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Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear

The nature of yield in amorphous materials under stress has yet to be fully elucidated. In particular, understanding how microscopic rearrangement gives rise to macroscopic structural and rheological signatures in disordered systems is vital for the prediction and characterization of yield and the s...

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Autores principales: Teich, Erin G., Galloway, K. Lawrence, Arratia, Paulo E., Bassett, Danielle S.
Formato: Online Artículo Texto
Lenguaje:English
Publicado: American Association for the Advancement of Science 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8115929/
https://www.ncbi.nlm.nih.gov/pubmed/33980482
http://dx.doi.org/10.1126/sciadv.abe3392
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author Teich, Erin G.
Galloway, K. Lawrence
Arratia, Paulo E.
Bassett, Danielle S.
author_facet Teich, Erin G.
Galloway, K. Lawrence
Arratia, Paulo E.
Bassett, Danielle S.
author_sort Teich, Erin G.
collection PubMed
description The nature of yield in amorphous materials under stress has yet to be fully elucidated. In particular, understanding how microscopic rearrangement gives rise to macroscopic structural and rheological signatures in disordered systems is vital for the prediction and characterization of yield and the study of how memory is stored in disordered materials. Here, we investigate the evolution of local structural homogeneity on an individual particle level in amorphous jammed two-dimensional (athermal) systems under oscillatory shear and relate this evolution to rearrangement, memory, and macroscale rheological measurements. We define the structural metric crystalline shielding, and show that it is predictive of rearrangement propensity and structural volatility of individual particles under shear. We use this metric to identify localized regions of the system in which the material’s memory of its preparation is preserved. Our results contribute to a growing understanding of how local structure relates to dynamic response and memory in disordered systems.
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spelling pubmed-81159292021-05-19 Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear Teich, Erin G. Galloway, K. Lawrence Arratia, Paulo E. Bassett, Danielle S. Sci Adv Research Articles The nature of yield in amorphous materials under stress has yet to be fully elucidated. In particular, understanding how microscopic rearrangement gives rise to macroscopic structural and rheological signatures in disordered systems is vital for the prediction and characterization of yield and the study of how memory is stored in disordered materials. Here, we investigate the evolution of local structural homogeneity on an individual particle level in amorphous jammed two-dimensional (athermal) systems under oscillatory shear and relate this evolution to rearrangement, memory, and macroscale rheological measurements. We define the structural metric crystalline shielding, and show that it is predictive of rearrangement propensity and structural volatility of individual particles under shear. We use this metric to identify localized regions of the system in which the material’s memory of its preparation is preserved. Our results contribute to a growing understanding of how local structure relates to dynamic response and memory in disordered systems. American Association for the Advancement of Science 2021-05-12 /pmc/articles/PMC8115929/ /pubmed/33980482 http://dx.doi.org/10.1126/sciadv.abe3392 Text en Copyright © 2021 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works. Distributed under a Creative Commons Attribution NonCommercial License 4.0 (CC BY-NC). https://creativecommons.org/licenses/by-nc/4.0/This is an open-access article distributed under the terms of the Creative Commons Attribution-NonCommercial license (https://creativecommons.org/licenses/by-nc/4.0/) , which permits use, distribution, and reproduction in any medium, so long as the resultant use is not for commercial advantage and provided the original work is properly cited.
spellingShingle Research Articles
Teich, Erin G.
Galloway, K. Lawrence
Arratia, Paulo E.
Bassett, Danielle S.
Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title_full Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title_fullStr Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title_full_unstemmed Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title_short Crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
title_sort crystalline shielding mitigates structural rearrangement and localizes memory in jammed systems under oscillatory shear
topic Research Articles
url https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8115929/
https://www.ncbi.nlm.nih.gov/pubmed/33980482
http://dx.doi.org/10.1126/sciadv.abe3392
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