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Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet

The transverse voltage generated by a temperature gradient in a perpendicularly applied magnetic field, termed the Nernst effect, has promise for thermoelectric applications and for probing electronic structure. In magnetic materials, an anomalous Nernst effect (ANE) is possible in a zero magnetic f...

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Autores principales: Asaba, T., Ivanov, V., Thomas, S. M., Savrasov, S. Y., Thompson, J. D., Bauer, E. D., Ronning, F.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7997519/
https://www.ncbi.nlm.nih.gov/pubmed/33771869
http://dx.doi.org/10.1126/sciadv.abf1467
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author Asaba, T.
Ivanov, V.
Thomas, S. M.
Savrasov, S. Y.
Thompson, J. D.
Bauer, E. D.
Ronning, F.
author_facet Asaba, T.
Ivanov, V.
Thomas, S. M.
Savrasov, S. Y.
Thompson, J. D.
Bauer, E. D.
Ronning, F.
author_sort Asaba, T.
collection PubMed
description The transverse voltage generated by a temperature gradient in a perpendicularly applied magnetic field, termed the Nernst effect, has promise for thermoelectric applications and for probing electronic structure. In magnetic materials, an anomalous Nernst effect (ANE) is possible in a zero magnetic field. We report a colossal ANE in the ferromagnetic metal UCo(0.8)Ru(0.2)Al, reaching 23 microvolts per kelvin. Uranium’s 5f electrons provide strong electronic correlations that lead to narrow bands, a known route to producing a large thermoelectric response. In addition, uranium’s strong spin-orbit coupling produces an intrinsic transverse response in this material due to the Berry curvature associated with the relativistic electronic structure. Theoretical calculations show that in UCo(0.8)Ru(0.2)Al at least 148 Weyl nodes, and two nodal lines, exist within 60 millielectron volt of the Fermi level. This work demonstrates that magnetic actinide materials can host strong Nernst and Hall responses due to their combined correlated and topological nature.
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spelling pubmed-79975192021-04-02 Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet Asaba, T. Ivanov, V. Thomas, S. M. Savrasov, S. Y. Thompson, J. D. Bauer, E. D. Ronning, F. Sci Adv Research Articles The transverse voltage generated by a temperature gradient in a perpendicularly applied magnetic field, termed the Nernst effect, has promise for thermoelectric applications and for probing electronic structure. In magnetic materials, an anomalous Nernst effect (ANE) is possible in a zero magnetic field. We report a colossal ANE in the ferromagnetic metal UCo(0.8)Ru(0.2)Al, reaching 23 microvolts per kelvin. Uranium’s 5f electrons provide strong electronic correlations that lead to narrow bands, a known route to producing a large thermoelectric response. In addition, uranium’s strong spin-orbit coupling produces an intrinsic transverse response in this material due to the Berry curvature associated with the relativistic electronic structure. Theoretical calculations show that in UCo(0.8)Ru(0.2)Al at least 148 Weyl nodes, and two nodal lines, exist within 60 millielectron volt of the Fermi level. This work demonstrates that magnetic actinide materials can host strong Nernst and Hall responses due to their combined correlated and topological nature. American Association for the Advancement of Science 2021-03-26 /pmc/articles/PMC7997519/ /pubmed/33771869 http://dx.doi.org/10.1126/sciadv.abf1467 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/ https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Asaba, T.
Ivanov, V.
Thomas, S. M.
Savrasov, S. Y.
Thompson, J. D.
Bauer, E. D.
Ronning, F.
Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title_full Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title_fullStr Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title_full_unstemmed Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title_short Colossal anomalous Nernst effect in a correlated noncentrosymmetric kagome ferromagnet
title_sort colossal anomalous nernst effect in a correlated noncentrosymmetric kagome ferromagnet
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC7997519/
https://www.ncbi.nlm.nih.gov/pubmed/33771869
http://dx.doi.org/10.1126/sciadv.abf1467
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