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Highly efficient, heat dissipating, stretchable organic light-emitting diodes based on a MoO(3)/Au/MoO(3) electrode with encapsulation

Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance...

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Detalles Bibliográficos
Autores principales: Choi, Dae Keun, Kim, Dong Hyun, Lee, Chang Min, Hafeez, Hassan, Sarker, Subrata, Yang, Jun Su, Chae, Hyung Ju, Jeong, Geon-Woo, Choi, Dong Hyun, Kim, Tae Wook, Yoo, Seunghyup, Song, Jinouk, Ma, Boo Soo, Kim, Taek-Soo, Kim, Chul Hoon, Lee, Hyun Jae, Lee, Jae Woo, Kim, Donghyun, Bae, Tae-Sung, Yu, Seung Min, Kang, Yong-Cheol, Park, Juyun, Kim, Kyoung-Ho, Sujak, Muhammad, Song, Myungkwan, Kim, Chang-Su, Ryu, Seung Yoon
Formato: Online Artículo Texto
Lenguaje:English
Publicado: Nature Publishing Group UK 2021
Materias:
Acceso en línea:https://www.ncbi.nlm.nih.gov/pmc/articles/PMC8128878/
https://www.ncbi.nlm.nih.gov/pubmed/34001906
http://dx.doi.org/10.1038/s41467-021-23203-y
Descripción
Sumario:Stretchable organic light-emitting diodes are ubiquitous in the rapidly developing wearable display technology. However, low efficiency and poor mechanical stability inhibit their commercial applications owing to the restrictions generated by strain. Here, we demonstrate the exceptional performance of a transparent (molybdenum-trioxide/gold/molybdenum-trioxide) electrode for buckled, twistable, and geometrically stretchable organic light-emitting diodes under 2-dimensional random area strain with invariant color coordinates. The devices are fabricated on a thin optical-adhesive/elastomer with a small mechanical bending strain and water-proofed by optical-adhesive encapsulation in a sandwiched structure. The heat dissipation mechanism of the thin optical-adhesive substrate, thin elastomer-based devices or silicon dioxide nanoparticles reduces triplet-triplet annihilation, providing consistent performance at high exciton density, compared with thick elastomer and a glass substrate. The performance is enhanced by the nanoparticles in the optical-adhesive for light out-coupling and improved heat dissipation. A high current efficiency of ~82.4 cd/A and an external quantum efficiency of ~22.3% are achieved with minimum efficiency roll-off.