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Electric-Field-Effect Spin Switching with an Enhanced Number of Highly Polarized Electron and Photon Spins Using p-Doped Semiconductor Quantum Dots
[Image: see text] Electric-field-effect spin switching with an enhanced number of highly polarized electron and photon spins has been demonstrated using p-doped semiconductor quantum dots (QDs). Remote p-doping in InGaAs QDs tunnel-coupled with an InGaAs quantum well (QW) significantly increased the...
Autores principales: | , , , , , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8015086/ https://www.ncbi.nlm.nih.gov/pubmed/33817516 http://dx.doi.org/10.1021/acsomega.1c00377 |
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author | Park, Soyoung Chen, Hang Hiura, Satoshi Takayama, Junichi Sueoka, Kazuhisa Murayama, Akihiro |
author_facet | Park, Soyoung Chen, Hang Hiura, Satoshi Takayama, Junichi Sueoka, Kazuhisa Murayama, Akihiro |
author_sort | Park, Soyoung |
collection | PubMed |
description | [Image: see text] Electric-field-effect spin switching with an enhanced number of highly polarized electron and photon spins has been demonstrated using p-doped semiconductor quantum dots (QDs). Remote p-doping in InGaAs QDs tunnel-coupled with an InGaAs quantum well (QW) significantly increased the circularly polarized, thus electron-spin-polarized, photoluminescence intensity, depending on the electric-field-induced electron spin injection from the QW as a spin reservoir into the QDs. The spin polarity and polarization degree during this spin injection can be controlled by the direction and the strength of the electric field, where the spin direction can be reversed by excess electron spin injection into the QDs via spin scattering at the QD excited states. We found that the maximum degrees of both parallel and antiparallel spin polarization to the initial spin direction in the QW can be enhanced by p-doping. The doped holes without spin polarization can effectively contribute to this electric-field-effect spin switching after the initial electron spin injection selectively removes the parallel hole spins. The optimized p-doping induces fast spin reversals at the QD excited states with a moderate electric-field application, resulting in an efficient electric-field-driven antiparallel spin injection into the QD ground state. Further excess hole doping prevents this efficient spin reversal due to multiple electron–hole spin scattering, in addition to a spin-state filling effect at the QD excited states, during the spin injection from the QW into the QDs. |
format | Online Article Text |
id | pubmed-8015086 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-80150862021-04-02 Electric-Field-Effect Spin Switching with an Enhanced Number of Highly Polarized Electron and Photon Spins Using p-Doped Semiconductor Quantum Dots Park, Soyoung Chen, Hang Hiura, Satoshi Takayama, Junichi Sueoka, Kazuhisa Murayama, Akihiro ACS Omega [Image: see text] Electric-field-effect spin switching with an enhanced number of highly polarized electron and photon spins has been demonstrated using p-doped semiconductor quantum dots (QDs). Remote p-doping in InGaAs QDs tunnel-coupled with an InGaAs quantum well (QW) significantly increased the circularly polarized, thus electron-spin-polarized, photoluminescence intensity, depending on the electric-field-induced electron spin injection from the QW as a spin reservoir into the QDs. The spin polarity and polarization degree during this spin injection can be controlled by the direction and the strength of the electric field, where the spin direction can be reversed by excess electron spin injection into the QDs via spin scattering at the QD excited states. We found that the maximum degrees of both parallel and antiparallel spin polarization to the initial spin direction in the QW can be enhanced by p-doping. The doped holes without spin polarization can effectively contribute to this electric-field-effect spin switching after the initial electron spin injection selectively removes the parallel hole spins. The optimized p-doping induces fast spin reversals at the QD excited states with a moderate electric-field application, resulting in an efficient electric-field-driven antiparallel spin injection into the QD ground state. Further excess hole doping prevents this efficient spin reversal due to multiple electron–hole spin scattering, in addition to a spin-state filling effect at the QD excited states, during the spin injection from the QW into the QDs. American Chemical Society 2021-03-15 /pmc/articles/PMC8015086/ /pubmed/33817516 http://dx.doi.org/10.1021/acsomega.1c00377 Text en © 2021 The Authors. Published by American Chemical Society Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Park, Soyoung Chen, Hang Hiura, Satoshi Takayama, Junichi Sueoka, Kazuhisa Murayama, Akihiro Electric-Field-Effect Spin Switching with an Enhanced Number of Highly Polarized Electron and Photon Spins Using p-Doped Semiconductor Quantum Dots |
title | Electric-Field-Effect Spin Switching with an Enhanced
Number of Highly Polarized Electron and Photon Spins Using p-Doped
Semiconductor Quantum Dots |
title_full | Electric-Field-Effect Spin Switching with an Enhanced
Number of Highly Polarized Electron and Photon Spins Using p-Doped
Semiconductor Quantum Dots |
title_fullStr | Electric-Field-Effect Spin Switching with an Enhanced
Number of Highly Polarized Electron and Photon Spins Using p-Doped
Semiconductor Quantum Dots |
title_full_unstemmed | Electric-Field-Effect Spin Switching with an Enhanced
Number of Highly Polarized Electron and Photon Spins Using p-Doped
Semiconductor Quantum Dots |
title_short | Electric-Field-Effect Spin Switching with an Enhanced
Number of Highly Polarized Electron and Photon Spins Using p-Doped
Semiconductor Quantum Dots |
title_sort | electric-field-effect spin switching with an enhanced
number of highly polarized electron and photon spins using p-doped
semiconductor quantum dots |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8015086/ https://www.ncbi.nlm.nih.gov/pubmed/33817516 http://dx.doi.org/10.1021/acsomega.1c00377 |
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