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Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite

Developing sustainable routes for the synthesis of zeolites is still a vital and challenging task in zeolite scientific community. One of the typical examples is sustainable synthesis of aluminosilicate EU-1 zeolite, which is not very efficient and environmental-unfriendly under hydrothermal conditi...

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Autores principales: Xu, Hao, Zhu, Jie, Wang, Xiong, Shen, Chao, Meng, Shengshen, Zheng, Kai, Lei, Chao, Zhu, Longfeng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7962662/
https://www.ncbi.nlm.nih.gov/pubmed/33800313
http://dx.doi.org/10.3390/molecules26051462
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author Xu, Hao
Zhu, Jie
Wang, Xiong
Shen, Chao
Meng, Shengshen
Zheng, Kai
Lei, Chao
Zhu, Longfeng
author_facet Xu, Hao
Zhu, Jie
Wang, Xiong
Shen, Chao
Meng, Shengshen
Zheng, Kai
Lei, Chao
Zhu, Longfeng
author_sort Xu, Hao
collection PubMed
description Developing sustainable routes for the synthesis of zeolites is still a vital and challenging task in zeolite scientific community. One of the typical examples is sustainable synthesis of aluminosilicate EU-1 zeolite, which is not very efficient and environmental-unfriendly under hydrothermal condition due to the use of a large amount of water as solvent. Herein, we report a sustainable synthesis route for aluminosilicate EU-1 zeolite without the use of solvent for the first time. The physicochemical properties of the obtained EU-1 zeolite are characterized by powder X-ray diffraction (XRD), scanning electron microscopy (SEM), thermogravimetry-differential thermal analysis (TG-DTA), N(2) sorption, inductively coupled plasma (ICP) analysis, and solid nuclear magnetic resonance (NMR), which show the product has high crystallinity, uniform morphology, large BET surface area, and four-coordinated aluminum species. Moreover, the impact of synthesis conditions is investigated in detail. The sustainable synthesis of aluminosilicate EU-1 zeolite under solvent-free
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spelling pubmed-79626622021-03-17 Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite Xu, Hao Zhu, Jie Wang, Xiong Shen, Chao Meng, Shengshen Zheng, Kai Lei, Chao Zhu, Longfeng Molecules Article Developing sustainable routes for the synthesis of zeolites is still a vital and challenging task in zeolite scientific community. One of the typical examples is sustainable synthesis of aluminosilicate EU-1 zeolite, which is not very efficient and environmental-unfriendly under hydrothermal condition due to the use of a large amount of water as solvent. Herein, we report a sustainable synthesis route for aluminosilicate EU-1 zeolite without the use of solvent for the first time. The physicochemical properties of the obtained EU-1 zeolite are characterized by powder X-ray diffraction (XRD), scanning electron microscopy (SEM), thermogravimetry-differential thermal analysis (TG-DTA), N(2) sorption, inductively coupled plasma (ICP) analysis, and solid nuclear magnetic resonance (NMR), which show the product has high crystallinity, uniform morphology, large BET surface area, and four-coordinated aluminum species. Moreover, the impact of synthesis conditions is investigated in detail. The sustainable synthesis of aluminosilicate EU-1 zeolite under solvent-free MDPI 2021-03-08 /pmc/articles/PMC7962662/ /pubmed/33800313 http://dx.doi.org/10.3390/molecules26051462 Text en © 2021 by the authors. Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (http://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Xu, Hao
Zhu, Jie
Wang, Xiong
Shen, Chao
Meng, Shengshen
Zheng, Kai
Lei, Chao
Zhu, Longfeng
Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title_full Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title_fullStr Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title_full_unstemmed Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title_short Sustainable Route for Synthesizing Aluminosilicate EU-1 Zeolite
title_sort sustainable route for synthesizing aluminosilicate eu-1 zeolite
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7962662/
https://www.ncbi.nlm.nih.gov/pubmed/33800313
http://dx.doi.org/10.3390/molecules26051462
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