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Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire

The roof and spire of Notre‐Dame cathedral in Paris that caught fire and collapsed on 15 April 2019 were covered with 460 t of lead (Pb). Government reports documented Pb deposition immediately downwind of the cathedral and a twentyfold increase in airborne Pb concentrations at a distance of 50 km i...

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Autores principales: van Geen, Alexander, Yao, Yuling, Ellis, Tyler, Gelman, Andrew
Formato: Online Artículo Texto
Lenguaje:English
Publicado: John Wiley and Sons Inc. 2020
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8027784/
https://www.ncbi.nlm.nih.gov/pubmed/33855247
http://dx.doi.org/10.1029/2020GH000279
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author van Geen, Alexander
Yao, Yuling
Ellis, Tyler
Gelman, Andrew
author_facet van Geen, Alexander
Yao, Yuling
Ellis, Tyler
Gelman, Andrew
author_sort van Geen, Alexander
collection PubMed
description The roof and spire of Notre‐Dame cathedral in Paris that caught fire and collapsed on 15 April 2019 were covered with 460 t of lead (Pb). Government reports documented Pb deposition immediately downwind of the cathedral and a twentyfold increase in airborne Pb concentrations at a distance of 50 km in the aftermath. For this study, we collected 100 samples of surface soil from tree pits, parks, and other sites in all directions within 1 km of the cathedral. Concentrations of Pb measured by X‐ray fluorescence range from 30 to 9,000 mg/kg across the area, with a higher proportion of elevated concentrations to the northwest of the cathedral, in the direction of the wind prevailing during the fire. By integrating these observations with a Gaussian process regression model, we estimate that the average concentration of Pb in surface soil downwind of the cathedral is 430 (95% interval, 300–590) mg/kg, nearly double the average Pb concentration in the other directions of 240 (95% interval, 170–320) mg/kg. The difference corresponds to an integrated excess Pb inventory within a 1 km radius of 1.0 (95% interval, 0.5–1.5) t, about 0.2% of all the Pb covering the roof and spire. This is over 6 times the estimated amount of Pb deposited downwind 1–50 km from the cathedral. To what extent the concentrated fallout within 1 km documented here temporarily exposed the downwind population to Pb is difficult to confirm independently because too few soil, dust, and blood samples were collected immediately after the fire.
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spelling pubmed-80277842021-04-13 Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire van Geen, Alexander Yao, Yuling Ellis, Tyler Gelman, Andrew Geohealth Research Articles The roof and spire of Notre‐Dame cathedral in Paris that caught fire and collapsed on 15 April 2019 were covered with 460 t of lead (Pb). Government reports documented Pb deposition immediately downwind of the cathedral and a twentyfold increase in airborne Pb concentrations at a distance of 50 km in the aftermath. For this study, we collected 100 samples of surface soil from tree pits, parks, and other sites in all directions within 1 km of the cathedral. Concentrations of Pb measured by X‐ray fluorescence range from 30 to 9,000 mg/kg across the area, with a higher proportion of elevated concentrations to the northwest of the cathedral, in the direction of the wind prevailing during the fire. By integrating these observations with a Gaussian process regression model, we estimate that the average concentration of Pb in surface soil downwind of the cathedral is 430 (95% interval, 300–590) mg/kg, nearly double the average Pb concentration in the other directions of 240 (95% interval, 170–320) mg/kg. The difference corresponds to an integrated excess Pb inventory within a 1 km radius of 1.0 (95% interval, 0.5–1.5) t, about 0.2% of all the Pb covering the roof and spire. This is over 6 times the estimated amount of Pb deposited downwind 1–50 km from the cathedral. To what extent the concentrated fallout within 1 km documented here temporarily exposed the downwind population to Pb is difficult to confirm independently because too few soil, dust, and blood samples were collected immediately after the fire. John Wiley and Sons Inc. 2020-08-21 /pmc/articles/PMC8027784/ /pubmed/33855247 http://dx.doi.org/10.1029/2020GH000279 Text en ©2020. The Authors. https://creativecommons.org/licenses/by/4.0/This is an open access article under the terms of the http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) License, which permits use, distribution and reproduction in any medium, provided the original work is properly cited.
spellingShingle Research Articles
van Geen, Alexander
Yao, Yuling
Ellis, Tyler
Gelman, Andrew
Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title_full Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title_fullStr Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title_full_unstemmed Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title_short Fallout of Lead Over Paris From the 2019 Notre‐Dame Cathedral Fire
title_sort fallout of lead over paris from the 2019 notre‐dame cathedral fire
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8027784/
https://www.ncbi.nlm.nih.gov/pubmed/33855247
http://dx.doi.org/10.1029/2020GH000279
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