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Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)

Novel effects induced by nonmagnetic impurities in frustrated magnets and quantum spin liquid represent a highly nontrivial and interesting problem. A theoretical proposal of extended modulated spin structures induced by doping of such magnets, distinct from the well-known skyrmions has attracted si...

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Autores principales: Park, Pyeongjae, Park, Kisoo, Oh, Joosung, Lee, Ki Hoon, Leiner, Jonathan C., Sim, Hasung, Kim, Taehun, Jeong, Jaehong, Rule, Kirrily C., Kamazawa, Kazuya, Iida, Kazuki, Perring, T. G., Woo, Hyungje, Cheong, S.-W., Zhitomirsky, M. E., Chernyshev, A. L., Park, Je-Geun
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8052335/
https://www.ncbi.nlm.nih.gov/pubmed/33863905
http://dx.doi.org/10.1038/s41467-021-22569-3
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author Park, Pyeongjae
Park, Kisoo
Oh, Joosung
Lee, Ki Hoon
Leiner, Jonathan C.
Sim, Hasung
Kim, Taehun
Jeong, Jaehong
Rule, Kirrily C.
Kamazawa, Kazuya
Iida, Kazuki
Perring, T. G.
Woo, Hyungje
Cheong, S.-W.
Zhitomirsky, M. E.
Chernyshev, A. L.
Park, Je-Geun
author_facet Park, Pyeongjae
Park, Kisoo
Oh, Joosung
Lee, Ki Hoon
Leiner, Jonathan C.
Sim, Hasung
Kim, Taehun
Jeong, Jaehong
Rule, Kirrily C.
Kamazawa, Kazuya
Iida, Kazuki
Perring, T. G.
Woo, Hyungje
Cheong, S.-W.
Zhitomirsky, M. E.
Chernyshev, A. L.
Park, Je-Geun
author_sort Park, Pyeongjae
collection PubMed
description Novel effects induced by nonmagnetic impurities in frustrated magnets and quantum spin liquid represent a highly nontrivial and interesting problem. A theoretical proposal of extended modulated spin structures induced by doping of such magnets, distinct from the well-known skyrmions has attracted significant interest. Here, we demonstrate that nonmagnetic impurities can produce such extended spin structures in h-YMnO(3), a triangular antiferromagnet with noncollinear magnetic order. Using inelastic neutron scattering (INS), we measured the full dynamical structure factor in Al-doped h-YMnO(3) and confirmed the presence of magnon damping with a clear momentum dependence. Our theoretical calculations can reproduce the key features of the INS data, supporting the formation of the proposed spin textures. As such, our study provides the first experimental confirmation of the impurity-induced spin textures. It offers new insights and understanding of the impurity effects in a broad class of noncollinear magnetic systems.
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spelling pubmed-80523352021-05-11 Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3) Park, Pyeongjae Park, Kisoo Oh, Joosung Lee, Ki Hoon Leiner, Jonathan C. Sim, Hasung Kim, Taehun Jeong, Jaehong Rule, Kirrily C. Kamazawa, Kazuya Iida, Kazuki Perring, T. G. Woo, Hyungje Cheong, S.-W. Zhitomirsky, M. E. Chernyshev, A. L. Park, Je-Geun Nat Commun Article Novel effects induced by nonmagnetic impurities in frustrated magnets and quantum spin liquid represent a highly nontrivial and interesting problem. A theoretical proposal of extended modulated spin structures induced by doping of such magnets, distinct from the well-known skyrmions has attracted significant interest. Here, we demonstrate that nonmagnetic impurities can produce such extended spin structures in h-YMnO(3), a triangular antiferromagnet with noncollinear magnetic order. Using inelastic neutron scattering (INS), we measured the full dynamical structure factor in Al-doped h-YMnO(3) and confirmed the presence of magnon damping with a clear momentum dependence. Our theoretical calculations can reproduce the key features of the INS data, supporting the formation of the proposed spin textures. As such, our study provides the first experimental confirmation of the impurity-induced spin textures. It offers new insights and understanding of the impurity effects in a broad class of noncollinear magnetic systems. Nature Publishing Group UK 2021-04-16 /pmc/articles/PMC8052335/ /pubmed/33863905 http://dx.doi.org/10.1038/s41467-021-22569-3 Text en © The Author(s) 2021 https://creativecommons.org/licenses/by/4.0/Open Access This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons license, and indicate if changes were made. The images or other third party material in this article are included in the article’s Creative Commons license, unless indicated otherwise in a credit line to the material. If material is not included in the article’s Creative Commons license and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this license, visit http://creativecommons.org/licenses/by/4.0/ (https://creativecommons.org/licenses/by/4.0/) .
spellingShingle Article
Park, Pyeongjae
Park, Kisoo
Oh, Joosung
Lee, Ki Hoon
Leiner, Jonathan C.
Sim, Hasung
Kim, Taehun
Jeong, Jaehong
Rule, Kirrily C.
Kamazawa, Kazuya
Iida, Kazuki
Perring, T. G.
Woo, Hyungje
Cheong, S.-W.
Zhitomirsky, M. E.
Chernyshev, A. L.
Park, Je-Geun
Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title_full Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title_fullStr Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title_full_unstemmed Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title_short Spin texture induced by non-magnetic doping and spin dynamics in 2D triangular lattice antiferromagnet h-Y(Mn,Al)O(3)
title_sort spin texture induced by non-magnetic doping and spin dynamics in 2d triangular lattice antiferromagnet h-y(mn,al)o(3)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8052335/
https://www.ncbi.nlm.nih.gov/pubmed/33863905
http://dx.doi.org/10.1038/s41467-021-22569-3
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