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On Compton scattering as a source of background in coherent diffraction imaging experiments

Compton scattering is generally neglected in diffraction experiments because the incoherent radiation it generates does not give rise to interference effects and therefore is negligible at Bragg peaks. However, as the scattering volume is reduced, the difference between the Rayleigh (coherent) and C...

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Detalles Bibliográficos
Autores principales: Bikondoa, Oier, Carbone, Dina
Formato: Online Artículo Texto
Lenguaje:English
Publicado: International Union of Crystallography 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7941292/
https://www.ncbi.nlm.nih.gov/pubmed/33650567
http://dx.doi.org/10.1107/S1600577521000722
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author Bikondoa, Oier
Carbone, Dina
author_facet Bikondoa, Oier
Carbone, Dina
author_sort Bikondoa, Oier
collection PubMed
description Compton scattering is generally neglected in diffraction experiments because the incoherent radiation it generates does not give rise to interference effects and therefore is negligible at Bragg peaks. However, as the scattering volume is reduced, the difference between the Rayleigh (coherent) and Compton (incoherent) contributions at Bragg peaks diminishes and the incoherent part may become substantial. The consequences can be significant for coherent diffraction imaging at high scattering angles: the incoherent radiation produces background that smears out the secondary interference fringes, affecting thus the achievable resolution of the technique. Here, a criterion that relates the object shape and the resolution is introduced. The Compton contribution for several object shapes is quantified, and it is shown that the maximum achievable resolution along different directions has a strong dependence on the crystal shape and size.
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spelling pubmed-79412922021-04-07 On Compton scattering as a source of background in coherent diffraction imaging experiments Bikondoa, Oier Carbone, Dina J Synchrotron Radiat Research Papers Compton scattering is generally neglected in diffraction experiments because the incoherent radiation it generates does not give rise to interference effects and therefore is negligible at Bragg peaks. However, as the scattering volume is reduced, the difference between the Rayleigh (coherent) and Compton (incoherent) contributions at Bragg peaks diminishes and the incoherent part may become substantial. The consequences can be significant for coherent diffraction imaging at high scattering angles: the incoherent radiation produces background that smears out the secondary interference fringes, affecting thus the achievable resolution of the technique. Here, a criterion that relates the object shape and the resolution is introduced. The Compton contribution for several object shapes is quantified, and it is shown that the maximum achievable resolution along different directions has a strong dependence on the crystal shape and size. International Union of Crystallography 2021-02-18 /pmc/articles/PMC7941292/ /pubmed/33650567 http://dx.doi.org/10.1107/S1600577521000722 Text en © Bikondoa and Carbone 2021 http://creativecommons.org/licenses/by/4.0/ This is an open-access article distributed under the terms of the Creative Commons Attribution (CC-BY) Licence, which permits unrestricted use, distribution, and reproduction in any medium, provided the original authors and source are cited.http://creativecommons.org/licenses/by/4.0/
spellingShingle Research Papers
Bikondoa, Oier
Carbone, Dina
On Compton scattering as a source of background in coherent diffraction imaging experiments
title On Compton scattering as a source of background in coherent diffraction imaging experiments
title_full On Compton scattering as a source of background in coherent diffraction imaging experiments
title_fullStr On Compton scattering as a source of background in coherent diffraction imaging experiments
title_full_unstemmed On Compton scattering as a source of background in coherent diffraction imaging experiments
title_short On Compton scattering as a source of background in coherent diffraction imaging experiments
title_sort on compton scattering as a source of background in coherent diffraction imaging experiments
topic Research Papers
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7941292/
https://www.ncbi.nlm.nih.gov/pubmed/33650567
http://dx.doi.org/10.1107/S1600577521000722
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