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High Light Outcoupling Efficiency from Periodically Corrugated OLEDs
[Image: see text] Organic light-emitting diodes (OLEDs) suffer from poor light outcoupling efficiency (η(out) < 20%) due to large internal waveguiding in the high-index layers/substrate, and plasmonic losses at the metal cathode interface. A promising approach to enhance light outcoupling is to u...
Autores principales: | , |
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Formato: | Online Artículo Texto |
Lenguaje: | English |
Publicado: |
American Chemical Society
2021
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Acceso en línea: | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8028165/ https://www.ncbi.nlm.nih.gov/pubmed/33842798 http://dx.doi.org/10.1021/acsomega.1c00903 |
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author | Zhang, Yu Biswas, Rana |
author_facet | Zhang, Yu Biswas, Rana |
author_sort | Zhang, Yu |
collection | PubMed |
description | [Image: see text] Organic light-emitting diodes (OLEDs) suffer from poor light outcoupling efficiency (η(out) < 20%) due to large internal waveguiding in the high-index layers/substrate, and plasmonic losses at the metal cathode interface. A promising approach to enhance light outcoupling is to utilize internal periodic corrugations that can diffract waveguided and plasmonic modes back to the air cone. Although corrugations can strongly diffract trapped modes, the optimal geometry of corrugations and limits to η(out) are not well-established. We develop a general rigorous scattering matrix theory for light emission from corrugated OLEDs, by solving Maxwell’s equations in Fourier space, incorporating the environment-induced modification of the optical emission rate (Purcell effect). We computationally obtain the spectrally emissive power inside and outside the OLED. We find conformally corrugated OLEDs, where all OLED interfaces are conformal with a photonic crystal substrate, having triangular lattice symmetry, exhibit high light outcoupling η(out) ∼60–65%, and an enhancement factor exceeding 3 for optimal pitch values between 1 and 2.5 μm. Waveguided and surface plasmon modes are strongly diffracted to the air cone through first-order diffraction. η(out) is insensitive to corrugation heights larger than 100 nm. There is a gradual roll-off in η(out) for a larger pitch and sharper decreases for small pitch values. Plasmonic losses remain below 10% for all corrugation pitch values. Our predicted OLED designs provide a pathway for achieving very high light outcoupling over the full optical spectrum that can advance organic optoelectronic science and solid-state lighting. |
format | Online Article Text |
id | pubmed-8028165 |
institution | National Center for Biotechnology Information |
language | English |
publishDate | 2021 |
publisher | American Chemical Society |
record_format | MEDLINE/PubMed |
spelling | pubmed-80281652021-04-09 High Light Outcoupling Efficiency from Periodically Corrugated OLEDs Zhang, Yu Biswas, Rana ACS Omega [Image: see text] Organic light-emitting diodes (OLEDs) suffer from poor light outcoupling efficiency (η(out) < 20%) due to large internal waveguiding in the high-index layers/substrate, and plasmonic losses at the metal cathode interface. A promising approach to enhance light outcoupling is to utilize internal periodic corrugations that can diffract waveguided and plasmonic modes back to the air cone. Although corrugations can strongly diffract trapped modes, the optimal geometry of corrugations and limits to η(out) are not well-established. We develop a general rigorous scattering matrix theory for light emission from corrugated OLEDs, by solving Maxwell’s equations in Fourier space, incorporating the environment-induced modification of the optical emission rate (Purcell effect). We computationally obtain the spectrally emissive power inside and outside the OLED. We find conformally corrugated OLEDs, where all OLED interfaces are conformal with a photonic crystal substrate, having triangular lattice symmetry, exhibit high light outcoupling η(out) ∼60–65%, and an enhancement factor exceeding 3 for optimal pitch values between 1 and 2.5 μm. Waveguided and surface plasmon modes are strongly diffracted to the air cone through first-order diffraction. η(out) is insensitive to corrugation heights larger than 100 nm. There is a gradual roll-off in η(out) for a larger pitch and sharper decreases for small pitch values. Plasmonic losses remain below 10% for all corrugation pitch values. Our predicted OLED designs provide a pathway for achieving very high light outcoupling over the full optical spectrum that can advance organic optoelectronic science and solid-state lighting. American Chemical Society 2021-03-23 /pmc/articles/PMC8028165/ /pubmed/33842798 http://dx.doi.org/10.1021/acsomega.1c00903 Text en © 2021 The Authors. Published by American Chemical Society Permits non-commercial access and re-use, provided that author attribution and integrity are maintained; but does not permit creation of adaptations or other derivative works (https://creativecommons.org/licenses/by-nc-nd/4.0/). |
spellingShingle | Zhang, Yu Biswas, Rana High Light Outcoupling Efficiency from Periodically Corrugated OLEDs |
title | High Light Outcoupling Efficiency from Periodically
Corrugated OLEDs |
title_full | High Light Outcoupling Efficiency from Periodically
Corrugated OLEDs |
title_fullStr | High Light Outcoupling Efficiency from Periodically
Corrugated OLEDs |
title_full_unstemmed | High Light Outcoupling Efficiency from Periodically
Corrugated OLEDs |
title_short | High Light Outcoupling Efficiency from Periodically
Corrugated OLEDs |
title_sort | high light outcoupling efficiency from periodically
corrugated oleds |
url | https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8028165/ https://www.ncbi.nlm.nih.gov/pubmed/33842798 http://dx.doi.org/10.1021/acsomega.1c00903 |
work_keys_str_mv | AT zhangyu highlightoutcouplingefficiencyfromperiodicallycorrugatedoleds AT biswasrana highlightoutcouplingefficiencyfromperiodicallycorrugatedoleds |