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Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)

The low-temperature scanning tunneling microscope and spectroscopy (STM/STS) are used to visualize superconducting states in the cleaved single crystal of 9% praseodymium-doped CaFe(2)As(2) (Pr-Ca122) with T(c) ≈ 30 K. The spectroscopy shows strong spatial variations in the density of states (DOS),...

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Autores principales: Nguyen, Giang D., Fu, Mingming, Zou, Qiang, Sanjeewa, Liurukara D., Li, An-Ping, Sefat, Athena S., Gai, Zheng
Formato: Online Artículo Texto
Lenguaje:English
Publicado: MDPI 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8074043/
https://www.ncbi.nlm.nih.gov/pubmed/33923517
http://dx.doi.org/10.3390/nano11041019
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author Nguyen, Giang D.
Fu, Mingming
Zou, Qiang
Sanjeewa, Liurukara D.
Li, An-Ping
Sefat, Athena S.
Gai, Zheng
author_facet Nguyen, Giang D.
Fu, Mingming
Zou, Qiang
Sanjeewa, Liurukara D.
Li, An-Ping
Sefat, Athena S.
Gai, Zheng
author_sort Nguyen, Giang D.
collection PubMed
description The low-temperature scanning tunneling microscope and spectroscopy (STM/STS) are used to visualize superconducting states in the cleaved single crystal of 9% praseodymium-doped CaFe(2)As(2) (Pr-Ca122) with T(c) ≈ 30 K. The spectroscopy shows strong spatial variations in the density of states (DOS), and the superconducting map constructed from spectroscopy discloses a localized superconducting phase, as small as a single unit cell. The comparison of the spectra taken at 4.2 K and 22 K (below vs. close to the bulk superconducting transition temperature) from the exact same area confirms the superconducting behavior. Nanoscale superconducting states have been found near Pr dopants, which can be identified using dI/dV conductance maps at +300 mV. There is no correlation of the local superconductivity to the surface reconstruction domain and surface defects, which reflects its intrinsic bulk behavior. We, therefore, suggest that the local strain of Pr dopants is competing with defects induced local magnetic moments; this competition is responsible for the local superconducting states observed in this Fe-based filamentary superconductor.
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spelling pubmed-80740432021-04-27 Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2) Nguyen, Giang D. Fu, Mingming Zou, Qiang Sanjeewa, Liurukara D. Li, An-Ping Sefat, Athena S. Gai, Zheng Nanomaterials (Basel) Article The low-temperature scanning tunneling microscope and spectroscopy (STM/STS) are used to visualize superconducting states in the cleaved single crystal of 9% praseodymium-doped CaFe(2)As(2) (Pr-Ca122) with T(c) ≈ 30 K. The spectroscopy shows strong spatial variations in the density of states (DOS), and the superconducting map constructed from spectroscopy discloses a localized superconducting phase, as small as a single unit cell. The comparison of the spectra taken at 4.2 K and 22 K (below vs. close to the bulk superconducting transition temperature) from the exact same area confirms the superconducting behavior. Nanoscale superconducting states have been found near Pr dopants, which can be identified using dI/dV conductance maps at +300 mV. There is no correlation of the local superconductivity to the surface reconstruction domain and surface defects, which reflects its intrinsic bulk behavior. We, therefore, suggest that the local strain of Pr dopants is competing with defects induced local magnetic moments; this competition is responsible for the local superconducting states observed in this Fe-based filamentary superconductor. MDPI 2021-04-16 /pmc/articles/PMC8074043/ /pubmed/33923517 http://dx.doi.org/10.3390/nano11041019 Text en © 2021 by the authors. https://creativecommons.org/licenses/by/4.0/Licensee MDPI, Basel, Switzerland. This article is an open access article distributed under the terms and conditions of the Creative Commons Attribution (CC BY) license (https://creativecommons.org/licenses/by/4.0/).
spellingShingle Article
Nguyen, Giang D.
Fu, Mingming
Zou, Qiang
Sanjeewa, Liurukara D.
Li, An-Ping
Sefat, Athena S.
Gai, Zheng
Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title_full Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title_fullStr Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title_full_unstemmed Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title_short Nanoscale Superconducting States in the Fe-Based Filamentary Superconductor of Pr-Doped CaFe(2)As(2)
title_sort nanoscale superconducting states in the fe-based filamentary superconductor of pr-doped cafe(2)as(2)
topic Article
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8074043/
https://www.ncbi.nlm.nih.gov/pubmed/33923517
http://dx.doi.org/10.3390/nano11041019
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