, Jianghui, et al.
Publicado: (2019)

Printable enzyme-embedded materials for methane to methanol conversion
por: Blanchette, Craig D., et al.
Publicado: (2016)

High-efficiency direct methane conversion to oxygenates on a cerium dioxide nanowires supported rhodium single-atom catalyst
por: Bai, Shuxing, et al.
Publicado: (2020)

Quasi Pd(1)Ni single-atom surface alloy catalyst enables hydrogenation of nitriles to secondary amines
por: Wang, Hengwei, et al.
Publicado: (2019)

Harnessing of Diluted Methane Emissions by Direct Partial Oxidation of Methane to Methanol over Cu/Mordenite
por: Álvarez, Mauro, et al.
Publicado: (2021)

Cannot write session to /tmp/vufind_sessions/sess_sjjkf3bo7r9o93o4etem0s3a7j